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arXiv:1707.09559

EIT-Enhanced Coupled-Resonance Spectroscopy

Junyi Zhang

Published Jul 29, 2017• 0 citations
arXivHTMLPDF

Abstract

Coupled-resonance spectroscopy has been recently reported and applied for spectroscopic measurements and laser stabilizations. With coupled-resonance spectroscopy, one may indirectly measure some transitions between the excited states that are hard to be measured directly because of the lack of populations in the excited states. An improvement of the coupled-resonance spectroscopy by combining the technology of electromagnetically induced transparency (EIT) is proposed. The coupled-resonance spectroscopy signal can be significantly enhanced by EIT. Several experimental schemes have been discussed. The line shape of the EIT-enhanced coupled-resonance spectroscopy has been calculated.The EIT-enhanced coupled-resonance spectroscopy can be used for simultaneously stabilizing two lasers to the same atomic source.

DOI
10.48550/arxiv.1707.09559

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Coupled-resonance spectroscopy has been recently reported and applied for spectroscopic measurements and laser stabilizations. With coupled-resonance spectroscopy, one may indirectly measure some transitions between the excited states that are hard to be measured directly because of the lack of populations in the excited states. An improvement of the coupled-resonance spectroscopy by combining the technology of electromagnetically induced transparency (EIT) is proposed. The coupled-resonance spectroscopy signal can be significantly enhanced by EIT. Several experimental schemes have been discussed. The line shape of the EIT-enhanced coupled-resonance spectroscopy has been calculated.The EIT-enhanced coupled-resonance spectroscopy can be used for simultaneously stabilizing two lasers to the same atomic source.
Laser spectroscopy experiments are reported on rubidium atoms by using two or three external cavity diode lasers to study multiple resonance transitions in Λ- and V-type systems as well as on (Λ+V)-type system. Electromagnetically induced transparency (EIT) peaks having sub-natural line-widths are found on the Doppler broadened transmission backgrounds with velocity selective enhanced absorption dips. In the presence of a pump laser, probe spectrum shows enhancement of EIT signal by tuning the control laser frequency when the Λ- and V-type EIT signals are made to overlap. Theoretical analysis is carried out by solving the optical Bloch equations for five-level atomic model under Λ configuration. With the numerically simulated spectra, variation of EIT transmission peak with ground state decay rate and excited state spontaneous decay rate are investigated. Effect of pump Rabi frequency on the transmission peak is also shown.
We use the phenomenon of electromagnetically induced transparency in a three-level atomic system for hyperfine spectroscopy of upper states that are not directly coupled to the ground state. The three levels form a ladder system: the probe laser couples the ground state to the lower excited state, while the control laser couples the two upper states. As the frequency of the control laser is scanned, the probe absorption shows transparency peaks whenever the control laser is resonant with a hyperfine level of the upper state. As an illustration of the technique, we measure hyperfine structure in the 7 S 1/2 states of 85 Rb and 87 Rb, and obtain an improvement of more than an order of magnitude over previous values.
Following our previous brief report [Phys. Rev. Lett. 88, 173003 (2002)], we report here a detailed study of electromagnetically induced transparency (EIT) and dark fluorescence in a cascade three-level diatomic lithium system using optical-optical double resonance (OODR) spectroscopy for both resonance and off resonance coupling. When a strong coupling laser couples the intermediate state $A\phantom{\rule{0.2em}{0ex}}^{1}\ensuremath{\Sigma}_{u}^{+}(v=13,J=14)$ to the upper state $G\phantom{\rule{0.2em}{0ex}}^{1}\ensuremath{\Pi}_{g}(v=11,J=14)$ of 7Li2^{7}\mathrm{Li}_{2}7Li2​, the fluorescence from both $A\phantom{\rule{0.2em}{0ex}}^{1}\ensuremath{\Sigma}_{u}^{+}$ and $G\phantom{\rule{0.2em}{0ex}}^{1}\ensuremath{\Pi}_{g}$ states was drastically reduced as the weak probe laser was tuned through the resonance transition between the ground state $X\phantom{\rule{0.2em}{0ex}}^{1}\ensuremath{\Sigma}_{g}^{+}(v=4,J=15)$ and the excited state $A\phantom{\rule{0.2em}{0ex}}^{1}\ensuremath{\Sigma}_{u}^{+}(v=13,J=14)$. The strong coupling laser makes an optically thick medium transparent for the probe transition. In addition, the fact that fluorescence from the upper state $G\phantom{\rule{0.2em}{0ex}}^{1}\ensuremath{\Pi}_{g}(v=11,J=14)$ was also dark when both lasers were tuned at resonance implies that the molecules were trapped in the ground state. We used density matrix methods to simulate the response of an open molecular three-level system to the action of a strong coupling field and a weak probe field. The analytical solutions were obtained under the steady-state condition. We have incorporated the magnetic sublevel (M)(M)(M) degeneracy of the rotational levels in the line shape analysis and report $\ensuremath{\mid}M\ensuremath{\mid}$ dependent line shape splitting. Our theoretical calculations are in excellent agreement with the observed fluorescence spectra. We show that the coherence is remarkably preserved even when the coupling field was detuned far from the resonance.
Electromagnetically induced transparency (EIT) is a well-known phenomenon due in part to its applicability to quantum devices such as quantum memories and quantum gates. EIT is commonly modeled with a three-level lambda system; however, this simplified model does not capture all the physics of EIT experiments with real systems. We present a theoretical study of the effect of two closely-spaced excited states on EIT and off-resonance Raman transitions. In addition to the expected broadening of the EIT resonance and reduction in EIT transparency due to multiple excited states, we find some unexpected and interesting results. A comparison with a model that does not allow for coupling of the excited states shows that the coherent interaction of the fields with two excited states whose separation is smaller than their Doppler broadened linewidth can enhance the EIT transparency under some conditions and can enhance and shift the resonance frequency of off-resonance Raman absorption. Furthermore, through a dressed state analysis of the full four-level system, we find that the underlying mechanism for the reduction in EIT transparency is a shift in the two-photon resonance due to unequal dipole moments of the transitions coupled by the control field. Complete transparency can only be recovered for systems with equal dipole moments or when the separation between the two excited states is at least of the order of the Doppler width. To support our theoretical study, we present experimental EIT measurements in the D1 lines of 85Rb and 87Rb that agree with our predictions of an enhancement or reduction of EIT transparency under specific conditions. The experimental results also verify the roles that the dipole moments and the separation between the two excited states have on recovering the EIT transparency.
Frequency locking to reference atomic lines using Rydberg electromagnetically induced transparency (EIT) has been recently introduced as an inexpensive and reliable technique for laser frequency stabilization. In this work, we carry out a systematic study of this technique using heterodyne beat spectroscopy. Two different commercial semi-conductor lasers are locked to the same reference frequency using EIT locking, and their relative frequency stability is analyzed and continuously monitored in real time. A substantial improvement in the laser frequency stability is achieved through searching for the optimal proportional–integral settings and EIT probe laser powers. The results show that the cutoff frequency of the beat signal can be lowered to less than 500 kHz. We also compare the frequencies of free running lasers with that of a locked laser and characterize their frequency drifts. This study is important in assessing the use of Rydberg EIT locking in atomic electrometers.