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arXiv:1604.07171 · Physical Review A

Stability analysis for bad cavity lasers using inhomogeneously broadened spin-1/2 atoms as a gain medium

Georgy A. Kazakov, Thorsten Schumm

Published Feb 24, 2017• 17 citations
arXivHTMLPDF

Abstract

Bad cavity lasers are experiencing renewed interest in the context of active optical frequency standards, due to their enhanced robustness against fluctuations of the laser cavity. The gain medium would consist of narrow-linewidth atoms, either trapped inside the cavity or intersecting the cavity mode dynamically. A series of effects like the atoms finite velocity distribution, atomic interactions, or interactions of realistic multilevel atoms with auxiliary or stray fields can lead to an inhomogeneous broadening of the atomic gain profile. This causes the emergence of unstable regimes of laser operation, characterized by complex temporal patterns of the field amplitude. We study the steady-state solutions and their stability for the metrology-relevant case of a bad cavity laser with spin-1/2 atoms, such as $^{171}\mathrm{Yb}$, interacting with an external magnetic field. For the stability analysis, we present an efficient method, which can be applied to a broad class of single-mode bad cavity lasers with inhomogeneously broadened multilevel atoms acting as a gain medium.

DOI
10.1103/physreva.95.023839

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Bad cavity lasers are experiencing renewed interest in the context of active optical frequency standards, due to their enhanced robustness against fluctuations of the laser cavity. The gain medium would consist of narrow-linewidth atoms, either trapped inside the cavity or intersecting the cavity mode dynamically. A series of effects like the atoms finite velocity distribution, atomic interactions, or interactions of realistic multilevel atoms with auxiliary or stray fields can lead to an inhomogeneous broadening of the atomic gain profile. This causes the emergence of unstable regimes of laser operation, characterized by complex temporal patterns of the field amplitude. We study the steady-state solutions and their stability for the metrology-relevant case of a bad cavity laser with spin-1/2 atoms, such as 171Yb^{171}\mathrm{Yb}171Yb, interacting with an external magnetic field. For the stability analysis, we present an efficient method, which can be applied to a broad class of single-mode bad cavity lasers with inhomogeneously broadened multilevel atoms acting as a gain medium.
Hybrid systems of cold atoms and optical cavities are promising systems for increasing the stability of laser oscillators used in quantum metrology and atomic clocks. In this paper we map out the atom-cavity dynamics in such a system and demonstrate limitations as well as robustness of the approach. We investigate the phase response of an ensemble of cold 88Sr^{88}\mathrm{Sr}88Sr atoms inside an optical cavity for use as an error signal in laser frequency stabilization. With this system we realize a regime where the high atomic phase shift limits the dynamical locking range. The limitation is caused by the cavity transfer function relating input field to output field. The cavity dynamics is shown to have only little influence on the prospects for laser stabilization, making the system robust towards cavity fluctuations and ideal for the improvement of future narrow linewidth lasers.
The instabilities in homogeneously broadened lasers, which we described in the previous chapter, have a paradigmatic importance because they arise in models which allow one to perform the linear-stability analysis in a simple analytic form. The treatment of the corresponding instabilities in the case of in homogeneously broadened lasers is substantially more complex in general. However, it is very interesting because, as we shall see, the instabilities arise in parametric domains that are much more accessible from the experimental viewpoint. A related issue is that of the possibility of multimodal emission in a laser. It is common knowledge that in order to attain multimode emission it is necessary to have a sort of in homogeneity in the gain medium, because in a completely homogeneous configuration all modes interact with all atoms, and the arising competition among modes implies that only one of them survives. There are basically two main kinds of in homogeneity, the first is of spatial nature and the other is of spectral nature. The first kind is realized in Fabry–Perot lasers, because different cavity modes interact with atoms at different spatial positions in the cavity thanks to the standing-wave configuration of the field and to the consequent phenomenon of spatial hole- burning (see Section 14.2 and Fig. 14.1). This circumstance is capable of weakening the mode–mode competition and allowing multimode operation. In unidirectional ring lasers, on the other hand, there is an “inhomogeneous” configuration in the case of inhomogeneous broadening, because different groups of atoms have different transition frequencies and therefore interact with different modes thanks to the spectral hole-burning (see Section 15.2 and Fig. 15.3). Again, this weakens the mode–mode competition and allows multimode operation. However, these are qualitative considerations, and the only reliable and quantitative method to determine the possibility of multimodal operation is the linear-stability analysis of the single-mode stationary solutions.
