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arXiv:1704.08245 · Physical Review A

Dynamics of bad-cavity-enhanced interaction with cold Sr atoms for laser stabilization

Stefan Alaric Schäffer, Bjarke T. R. Christensen, Martin R. Henriksen, Jan W. Thomsen

Published Jul 24, 2017• 23 citations
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Abstract

Hybrid systems of cold atoms and optical cavities are promising systems for increasing the stability of laser oscillators used in quantum metrology and atomic clocks. In this paper we map out the atom-cavity dynamics in such a system and demonstrate limitations as well as robustness of the approach. We investigate the phase response of an ensemble of cold $^{88}\mathrm{Sr}$ atoms inside an optical cavity for use as an error signal in laser frequency stabilization. With this system we realize a regime where the high atomic phase shift limits the dynamical locking range. The limitation is caused by the cavity transfer function relating input field to output field. The cavity dynamics is shown to have only little influence on the prospects for laser stabilization, making the system robust towards cavity fluctuations and ideal for the improvement of future narrow linewidth lasers.

DOI
10.1103/physreva.96.013847

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Hybrid systems of cold atoms and optical cavities are promising systems for increasing the stability of laser oscillators used in quantum metrology and atomic clocks. In this paper we map out the atom-cavity dynamics in such a system and demonstrate limitations as well as robustness of the approach. We investigate the phase response of an ensemble of cold 88Sr^{88}\mathrm{Sr}88Sr atoms inside an optical cavity for use as an error signal in laser frequency stabilization. With this system we realize a regime where the high atomic phase shift limits the dynamical locking range. The limitation is caused by the cavity transfer function relating input field to output field. The cavity dynamics is shown to have only little influence on the prospects for laser stabilization, making the system robust towards cavity fluctuations and ideal for the improvement of future narrow linewidth lasers.
Ultra stable frequency references such as the ones used in optical atomic clocks and for quantum metrology may be obtained by stabilizing a laser to an optical cavity that is stable over time. State-of-the-art frequency references are constructed in this way, but their stabilities are currently limited by thermally induced length fluctuations in the reference cavity. Several alternative approaches using the potential for frequency discriminating of highly forbidden narrow atomic transitions have been proposed in, e.g., [1] and [2]. In this proceeding we will present some of the ongoing experimental efforts derived from these proposals, to use cavity-enhanced interaction with atomic 88 Sr samples as a frequency reference for laser stabilization. Such systems can be realized using both passive and active approaches where either the atomic phase response is used as an error signal, or the narrow atomic transition itself is used as a source for a spectrally pure laser. Both approaches shows the promise of being able to compete with the current state of the art in stable lasers and have similar limitations on their ultimately achievable linewidths [1, 2].
We study the nonlinear interaction of a cold sample of 88Sr^{88}\mathrm{Sr}88Sr atoms coupled to a single mode of a low finesse optical cavity in the so-called bad cavity limit, and we investigate the implications for applications to laser stabilization. The atoms are probed on the weak intercombination line $|5{s}^{2}{\phantom{\rule{0.16em}{0ex}}}^{1}{S}_{0}\ensuremath{\rangle}\phantom{\rule{0.16em}{0ex}}\ensuremath{-}\phantom{\rule{0.16em}{0ex}}|5s5p{\phantom{\rule{0.16em}{0ex}}}^{3}{P}_{1}\ensuremath{\rangle}$ at 689 nm in a strongly saturated regime. Our measured observables include the atomic induced phase shift and absorption of the light field transmitted through the cavity represented by the complex cavity transmission coefficient. We demonstrate high signal-to-noise-ratio measurements of both quadratures---the cavity transmitted phase and absorption---by employing frequency modulation (FM) spectroscopy (noise-immune cavity-enhanced optical-heterodyne molecular spectroscopy). We also show that when FM spectroscopy is employed in connection with a cavity locked to the probe light, observables are substantially modified compared to the free-space situation in which no cavity is present. Furthermore, the nonlinear dynamics of the phase dispersion slope is experimentally investigated, and the optimal conditions for laser stabilization are established. Our experimental results are compared to state-of-the-art cavity QED theoretical calculations.
The development of simple and reliable high stability clock lasers is of great importance for future state-of-the-art optical clocks [1]-[5] and for future transportable optical clocks [6], [7]. Further development of clock lasers with better stability has so far been hindered by thermal noise in the reference cavity used for laser stabilization and conventional approaches for improvements may be technically challenging. It has been proposed [8]-[11] to improve the stability and reduce the complexity of state-of-the-art laser frequency stabilization by exploiting cavity QED systems consisting of atoms with a narrow optical transition coupled to a single mode of an optical cavity. The laser stabilization performance of a cavity QED system is affected by a number of system parameters such as the finite temperature of the atoms, the number of involved atoms and the laser power [12]-[14]. However, the dynamics of those elements have not yet been fully explored. Here we present a simple cavity QED system consisting of laser cooled strontium-88 atoms coupled to an optical cavity. We relate measurable quantities to the complex transmission coefficient which relates the input field to the output field. The optimal input power for stabilizing a laser to this system is experimentally determined and the optimal shot-noise-limited linewidth of the system is evaluated to 500 mHz. Furthermore, theoretical shot-noise-limited linewidths of similar cavity QED systems are evaluated for a number of different two electron systems.
Bad cavity lasers are experiencing renewed interest in the context of active optical frequency standards, due to their enhanced robustness against fluctuations of the laser cavity. The gain medium would consist of narrow-linewidth atoms, either trapped inside the cavity or intersecting the cavity mode dynamically. A series of effects like the atoms finite velocity distribution, atomic interactions, or interactions of realistic multilevel atoms with auxiliary or stray fields can lead to an inhomogeneous broadening of the atomic gain profile. This causes the emergence of unstable regimes of laser operation, characterized by complex temporal patterns of the field amplitude. We study the steady-state solutions and their stability for the metrology-relevant case of a bad cavity laser with spin-1/2 atoms, such as 171Yb^{171}\mathrm{Yb}171Yb, interacting with an external magnetic field. For the stability analysis, we present an efficient method, which can be applied to a broad class of single-mode bad cavity lasers with inhomogeneously broadened multilevel atoms acting as a gain medium.
We consider various approaches to the creation of a high-stability active optical frequency standard, where the atomic ensemble itself produces a highly stable and accurate frequency signal. The short-time frequency stability of such standards may overcome the stability of lasers stabilized to macroscopic cavities which are used as local oscillators in the modern optical frequency standard systems. The main idea is to create a “superradiant” laser operating deep in the bad cavity regime, where the decay rate of the cavity field significantly exceeds the decoherence rate of the lasing transition. Two main approaches towards the realization of an active optical frequency standard have been proposed already: the optical lattice laser, and the atomic beam laser. We consider these and some alternative approaches, and discuss the parameters for atomic ensembles necessary to attain the metrology relevant level of short-time frequency stability, and various effects and main challenges critical for practical implementations.
Superradiant lasers may soon achieve state-of-the-art frequency purity, with linewidths of 1 mHz or less. In a superradiant (or bad-cavity) laser, coherence is primarily stored in the atomic gain medium instead of the optical field. This phase storage is characterized by spontaneous quantum synchronization of the optical dipole moments of each atom. To observe this synchronization, we create two independent superradiant atomic ensembles lasing in a single optical cavity and observe the dynamics of phase realignment, collective power enhancement, and steady-state frequency locking. This work introduces superradiant ensembles as a testbed for fundamental study of quantum synchronization as well and informs research on narrow linewidth superradiant lasers.