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arXiv:1705.06673 · Physical Review Letters

Quantum Emitters in Two-Dimensional Structured Reservoirs in the Nonperturbative Regime

Alejandro González-Tudela, J. I. Cirac

Published Oct 4, 2017• 119 citations
arXivHTMLPDF

Abstract

We show that the coupling of quantum emitters to a two-dimensional reservoir with a simple band structure gives rise to exotic quantum dynamics with no analogue in other scenarios and which cannot be captured by standard perturbative treatments. In particular, for a single quantum emitter with its transition frequency in the middle of the band, we predict an exponential relaxation at a rate different from that predicted by Fermi's golden rule, followed by overdamped oscillations and slow relaxation decay dynamics. This is accompanied by directional emission into the reservoir. This directionality leads to a modification of the emission rate for few emitters and even perfect subradiance, i.e., suppression of spontaneous emission, for four quantum emitters.

DOI
10.1103/physrevlett.119.143602

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We show that the coupling of quantum emitters to a two-dimensional reservoir with a simple band structure gives rise to exotic quantum dynamics with no analogue in other scenarios and which cannot be captured by standard perturbative treatments. In particular, for a single quantum emitter with its transition frequency in the middle of the band, we predict an exponential relaxation at a rate different from that predicted by Fermi's golden rule, followed by overdamped oscillations and slow relaxation decay dynamics. This is accompanied by directional emission into the reservoir. This directionality leads to a modification of the emission rate for few emitters and even perfect subradiance, i.e., suppression of spontaneous emission, for four quantum emitters.
The interaction of quantum emitters with structured baths modifies both their individual and collective dynamics. In A. Gonz\'alez-Tudela and J. I. Cirac, Phys. Rev. Lett. 119, 143602 (2017), we show how exotic quantum dynamics emerges when quantum emitters are spectrally tuned around the middle of the band of a two-dimensional structured reservoir, where we predict the failure of perturbative treatments, anisotropic non-Markovian interactions, and remarkable superradiant and subradiant behavior. In this work, we provide further analysis of that situation, together with a complete analysis for the quantum emitter dynamics in spectral regions different from the center of the band.
Spontaneous emission of a quantum emitter, such as an excited atom, is a fundamental process in quantum electrodynamics (QED), typically associated with exponential decay to the ground state accompanied by irreversible photon emission. This simple Markovian picture, however, is profoundly modified in the presence of time-delayed feedback, structured continua, or cooperative emission, as occurs when an emitter radiates in front of a mirror, when several emitters radiate collectively, or in the case of a giant atom. In such regimes, strong non-Markovian dynamics arise from photon reabsorption and interference effects, leading to pronounced deviations from exponential decay. Here we demonstrate the emergence of exceptional points (EPs) in these highly non-Markovian waveguide-QED environments, i.e., non-Markovian EPs. These EPs appear directly in the relaxation dynamics as sharp transitions to oscillatory behavior, manifested by the appearance of real zeros in the excited-state amplitude. We analyze in detail the spontaneous emission of giant atoms with two or more coupling points, highlighting the mechanisms leading to non-Markovian EPs, and show that similar phenomena arise in other waveguide-QED settings, such as the collective spontaneous emission of spatially separated point-like emitters. Our results reveal waveguide-QED systems as experimentally accessible platforms for realizing and exploring non-Markovian EP physics.
In this work we study the quantum dynamics emerging when quantum emitters exchange excitations with a two-dimensional bosonic bath with a Dirac cone dispersion. We show that a single quantum emitter spectrally tuned in the vicinity of the Dirac point relaxes following a logarithmic law in time. Moreover, when several emitters are coupled to the bath at that frequency, long-range coherent interactions between them appear which decay inversely proportional to their distance without exponential attenuation. We analyze both the finite and infinite system situation using both perturbative and nonperturbative methods.
The resonant quantum dynamics of an excited two-level emitter is investigated via classical modulation of its transition frequency while simultaneously the radiator interacts with a broadband electromagnetic field reservoir. The frequency of modulation is selected to be of the order of the bare-state spontaneous decay rate. In this way, one can induce quantum interference effects, and consequently, quantum coherences among multiple decaying transition pathways. Depending on the modulation depth and its absolute phase, both the spontaneous emission and the frequency shift may be conveniently modified and controlled.
Spontaneous emission is one of the most fundamental out-of-equilibrium processes in which an excited quantum emitter relaxes to the ground state due to quantum fluctuations. In this process, a photon is emitted that can interact with other nearby emitters and establish quantum correlations between them, e.g., via super and subradiance effects. One way to modify these photon-mediated interactions is to alter the dipole radiation patterns of the emitter, e.g., by placing photonic crystals near them. One recent example is the generation of strong directional emission patterns-key to enhancing super and subradiance effects-in two dimensions by employing photonic crystals with band structures characterized by linear isofrequency contours and saddle-points. However, these studies have predominantly used oversimplified toy models, overlooking the electromagnetic field's intricacies in actual materials, including aspects like geometrical dependencies, emitter positions, and polarization. Our study delves into the interaction between these directional emission patterns and the aforementioned variables, revealing the untapped potential to fine-tune collective quantum optical phenomena.
Spontaneous emission is one of the most fundamental out-of-equilibrium processes in which an excited quantum emitter relaxes to the ground state due to quantum fluctuations. In this process, a photon is emitted that can interact with other nearby emitters and establish quantum correlations between them, e.g., via super and subradiance effects. One way to modify these photon-mediated interactions is to alter the dipole radiation patterns of the emitter, e.g., by placing photonic crystals near them. One recent example is the generation of strong directional emission patterns - key to enhancing super and subradiance effects - in two dimensions by employing photonic crystals with band structures characterized by linear isofrequency contours and saddle points. However, these studies have predominantly used oversimplified toy models, overlooking the electromagnetic field's intricacies in actual materials, including aspects like geometrical dependencies, emitter positions, and polarization. Our study delves into the interaction between these directional emission patterns and the variables mentioned above, revealing the untapped potential to fine-tune collective quantum optical phenomena.