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arXiv:1706.03077 · Atoms

Decoherence in Excited Atoms by Low-Energy Scattering

Diego Quiñones, Benjamin Varcoe

Published Dec 9, 2016• 3 citations
arXivHTMLPDF

Abstract

We describe a new mechanism of decoherence in excited atoms as a result of thermal particles scattering by the atomic nucleus. It is based on the idea that a single scattering will produce a sudden displacement of the nucleus, which will be perceived by the electron in the atom as an instant shift in the electrostatic potential. This will leave the atom’s wave-function partially projected into lower-energy states, which will lead to decoherence of the atomic state. The decoherence is calculated to increase with the excitation of the atom, making observation of the effect easier in Rydberg atoms. We estimate the order of the decoherence for photons and massive particles scattering, analyzing several commonly presented scenarios. Our scheme can be applied to the detection of weakly-interacting particles, like those which may be the constituents of Dark Matter, the interaction of which was calculated to have a more prominent effect that the background radiation.

DOI
10.3390/atoms4040028

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Decoherence in Excited Atoms by Low-Energy Scattering

Quiñones, DA, Varcoe, BTH

We describe a new mechanism of decoherence in excited atoms that arise from particle scattering by the atomic nucleus. It is based on the idea that the scattering will produce a sudden displacement of the nucleus which will be perceived by the electron of the atom as an instant shift in the electrostatic potential. This will leave the atom’s wavefunction partially projected into lower-energy states which will lead to the decoherence of the atomic state. The decoherence is calculated to increase with the excitation of the atom, making observations of the effect easier in Rydberg atoms. We estimate the order of the decoherence for photons and massive particles scattering, analyzing several commonly presented scenarios. By maximizing the order of the effect it can be used for detection of weakly-interacting particles, like those which may be the constituents of Dark Matter, through applying very precise atomic spectroscopy.

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Tara Cubel Liebisch, Michael Schlagmüller, Felix Engel +8 more

A single Rydberg atom impurity excited in a BEC is a system that can be utilized to measure the quantum mechanical properties of electron - neutral scattering andthe electron probability density of a Rydberg atom. The Rydberg electron – neutral atom scattering process, is a fundamental scattering process, which can be described via Fermi’s pseudopotential as V{vec{r},vec{R} )=2pi textit{a}[k(R)]delta^{(3)}(vec{r}-vec{R}). The scattering length is dependent on the momentum of the Rydberg electron, and therefore is dependent on the separation of the Rydberg electron from the ion core. At the classical outermost turning point of the electron, it has the slowest momentum leading to s-wave dominated scattering potentials 10’s of MHz in depth for n<40 (Greene et al. PRL 85 2458 (2000), Bendkowsky et al. PRL 105 163201 (2010)). In alkali atoms there is a shape resonance for p-wave scattering, which becomes relevant at ion-neutral separations of ~75nm (I.I. Fabrikant J.Phys B 19, 1527 (1985)). This shape resonance potential is several GHz deep, spanning the energy level spacing between n and n-1 principal quantum numbers. At high BEC densities of 5x10^14cm-3 the nearest neighbor spacing is less than 70nm. A Rydberg atom excited within a BEC, is an excitation of the Rydberg atom and all N neutral atoms located within the Rydberg orbit, described as nS+N x 5S. The nS+N x 5S state is density shifted from the Rydberg resonance. Not only does the distribution of atoms within the Rydberg orbit lead to a density shift, but, at these high densities, atoms excited in the nS+N x 5S state near the shape resonance potential cause large perturbations to the density shift, leading to a line broadening. Therefore the spectroscopic line shape of a Rydberg atom in a BEC allows us to probe the theoretically calculated p-wave shape resonance potential. Furthermore, we can observe and measure the dynamics of neutrals excited in the nS+N x 5S state. In the ultracold regime of a BEC, the background neutral atoms within the Rydberg orbit have kinetic energies of a few kHz, and experience large forces due to the GHz-deep shape resonance potentials. An atom dragged into this deep potential leads to an exothermic state-changing collision. We measure the timescale of this state-changing collision and compare to semi-classical calculations of the neutral atoms evolving in the potential of the two-particle nS+ 5S system. We also measure the change in energy from the original nS state to the product state, (n-4)L (L<3). On time scales shorter than the state-changing collisions, which for n<100 is on the order of 10 microseconds, the neutral atoms will evolve and collect in the shallower electron-neutral potentials, which mimic the electron probability density of the Rydberg atom.With n<100, the Rydberg atom has a diameter greater than 2 micrometers. With an imaging system with <1 micrometer resolution, we expect to observe a macroscopic change in the density profile of the BEC indicating an nS versus nD Rydberg state. The BEC would serve as a contrast agent for observing textbook atomic wavefunctions (Karpiuk et al. New Journal of Physics 17, 053046 (2015)).

