The spin of a charged semiconductor quantum dot (QD) coupled to an optical cavity is a promising candidate for high-fidelity spin-photon interfaces; the cavity selectively modifies the decay rates of optical transitions such that spin initialization, manipulation, and readout are all possible in a single magnetic field geometry. By performing cavity QED calculations, we show that a cavity with a single, linearly polarized mode can simultaneously support both high-fidelity optical spin initialization and readout in a single, in-plane (Voigt geometry) magnetic field. Furthermore, we demonstrate that single-mode cavities always outperform bimodal cavities in experimentally favorable driving regimes. Our analysis, when combined with established methods of control in a Voigt geometry field, provides optimal parameter regimes for high-fidelity initialization and readout, and coherent control in both cavity configurations, providing insights for the design and development of QD spin-photon interfaces as the basis of quantum network nodes and for the generation of photonic graph states. Published by the American Physical Society 2024
The spin of a charged semiconductor quantum dot (QD) coupled to an optical cavity is a promising candidate for high-fidelity spin-photon interfaces; the cavity selectively modifies the decay rates of optical transitions such that spin initialization, manipulation, and readout are all possible in a single magnetic field geometry. By performing cavity QED calculations, we show that a cavity with a single, linearly polarized mode can simultaneously support both high-fidelity optical spin initialization and readout in a single, in-plane (Voigt geometry) magnetic field. Furthermore, we demonstrate that single-mode cavities always outperform bimodal cavities in experimentally favorable driving regimes. Our analysis, when combined with established methods of control in a Voigt geometry field, provides optimal parameter regimes for high-fidelity initialization and readout, and coherent control in both cavity configurations, providing insights for the design and development of QD spin-photon interfaces as the basis of quantum network nodes and for the generation of photonic graph states. Published by the American Physical Society 2024
Quantum networking is a crucial technology towards constructing large-scale distributed quantum systems. The structure of photonic link and distributed network nodes allows high-speed and high-fidelity interconnect, enabling various applications such as distributed quantum computing and sensing, as well as secure quantum communications. Optically interfaced solid-sate spins are promising candidates for building a quantum network due to their active spin-photon interfaces, compatibility, and scalability for device integration. Especially for defect spins in silicon, the platform benefits from mature silicon photonic industry, and can access to the integration techniques developed over the past decades. T center in silicon particularly holds great expectations because of the telecom-O band optical interface, ground state doublet spin manifold, and long-lived nuclear spin coherence. Their telecom spin-photon interface provides a direct link between stationary quantum memory and flying qubits that are compatible with the existing telecommunication fiber network infrastructure. This work focuses on investigating cavity quantum electrodynamics (cQED) for cavity-coupled single T centers, its applications in quantum optical control of T center optical properties, and in realizing single-shot spin state readout. The cavity enhanced light-matter interaction mitigates the caveats of T center, such as long radiative lifetime, low Debye-Waller factor, and lack of polarization selection rule for the optical transitions. In this work, by integrating single T centers with a low-loss, small mode volume silicon photonic cavity, we have achieved the Purcell enhancement for boosting the T center fluorescence rate with a factor of 6.89. We build up the theoretical framework based on the Jaynes-Cummings model and Lindblad master equation to explain experimental observations and reveal cQED parameters. The further study on the electronic spin state readout is carried out as the fast, high-fidelity single-shot readout is critical for quantum information processing. Two methods are proposed based on realistic cQED parameters: resonant fluorescence readout in the low-cooperativity regime and spin-dependent cavity-reflection readout for intermediate- and high-cooperativity regimes. Both approaches demonstrate feasibility of high-fidelity (F > 0.95) readout, particularly the reflection readout allows F > 0.99 within a short readout time of 50 μs. This work demonstrates a promising telecom spin-photon interface with high-fidelity readout based on cavity-coupled single T centers in silicon, which are promising candidates for building future large-scale quantum networks.
