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arXiv:1712.03117 · Physical Review Letters

Spin Polarization through Floquet Resonances in a Driven Central Spin Model

Pieter W. Claeys, Stijn De Baerdemacker, Omar El Araby, Jean-Sébastien Caux

Published Aug 21, 2018• 41 citations
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Abstract

Adiabatically varying the driving frequency of a periodically driven many-body quantum system can induce controlled transitions between resonant eigenstates of the time-averaged Hamiltonian, corresponding to adiabatic transitions in the Floquet spectrum and presenting a general tool in quantum many-body control. Using the central spin model as an application, we show how such controlled driving processes can lead to a polarization-based decoupling of the central spin from its decoherence-inducing environment at resonance. While it is generally impossible to obtain the exact Floquet Hamiltonian in driven interacting systems, we exploit the integrability of the central spin model to show how techniques from quantum quenches can be used to explicitly construct the Floquet Hamiltonian in a restricted many-body basis and model Floquet resonances.

DOI
10.1103/physrevlett.121.080401

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Adiabatically varying the driving frequency of a periodically driven many-body quantum system can induce controlled transitions between resonant eigenstates of the time-averaged Hamiltonian, corresponding to adiabatic transitions in the Floquet spectrum and presenting a general tool in quantum many-body control. Using the central spin model as an application, we show how such controlled driving processes can lead to a polarization-based decoupling of the central spin from its decoherence-inducing environment at resonance. While it is generally impossible to obtain the exact Floquet Hamiltonian in driven interacting systems, we exploit the integrability of the central spin model to show how techniques from quantum quenches can be used to explicitly construct the Floquet Hamiltonian in a restricted many-body basis and model Floquet resonances.
Periodically driven systems have emerged as a useful technique to engineer the properties of quantum systems, and are in the process of being developed into a standard toolbox for quantum simulation. An outstanding challenge that leaves this toolbox incomplete is the manipulation of the states dressed by strong periodic drives. The state-of-the-art in Floquet control is the adiabatic change of parameters. Yet, this requires long protocols conflicting with the limited coherence times in experiments. To achieve fast control of nonequilibrium quantum matter, we generalize the notion of variational counterdiabatic driving away from equilibrium focusing on Floquet systems. We derive a nonperturbative variational principle to find local approximations to the adiabatic gauge potential for the effective Floquet Hamiltonian. It enables transitionless driving of Floquet eigenstates far away from the adiabatic regime. We discuss applications to two-level, Floquet band, and interacting periodically driven models. The developed technique allows us to capture nonperturbative photon resonances and obtain high-fidelity protocols that respect experimental limitations like the locality of the accessible control terms.
Periodically driven quantum systems have emerged as one of the most versatile tools for quantum simulation, enabling the engineering of effective Hamiltonians, topological phases, and inherently nonequilibrium phenomena such as discrete time crystals. Yet fundamental challenges persist: from a spectral ambiguity that precludes a unique Floquet ground state to an inability to manipulate Floquet eigenstates beyond the adiabatic regime. This thesis demonstrates that counterdiabatic driving—a technique from adiabatic quantum control—provides a unifying framework to address these challenges. We first show that the periodic lab-frame Hamiltonian generates counterdiabatic driving for the Floquet eigenstates, revealing Floquet theory as an inverse counterdiabatic driving problem. Exploiting this equivalence, we develop geometric Floquet theory: a reformulation based on the parallel-transport gauge, which uniquely decomposes Floquet dynamics into a geometric contribution, encoded in Berry phases, and a dynamical contribution, generated by the average-energy operator. The average-energy operator provides an unambiguous sorting of the quasienergy spectrum, identifies a unique Floquet ground state at all drive frequencies, and serves as a sensitive diagnostic for heating and symmetry-breaking transitions. Inherently nonequilibrium phenomena—the 𝜋-quasienergy splitting of discrete time crystals and the anomalous edge modes of Floquet topological insulators—are traced to geometric phases. On the practical side, we exploit the intrinsic robustness of prethermal discrete time crystals for a highly frequency-selective DTC-based AC magnetic field sensing scheme and demonstrate it experimentally on a nuclear spin quantum simulator. We then generalize counterdiabatic driving to periodically driven systems. In particular, we derive a non-perturbative variational principle for the Floquet adiabatic gauge potential; this yields local, experimentally feasible control protocols for transitionless manipulation of Floquet states. We demonstrate this formalism on Floquet state preparation in an ultracold atom quantum simulator and many-body state transfer across a quantum phase transition, with significant improvements over unassisted protocols in both cases.
We study the fate of interacting quantum systems which are periodically driven by switching back and forth between two integrable Hamiltonians. This provides an unconventional and tunable way of breaking integrability, in the sense that the stroboscopic time evolution will generally be described by a Floquet Hamiltonian which progressively becomes less integrable as the driving frequency is reduced. Here, we exemplify this idea in spin chains subjected to periodic switching between two integrable anisotropic Heisenberg Hamiltonians. We distinguish the integrability-breaking effects of resonant interactions and perturbative (local) interactions, and illustrate these by contrasting different measures of energy in Floquet states and through a study of level spacing statistics. This scenario is argued to be representative for general driven interacting integrable systems.
Near-resonant periodic driving of quantum systems promises the implementation of a large variety of novel quantum states, though their preparation and measurement remains challenging. We address these aspects in a model system consisting of interacting fermions in a periodically driven array of double wells created by an optical lattice. The singlet and triplet fractions and the double occupancy of the Floquet states are measured and their behavior as a function of the interaction strength is analyzed in the high- and low-frequency regimes. We demonstrate full control of the Floquet state population and find suitable ramping protocols and time scales that adiabatically connect the initial ground state to different targeted Floquet states. The micromotion that exactly describes the time evolution of the system within one driving cycle is observed. Additionally, we provide an analytic description of the model and compare it to numerical simulations.
Controlling the decoherence induced by the interaction of quantum system with its environment is a fundamental challenge in quantum technology. Utilizing Floquet theory, we explore the constructive role of temporal periodic driving in suppressing decoherence of a spin-1/2 particle coupled to a spin bath. It is revealed that, accompanying the formation of a Floquet bound state in the quasienergy spectrum of the whole system including the system and its environment, the dissipation of the spin system can be inhibited and the system tends to coherently synchronize with the driving. It can be seen as an analog to the decoherence suppression induced by the structured environment in spatially periodic photonic crystal setting. Comparing with other decoherence control schemes, our protocol is robust against the fluctuation of control parameters and easy to realize in practice. It suggests a promising perspective of periodic driving in decoherence control.
Counterdiabatic (CD) driving presents a way of generating adiabatic dynamics at an arbitrary pace, where excitations due to nonadiabaticity are exactly compensated by adding an auxiliary driving term to the Hamiltonian. While this CD term is theoretically known and given by the adiabatic gauge potential, obtaining and implementing this potential in many-body systems is a formidable task, requiring knowledge of the spectral properties of the instantaneous Hamiltonians and control of highly nonlocal multibody interactions. We show how an approximate gauge potential can be systematically built up as a series of nested commutators, remaining well defined in the thermodynamic limit. Furthermore, the resulting CD driving protocols can be realized up to arbitrary order without leaving the available control space using tools from periodically driven (Floquet) systems. This is illustrated on few- and many-body quantum systems, where the resulting Floquet protocols significantly suppress dissipation and provide a drastic increase in fidelity.