•Aug 3, 2016•0 citations
We describe a new mechanism of decoherence in excited atoms as a result of thermal particles scattering by the atomic nucleus. It is based on the idea that a single scattering will produce a sudden displacement of the nucleus, which will be perceived by the electron in the atom as an instant shift in the electrostatic potential. This will leave the atom’s wave-function partially projected into lower-energy states, which will lead to decoherence of the atomic state. The decoherence is calculated to increase with the excitation of the atom, making observation of the effect easier in Rydberg atoms. We estimate the order of the decoherence for photons and massive particles scattering, analyzing several commonly presented scenarios. Our scheme can be applied to the detection of weakly-interacting particles, like those which may be the constituents of Dark Matter, the interaction of which was calculated to have a more prominent effect that the background radiation.
We describe a new mechanism of decoherence in excited atoms that arise from particle scattering by the atomic nucleus. It is based on the idea that the scattering will produce a sudden displacement of the nucleus which will be perceived by the electron of the atom as an instant shift in the electrostatic potential. This will leave the atom’s wavefunction partially projected into lower-energy states which will lead to the decoherence of the atomic state. The decoherence is calculated to increase with the excitation of the atom, making observations of the effect easier in Rydberg atoms. We estimate the order of the decoherence for photons and massive particles scattering, analyzing several commonly presented scenarios. By maximizing the order of the effect it can be used for detection of weakly-interacting particles, like those which may be the constituents of Dark Matter, through applying very precise atomic spectroscopy.
We present a new model of atomic decoherence by space-time perturbations. We propose that decoherence will arise as a result of two possible effects that gravitational fluctuations will have on the atom. One is that the nucleus will be displaced relative to the valence electron, which will be perceived as a sudden change in the electric potential. This will result in the wave function of the atom being partially projected into lower energy levels. The other is that the strain in space will change the local electric field as felt by the electron. This interaction will either induce a change in the angular momentum of the atom or a small shift in the transition of the energy levels, presenting two different experimental approaches for the detection of the effect. We calculate how the decoherence is related to the internal degrees of freedom of the atoms, obtaining that the effect will be more prominent for atoms initially in a highly excited state (Rydberg atoms). By applying the nuclear displacement model for the scatter- ing of neutral particles, we suggest that it could be potentially useful for the detection of weakly-interacting particles, like possible candi- dates of Dark Matter. The overall effect of gravitational waves for the strained-space model was calculated to be several orders of magnitude higher than for the nuclear displacement model, allowing for detection in different ranges of frequencies. We analyze how different quantum states are affected according to the proposed model, calculating that the information from the measurement of correlated atoms will be significantly higher. The optimal quantum state that minimizes the uncertainty of the measurement is described for an arbitrary number of atoms, giving a relation that follows closely the Heisenberg limit.
A new heuristic model of interaction of an atomic system with a gravitational wave (GW) is proposed. In it, the GW alters the local electromagnetic field of the atomic nucleus, as perceived by the electron, changing the state of the system. The spectral decomposition of the wave function is calculated, from which the energy is obtained. The results suggest a shift in the difference of the atomic energy levels, which will induce a small detuning to a resonant transition. The detuning increases with the quantum numbers of the levels, making the effect more prominent for Rydberg states. We performed calculations on the Rabi oscillations of atomic transitions, estimating how they would vary as a result of the proposed effect.
