The initialization, control, and readout of a single-hole spin qubit is precisely simulated by accurately solving the extended Anderson impurity model in the real-time domain with the hierarchical equations of motion approach. The initialization is realized by ionization of an exciton with high fidelity. Then, a SU(2) control is achieved via the combination of Larmor precession of the hole spin in Voigt geometry magnetic field and rotation about the optical axis with a geometric phase. Finally, the readout of the qubit is implemented through photocurrent recording. Our theory not only reproduces the recent experimental results with one set of internal parameters but also predicts a maximal fidelity by adjusting the dot-electrode coupling strength.
The initialization, control, and readout of a single-hole spin qubit is precisely simulated by accurately solving the extended Anderson impurity model in the real-time domain with the hierarchical equations of motion approach. The initialization is realized by ionization of an exciton with high fidelity. Then, a SU(2) control is achieved via the combination of Larmor precession of the hole spin in Voigt geometry magnetic field and rotation about the optical axis with a geometric phase. Finally, the readout of the qubit is implemented through photocurrent recording. Our theory not only reproduces the recent experimental results with one set of internal parameters but also predicts a maximal fidelity by adjusting the dot-electrode coupling strength.
We demonstrate coherent optical control of a single hole spin confined to an InAs/GaAs quantum dot. A superposition of hole-spin states is created by fast (10-100 ps) dissociation of a spin-polarized electron-hole pair. Full control of the hole spin is achieved by combining coherent rotations about two axes: Larmor precession of the hole spin about an external Voigt geometry magnetic field, and rotation about the optical axis due to the geometric phase shift induced by a picosecond laser pulse resonant with the hole-trion transition.
Single spins in semiconductor quantum dots form a promising platform for solid-state quantum information processing. The spin-up and spin-down states of a single electron or hole, trapped inside a quantum dot, can represent a single qubit with a reasonably long decoherence time. The spin qubit can be optically coupled to excited (charged exciton) states that are also trapped in the quantum dot, which provides a mechanism to quickly initialize, manipulate and measure the spin state with optical pulses, and to interface between a stationary matter qubit and a 'flying' photonic qubit for quantum communication and distributed quantum information processing. The interaction of the spin qubit with light may be enhanced by placing the quantum dot inside a monolithic microcavity. An entire system, consisting of a two-dimensional array of quantum dots and a planar microcavity, may plausibly be constructed by modern semiconductor nano-fabrication technology and could offer a path toward chip-sized scalable quantum repeaters and quantum computers. This article reviews the recent experimental developments in optical control of single quantum dot spins for quantum information processing. We highlight demonstrations of a complete set of all-optical single-qubit operations on a single quantum dot spin: initialization, an arbitrary SU(2) gate, and measurement. We review the decoherence and dephasing mechanisms due to hyperfine interaction with the nuclear-spin bath, and show how the single-qubit operations can be combined to perform spin echo sequences that extend the qubit decoherence from a few nanoseconds to several microseconds, more than 5 orders of magnitude longer than the single-qubit gate time. Two-qubit coupling is discussed, both within a single chip by means of exchange coupling of nearby spins and optically induced geometric phases, as well as over longer-distances. Long-distance spin-spin entanglement can be generated if each spin can emit a photon that is entangled with the spin, and these photons are then interfered. We review recent work demonstrating entanglement between a stationary spin qubit and a flying photonic qubit. These experiments utilize the polarization- and frequency-dependent spontaneous emission from the lowest charged exciton state to single spin Zeeman sublevels.
Spin qubits in gate-defined semiconductor quantum dots are a promising platform for realising a scalable quantum computer. This platform encodes quantum information into the intrinsic angular momentum (spin) of individual electrons or holes. In particular, hole spins in quantum dots enable the possibility of all-electrical spin control due to their intrinsic spin-orbit coupling. One important criterion of a quantum computer is the ability to reliably read out the state of the qubit. This is done by mapping spin information to the charge degree of freedom, combined with a method for charge detection. Charge detection can be facilitated by coupling a resonator directly to the quantum dot gate or to a charge sensor and measuring the resonator's phase or amplitude response. In this thesis, we describe a set of experiments relating to the implementation of hole spin qubit readout with superconducting resonators. First, we study gate-based charge sensing in a Si fin field-effect transistor (finFET) device using a superconducting NbN nanowire resonator. We find that the resonator amplifies capacitive crosstalk when electrical control pulses are applied to gate electrodes in this device. This occurs whenever a spectral component of qubit control pulses overlaps with the resonance frequency, which we show may occur for both baseband and radio-frequency (RF) drive signals. We quantify this crosstalk in a transport-based method, and attribute its source to the capacitance between the bondpads of neighbouring gate electrodes. In a second experiment, we use an RF charge sensor with the same nanowire technology to read out hole spin qubits formed in the quantum well of a Ge/SiGe heterostructure. A screening layer approach is used to facilitate RF matching due to large RF dissipation found in the heterostructure. We implement a double-latched readout scheme in this system to reduce errors arising from both spin and charge decay during readout. The spin-to-charge conversion process and its dependence on magnetic field orientation is studied. Spin and charge decay processes arising after spin-to-charge conversion are mitigated by choosing an optimal working point for the field orientation, field amplitude and readout pulse times. By doing so, we achieve an average single-shot state-preparation-and-measurement fidelity of 97%, primarily bounded by imperfect state preparation and limited signal-to-noise ratio. Finally, we study coplanar waveguide resonators fabricated from NbN. We investigate the feasibility of integrating this type of resonator onto the same chip as the Si finFET quantum dots. We then develop a novel resonator readout technique by the interference of two microwave sidebands. We demonstrate the insensitivity of this technique to common-mode phase and amplitude noise both theoretically and experimentally. This technique is then used to study resonator noise arising from two-level system defects. These results highlight both the practical constraints and the potential for achieving high readout fidelities using resonator-based hole spin qubit readout. This work establishes a blueprint for mitigating resonator-induced crosstalk and enabling high-fidelity readout in lossy materials by incorporating a screening layer.
