Perfectly polarized, pure and mixed, quantum states of light are investigated. Using symmetry and geometry arguments, the canonical degree of polarization is reinterpreted, which can be used as a benchmark for applications where extremely precise experimental control of the polarization is required.
It takes some convincing to realize that light has a polarization degree of freedom, as our eyes are usually ignorant of light's polarization. Since overcoming this hurdle of intuition, polarization has become a fantastic resource that can be easily manipulated both physically and mathematically, opening the door to a wide variety of applications. We have only recently begun to appreciate how many more doors are opened by the quantum mechanical degrees of freedom inherent to optical polarization. One use of optical polarization is for polarimetry: measuring the changes in light's polarization after it interacts with a material is an excellent procedure for nondestructively probing the characteristics and composition of the intervening material. More sensitive measurements require brighter probe light; however, sufficiently intense light will begin to destroy the sample being probed. In this thesis, we seek to provide more sensitive polarimetry without resorting to bright beams of light. Tailoring the quantum properties of various states of light has been shown to increase their usefulness for other estimation protocols and we show how to extend this paradigm to quantum enhancements in polarimetry. We begin by finding the quantum states underlying classical polarization. Each particular set of classical polarization properties corresponds to a large variety of quantum states. Next, we establish quantum descriptions of classical polarization transformations corresponding to arbitrary Jones and Mueller matrices, including quantum mechanical insights into the distinction between processes that can and cannot be described by Jones matrices. We propose candidates for the most likely quantum states underlying classical decompositions into polarized and unpolarized fractions, carefully inspecting how these quantum states behave under polarization transformations. This language allows us to inspect quantum-enhanced sensing in the multiparameter context of polarimetry. We show the dramatic possibilities for quantum enhancements in any metrological scenario that is mathematically equivalent to a rotation, of which polarization rotations are a primary example; in contrast, we also show most attenuating and depolarizing polarization transformations to forbid such dramatic enhancements. Finally, we discuss polarization and its generalizations in the context of generating quantum entanglement via linear optics. These applications serve as mere examples of the usefulness promised by light’s quantum polarization degrees of freedom.
Classically entangled light is used to refer to a class of structured beams with space-polarization, polarization-time, and space-time non-separable states akin to entangled states, which enable novel quantum-analog methods and applications in structured light. Here, we argue that classical entanglement is also available for pure scalar beams with multiple non-separable spatial degrees of freedom (DoFs). We theoretically and experimentally demonstrate a class of scalar ray-wave structured light with multiple controllable local DoFs to emulate multipartite entangled states, including the Greenberger-Horne-Zeilinger states. Our work unveils a rich parameter space for high-dimensional and multi-DoF control of structured light to extend applications in classical-quantum regimes.
Inherent spin angular momentum (SAM) and orbital angular momentum (OAM), which manifest as polarization and spatial degrees of freedom (DOFs) of photons, hold a promise of large capability for applications in classical and quantum information processing. To enable these photonic spin and orbital dynamic properties strongly coupled with each other, Poincaré states have been proposed and offer advantages in data multiplexing, information encryption, precision metrology, and quantum memory. However, since the transverse size of Laguerre-Gaussian beams strongly depends on their topological charge numbers | l |, it is difficult to store asymmetric Poincaré states due to the significantly different light-matter interaction for distinct spatial modes. Here, we experimentally realize the storage of perfect Poincaré states with arbitrary OAM quanta using the perfect optical vortex, in which 121 arbitrarily selected perfect Poincaré states have been stored with high fidelity. The reported work has great prospects in optical communication and quantum networks for dramatically increased encoding flexibility of information.
Quantum polarization is an important property that has been extensively used for quantum communication purposes. In this work, the mixture of an unpolarized two-mode state and a two-mode pure state is analysed. This mixture is controlled by a single parameter, namely the degree of purity. The quantum polarization of the two-mode mixed state is discussed using the quantum Stokes parameters and the quantum degree of polarization. A relation between the degree of purity and the quantum degree of polarization is established. The mixture is used to model coherent light amplified by an erbium-doped fibre amplifier, which focuses the loss of polarization due to the unpolarized light resulting from spontaneous emission. Finally, the use of such a mixed state in the quantum key distribution using multiphoton pulses is analysed.