The conventional notion of elastic, coherent atom-surface scattering originates from the scattering particles acting as a quantum-mechanical matter wave, which coherently interfere to produce distinct Bragg peaks which persist at finite temperature. If we introduce inelastic scattering to this scenario, the result is that the surface particles become displaced by the scattering atoms, resulting in emission or absorption of phonons that shift the final energy and momentum of the scatterer. As the lowest-lying phonons are gapless excitations, the ability to measure these phonons is very difficult and this difficulty is exacerbated by the roughly 1-eV resolution found in high-energy helium scattering experiments. Even though the surface has in effect measured the presence of the scatterer which decoheres the particle, we retain the diffraction spots which are referred to as coherent scattering. How do we reconcile these disparate viewpoints? We propose an experiment to more precisely examine the question of coherence in atom-surface scattering. We begin with an initially coherent superposition of helium particles with equal probabilities of interacting with the surface or not interacting with the surface. The beams are directed so that after the scattering event, the atoms are recombined so that we can observe the resulting interference pattern. The degree to which phonons are excited in the lattice by the scattering process dictates the fringe contrast of the interference pattern of the resulting beams. We use semiclassical techniques to simulate and test the viability of this experiment and show that for a wide range of conditions, despite the massive change in the momentum perpendicular to the surface, we can still expect to have coherent (in the superposition sense) scattering.
Abstract A new heuristic model of interaction of an atomic system with a gravitational wave (GW) is proposed. In it, the GW alters the local electromagnetic field of the atomic nucleus, as perceived by the electron, changing the state of the system. The spectral decomposition of the wave function is calculated, from which the energy is obtained. The results suggest a shift in the difference of the atomic energy levels, which will induce a small detuning to a resonant transition. The detuning increases with the quantum numbers of the levels, making the effect more prominent for Rydberg states. We performed calculations on the Rabi oscillations of atomic transitions, estimating how they would vary as a result of the proposed effect.
A single Rydberg atom impurity excited in a BEC is a system that can be utilized to measure the quantum mechanical properties of electron - neutral scattering andthe electron probability density of a Rydberg atom. The Rydberg electron – neutral atom scattering process, is a fundamental scattering process, which can be described via Fermi’s pseudopotential as V{vec{r},vec{R} )=2pi textit{a}[k(R)]delta^{(3)}(vec{r}-vec{R}). The scattering length is dependent on the momentum of the Rydberg electron, and therefore is dependent on the separation of the Rydberg electron from the ion core. At the classical outermost turning point of the electron, it has the slowest momentum leading to s-wave dominated scattering potentials 10’s of MHz in depth for n<40 (Greene et al. PRL 85 2458 (2000), Bendkowsky et al. PRL 105 163201 (2010)). In alkali atoms there is a shape resonance for p-wave scattering, which becomes relevant at ion-neutral separations of ~75nm (I.I. Fabrikant J.Phys B 19, 1527 (1985)). This shape resonance potential is several GHz deep, spanning the energy level spacing between n and n-1 principal quantum numbers. At high BEC densities of 5x10^14cm-3 the nearest neighbor spacing is less than 70nm. A Rydberg atom excited within a BEC, is an excitation of the Rydberg atom and all N neutral atoms located within the Rydberg orbit, described as nS+N x 5S. The nS+N x 5S state is density shifted from the Rydberg resonance. Not only does the distribution of atoms within the Rydberg orbit lead to a density shift, but, at these high densities, atoms excited in the nS+N x 5S state near the shape resonance potential cause large perturbations to the density shift, leading to a line broadening. Therefore the spectroscopic line shape of a Rydberg atom in a BEC allows us to probe the theoretically calculated p-wave shape resonance potential. Furthermore, we can observe and measure the dynamics of neutrals excited in the nS+N x 5S state. In the ultracold regime of a BEC, the background neutral atoms within the Rydberg orbit have kinetic energies of a few kHz, and experience large forces due to the GHz-deep shape resonance potentials. An atom dragged into this deep potential leads to an exothermic state-changing collision. We measure the timescale of this state-changing collision and compare to semi-classical calculations of the neutral atoms evolving in the potential of the two-particle nS+ 5S system. We also measure the change in energy from the original nS state to the product state, (n-4)L (L<3). On time scales shorter than the state-changing collisions, which for n<100 is on the order of 10 microseconds, the neutral atoms will evolve and collect in the shallower electron-neutral potentials, which mimic the electron probability density of the Rydberg atom.With n<100, the Rydberg atom has a diameter greater than 2 micrometers. With an imaging system with <1 micrometer resolution, we expect to observe a macroscopic change in the density profile of the BEC indicating an nS versus nD Rydberg state. The BEC would serve as a contrast agent for observing textbook atomic wavefunctions (Karpiuk et al. New Journal of Physics 17, 053046 (2015)).