Optically driven self-assembled quantum dots are leading candidates for use in quantum computers because of their potential for high speed gate operations and relatively compact design. In this approach, each dot is charged with a single electron whose spin serves as the quantum bit (qubit). This thesis addresses the need for a universal set of gates to physically implement quantum computing and discusses initial steps toward spin-photon entanglement. Both are addressed through coherent control of the spin state in a magnetic field with optical pulses. This work experimentally demonstrates coherent rotations of the electron spin. First, the electron spin is rotated at up to 0.5 terahertz about the optical axis by a detuned picosecond optical pulse. The rotation occurs via a nearly resonant stimulated spin-flip Raman process involving a negatively charged exciton (trion). Second, rotation about an orthogonal axis is demonstrated due to electron spin precession about the magnetic field between two detuned optical pulses. The magnitude of the electron g factor is measured to be 0.4, and the rotation speed is 30 gigahertz in a 6.6 Tesla field. Geometric phases are detected in quantum dots for the first time due to cyclic Rabi oscillations driven by a resonant continuous-wave laser. These geometric phases provide another method of spin rotation and can be used in a gate. Any combination of these methods that provides spin rotation about two orthogonal axes can form an arbitrary rotation and together with a phase gate can form any unitary single qubit gate. Finally, this thesis also presents a detailed experimental procedure for creating a partial entanglement of internal variables within a quantum dot spin-exciton system, as a preliminary step to spin-photon entanglement. It has been proposed that entanglement between non-adjacent qubits in a large qubit network could occur via a photon, fueling research to demonstrate spin-photon entanglement. The experiment proposed here will create the precursor state in 25 picoseconds with a predicted fidelity of 0.985, and the precursor superposition state has a theoretical entropy of entanglement of 0.92.
The spin of a charged semiconductor quantum dot (QD) coupled to an optical cavity is a promising candidate for high-fidelity spin-photon interfaces; the cavity selectively modifies the decay rates of optical transitions such that spin initialization, manipulation, and readout are all possible in a single magnetic field geometry. By performing cavity QED calculations, we show that a cavity with a single, linearly polarized mode can simultaneously support both high-fidelity optical spin initialization and readout in a single, in-plane (Voigt geometry) magnetic field. Furthermore, we demonstrate that single-mode cavities always outperform bimodal cavities in experimentally favorable driving regimes. Our analysis, when combined with established methods of control in a Voigt geometry field, provides optimal parameter regimes for high-fidelity initialization and readout, and coherent control in both cavity configurations, providing insights for the design and development of QD spin-photon interfaces as the basis of quantum network nodes and for the generation of photonic graph states. Published by the American Physical Society 2024
Self-assembled quantum dots (QDs) containing a single electron are one of the leading candidate systems for the realization of a quantum computer. The spin states of charges confined in these dots have been shown to possess a number of qualities that are attractive for use as the quantum bits (qubits) in quantum computing implementations, particularly their long lifetimes and coherence times. In addition, these spin qubits may be controlled optically, offering the prospect of ultrafast qubit gate operations, a crucial necessity for the execution of quantum algorithms. Due to the weak interaction of self-assembled QDs with light, however, the coherent optical control and read-out of the spin states of charged self-assembled QDs has proven to be a considerable challenge. This thesis presents two sets of experiments demonstrating the coherent optical control and read-out of the quantum states of a self-assembled InAs QD containing a single electron. The first utilizes mode-locked picosecond optical pulses to control the optical transitions in the dot and to detect QD level occupations. These capabilities are used to observe transient phenomena in a singly charged InAs QD such as the generation and decay of excited state population and spin precession. Further, Rabi oscillations between the electron and the lowest-lying excited state are observed, demonstrating the ability to coherently control the optical transitions of the QD, a prerequisite for spin control. These results are built upon in the second set of experiments, in which a combination of optical pulses, an externally applied DC magnetic field and a continuous-wave (CW) optical field are employed to initialize and completely control the states of a QD confined electron spin. Spin control by the use of pulse-driven two-photon Raman processes, spin precession about the external magnetic field and geometric phases generated by CW-driven cyclic evolutions in the dot is demonstrated. A number of spin qubit gate operations are shown for these spin control mechanisms, forming a foundational set of single qubit gates required for the implementation of quantum computing with singly charged self-assembled QDs.