Essentially closed-form formulae are given for the linewidth of inhomogeneously broadened lasers, with arbitrary cavity detuning and pumping statistics (Poissonian or quiet pumps). The so-called `bad-cavity' mode of operation is treated. The general formula is obtained from a semiclassical theory first derived from a linearized symmetrically ordered quantum theory in the limit of a large number of atoms. This semiclassical theory is most easily explained in terms of independent quantum jumps performed by emitting and absorbing atoms. The effect of inhomogeneous broadening on linewidth is found to be negligible for some pumping schemes, but when the atoms are independently pumped the linewidth is proportional (at some constant power level) to the gain-medium spectral width. We consider, in particular, an intermediate situation in which the rate at which atoms are promoted from the lower to the upper level (pump rate) is proportional to the lower-state population for each atom class. For that particular model, pump fluctuations do not affect the linewidth, even when the cavity is detuned from the centre of the atomic transition frequency distribution.
Up to this point we have always assumed that all the atoms which interact with the radiation field have the same atomic transition frequency, with an atomic linewidth given by γ ⊥ . This configuration is called homogeneous broadening. However, in the great majority of lasers the linewidth is inhomogeneously broadened , because the atomic frequency follows a distribution. For example, in solid-state lasers such as the ruby laser and fiber lasers the inhomogeneity is due to the imperfections in the crystalline structure of the material. In gas lasers, where the atoms or molecules are free to move, the inhomogeneous broadening is due to the Doppler effect, for which a molecule moving with velocity v in a field of frequency ω and wave vector k experiences an effective frequency ω ′ = ω − k · v [8]. Since what matters is the difference between the atomic transition frequency and the field frequency, we can keep the field frequency fixed and imagine that the field interacts with different groups of atoms that move with different velocities and therefore have different transition frequencies. The realistic velocity distribution is a Gaussian, for which the corresponding distribution for the modulus of the velocity is Maxwellian. However, in the following we will mainly analyze the case of a Lorentzian distribution for the atomic transition frequency, because this allows an analytical treatment. Again for the sake of simplicity, we will limit our analysis to the case of a ring cavity. In Section 15.1 we will generalize to the inhomogeneous-broadening configuration the modal equations for the case of homogeneous broadening, which were formulated in Chapter 12. In Section 15.2 we will specialize to the single-mode model and discuss its stationary solutions for the laser case. Multimode dynamical equations The atomic transition frequency of the generic group of atoms is given by ω a + δ D , where ω a is the central atomic frequency and δ D takes positive and negative values. We call ω c the frequency of the cavity mode nearest to ω a and denote by δ ac the difference ω a − ω c .
Pattern formation in large-aspect-ratio single-mode inhomogeneously broadened lasers is studied by means of the integro-differential Maxwell-Bloch equations. As the inhomogeneous linewidth increases, the neutral stability curve shows a relaxation in the traveling wave selection allowing structures with different sizes to grow. We have performed numerical simulations with a simplified model based on a few discrete groups of atoms at different resonant frequencies to observe transverse dynamics above threshold for good and bad cavity configurations. We obtain, in general, that close to threshold the inhomogeneous broadening leads to a more complex pattern in comparison to the homogeneous broadening case. At higher pumpings, a stabilization in the number of spatial frequencies taking part in the transverse pattern is found. The influence of the laser aperture on temporal dynamics is also studied. It is shown how the typical self-pulsing regime present in single-mode inhomogeneously broadened lasers is destroyed for a wide enough aperture.
We consider the dynamics of an inhomogeneously broadened unidirectional ring laser formulated in the traditional Maxwell-Bloch configuration of a two-level atom with transverse modes. We numerically analyze the model for a single-longitudinal mode in the paraxial approximation, using the uniform field limit with cylindrical symmetry and a Gaussian profile for inhomogeneous broadening. Several domains of solutions are found for the resonant case in the good cavity limit. The laser threshold is found to be dependent on the mode spacing as well as on the gain and scaled Doppler broadening. Hysteresis between stable and unstable solutions is obtained in realistic operating conditions for both increasing (decreasing) gain and increasing (decreasing) mode spacing (i.e., for changes in the initial conditions).