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arXiv:1709.02553 · Physical review. B./Physical review. B

Enhanced superconducting fluctuation effects on thermodynamic properties in the BCS-BEC crossover regime

Kyosuke Adachi, Ryusuke Ikeda

Published Nov 8, 2017• 6 citations
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Abstract

The effects of superconducting fluctuation (SCF) on the thermodynamic properties of electron systems in the so-called BCS-BEC crossover regime are studied. As the attractive interaction between electrons becomes stronger upon approaching the BCS-BEC crossover regime, the importance of the mode coupling between SCF drastically increases. The enhanced mode coupling leads to lowering of both the zero-field superconducting critical temperature and the depairing field ${B}_{\text{c2}}(T)$. Consequently, SCF-induced contributions to the specific heat and the diamagnetic susceptibility can seemingly exceed the corresponding values in the Gaussian approximation. We discuss the relevance of the present results to the anomalous SCF-induced diamagnetic response observed in the iron selenide (FeSe).

DOI
10.1103/physrevb.96.184507

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The effects of superconducting fluctuation (SCF) on the thermodynamic properties of electron systems in the so-called BCS-BEC crossover regime are studied. As the attractive interaction between electrons becomes stronger upon approaching the BCS-BEC crossover regime, the importance of the mode coupling between SCF drastically increases. The enhanced mode coupling leads to lowering of both the zero-field superconducting critical temperature and the depairing field Bc2(T){B}_{\text{c2}}(T)Bc2​(T). Consequently, SCF-induced contributions to the specific heat and the diamagnetic susceptibility can seemingly exceed the corresponding values in the Gaussian approximation. We discuss the relevance of the present results to the anomalous SCF-induced diamagnetic response observed in the iron selenide (FeSe).
We investigate the dynamical effects of pairing interaction on superconductivity in BCS-BEC crossover by studying the Holstein model at half filling where the electron-phonon coupling ggg controls the crossover. The dynamical mean-field theory was employed in combination with the numerical renormalization group technique to study the frequency dependence of phonon mediated interaction between electrons in a superconductive state. The frequency dependence induces distinct features such as the absence of the dispersion back bending of Bogoliubov quasiparticles, nonmonotonous coupling dependence of the pairing gap, and the critical temperature Tc{T}_{c}Tc​ being maximum at gc1{g}_{c1}gc1​, the lower critical coupling of the normal state insulator to metal transition. Some of these features have intriguing similarities with the recent observations in the ${\mathrm{FeSe}}_{1\ensuremath{-}x}{\mathrm{S}}_{x}$ and ${\mathrm{Fe}}_{1+y}{\mathrm{Se}}_{x}{\mathrm{Te}}_{1\ensuremath{-}x}$ iron chalcogenides in the BCS-BEC crossover.
Nonadiabatic effects in the electron-phonon coupling are important whenever the ratio between the phononic and the electronic energy scales---the adiabatic ratio---is non-negligible. For superconducting systems, this gives rise to additional diagrams in the superconducting self-energy, the vertex, and cross-corrections. In this work, we explore these corrections in a two-dimensional single-band system through the crossover between the weak-coupling Bardeen-Cooper-Schrieffer (BCS) and strong-coupling Bose-Einstein regimes. By focusing on the pseudogap phase, we identify the parameter range in which the pairing amplitude is amplified by nonadiabatic effects and, due to controlled approximations, we map them throughout the BCS-BEC crossover. These effects become stronger as the system is driven deeply in the crossover regime, for phonon frequencies of the order of the hopping energy and for large enough electron-phonon coupling. Finally, we provide the phase space regions in which the effects of nonadiabaticity are more relevant for unconventional superconductors.
Fermi systems in the cross-over regime between weakly coupled Bardeen-Cooper-Schrieffer (BCS) and strongly coupled Bose-Einstein-condensate (BEC) limits are among the most fascinating objects to study the behavior of an assembly of strongly interacting particles. The physics of this cross-over has been of considerable interest both in the fields of condensed matter and ultracold atoms. One of the most challenging issues in this regime is the effect of large spin imbalance on a Fermi system under magnetic fields. Although several exotic physical properties have been predicted theoretically, the experimental realization of such an unusual superconducting state has not been achieved so far. Here we show that pure single crystals of superconducting FeSe offer the possibility to enter the previously unexplored realm where the three energies, Fermi energy εF, superconducting gap Δ, and Zeeman energy, become comparable. Through the superfluid response, transport, thermoelectric response, and spectroscopic-imaging scanning tunneling microscopy, we demonstrate that εF of FeSe is extremely small, with the ratio Δ/εF ~ 1(~0.3) in the electron (hole) band. Moreover, thermal-conductivity measurements give evidence of a distinct phase line below the upper critical field, where the Zeeman energy becomes comparable to εF and Δ. The observation of this field-induced phase provides insights into previously poorly understood aspects of the highly spin-polarized Fermi liquid in the BCS-BEC cross-over regime.
We theoretically investigate the specific heat at constant volume C V in the BCS(Bardeen-Cooper-Schrieffer)-BEC(Bose-Einstein-condensation)-crossover regime of an ultracold Fermi gas, below the superfluid phase transition temperature T c . Within the strong-coupling framework developed by Nozières and Schmitt-Rink, we show that the temperature dependence of C V drastically changes as one passes through the crossover region, and is sensitive to strong fluctuations in the Cooper channel near the unitarity limit. We also compare our results to a recent experiment on a 6 Li unitary Fermi gas. Since fluctuation effects are a crucial key in the BCS-BEC-crossover phenomenon, our results would be helpful in considering how the fermionic BCS superfluid changes into BEC with increasing the interaction strength, from the viewpoint of specific heat.
The appearance of a shallow band(s) drives a superconductor towards the BCS-BEC crossover, conventionally associated with notable changes in single-particle properties and an elevated critical temperature. Here we demonstrate that the proximity to the crossover induced by a shallow band has also a dramatic effect on the phase diagram of the superconducting magnetic properties. When the system passes from the BCS to BEC regime, the intertype domain between superconductivity types I and II enlarges systematically, being inversely proportional to the square of the Cooper-pair radius, the main parameter that controls the BCS-BEC superconductivity. We also show that despite the presence of a shallow band, the condensate fluctuations are suppressed when it coexists in one material with standard deep bands, as in recent iron chalcogenides ${\mathrm{Fe}\mathrm{Se}}_{x}{\mathrm{Te}}_{1\ensuremath{-}x}$ and FeSe\mathrm{FeSe}FeSe.
The BCS-BEC crossover is studied in a systematic way in the broken-symmetry phase between zero temperature and the critical temperature. This study bridges two regimes where quantum and thermal fluctuations are, respectively, important. The theory is implemented on physical grounds, by adopting a fermionic self-energy in the broken-symmetry phase that represents fermions coupled to superconducting fluctuations in weak coupling and to bosons described by the Bogoliubov theory in strong coupling. This extension of the theory beyond mean field proves important at finite temperature, to connect with the results in the normal phase. The order parameter, the chemical potential, and the single-particle spectral function are calculated numerically for a wide range of coupling and temperature. This enables us to assess the quantitative importance of superconducting fluctuations in the broken-symmetry phase over the whole BCS-BEC crossover. Our results are relevant to the possible realizations of this crossover with high-temperature cuprate superconductors and with ultracold fermionic atoms in a trap.