The realization of quantum-photonic networks is a key challenge for optical quantum technologies. To scale such networks to many nodes and long distances, an efficient interface between stationary and flying qubits is necessary. One of the front-runners towards this goal is a spin-photon interface realised with a single charged QD with a localized electron spin that is strongly coupled to a micropillar cavity [1] . Through the strong spin-photon coupling, the polarization state of the optical field is controlled by the QD spin, thus modulating the cavity’s transmission properties. Controlling the polarization state over a wide angle is particularly useful for realizing high-fidelity polarization states and conditional phase quantum gates (e.g. CNOT) for photon-based quantum computing.
A basic system with important potential applications in quantum technologies is a quantum dot in the
Voigt geometry. The spin states of the quantum dot in the Voigt geometry can act as a prototype qubit which
can be manipulated by applied optical fields in order to produce the necessary quantum gates. The basic method
for spin initialization in a quantum dot in the Voigt geometry is optical pumping. Here, we propose and analyze
a new method for the coherent preparation of the quantum dot spin states based on adiabatic control methods.
Specifically, we show that the application of two mutually delayed and partially overlapping optical pulses, similar
to those used in stimulated Raman adiabatic passage, can lead to initialization of one of the spin states with high
fidelity. We also demonstrate that the fidelity of the method may be increased by integrating the quantum dot with
a micropillar cavity. Specifically, we show that a preferential Purcell-enhanced decay rate towards the target spin
state, in certain cases, increases the fidelity of spin initialization of the adiabatic method. Our results are based on
the numerical solution of the relevant density matrix equations for the quantum dot system, either in an isotropic
photonic environment or in a micropillar cavity. The calculations presented in this paper are not limited to quantum
dots in micropillar cavities. Similar effects can be obtained by other photonic structures as well, as for example,
for quantum dots in photonic crystal cavities.
Hybrid quantum photonic systems connect classical photonics to the quantum world and promise to deliver efficient light-matter quantum interfaces while leveraging the advantages of both, the classical and the quantum, subsystems. However, combining efficient, scalable photonics and solid-state quantum systems with desirable optical and spin properties remains a formidable challenge. In particular, the access to individual spin states and coherent mapping to photons remains unsolved for hybrid systems. In this paper, we demonstrate all-optical initialization and readout of the electron spin of a negatively charged silicon-vacancy center in a nanodiamond coupled to a silicon nitride photonic crystal cavity. We characterize relevant parameters of the coupled emitter-cavity system and determine the silicon-vacancy center’s spin-relaxation and spin-decoherence rate. Our results mark a key step towards the realization of a hybrid spin-photon interface based on silicon nitride photonics and the silicon-vacancy center’s electron spin in nanodiamonds with potential use for quantum networks, quantum communication, and distributed quantum computation. Published by the American Physical Society 2024
In the framework of optical quantum computing and communications, a major objective consists in building receiving nodes that implement conditional operations on incoming photons, using the interaction with a single stationary qubit. In particular, the quest for scalable nodes motivated the development of cavity-enhanced spin-photon interfaces with solid-state emitters. An important challenge remains, however, to produce a stable, controllable, spin-dependant photon state, in a deterministic way. Here we use a pillar-based high-Q cavity, embedding a singly-charged semiconductor quantum dot, to demonstrate the control of giant polarisation rotations induced by a single electron spin. A complete tomography approach is used to deduce the output polarisation Stokes vector, conditioned by a single spin state. We experimentally demonstrate rotation amplitudes such as ±2π and π in the Poincaré sphere, as required for applications based on spin-polarisation mapping and spin-mediated photon-photon gates. In agreement with our modeling, we observe that the environmental noise does not limit the amplitude of the spin-induced rotation, yet slightly degrades the polarisation purity of the output states. We find that the polarisation state of the reflected photons can be manipulated in most of the Poincaré sphere, through controlled spin-induced rotations, thanks to moderate cavity birefringence and limited noise. This control allows the operation of spin-photon interfaces in various configurations, including at zero or low magnetic fields, which ensures compatibility with key protocols for photonic cluster state generation.
The ultimate goal of quantum information science is to build quantum networks for distributed quantum computing or for the secure sharing of information between spatially remote parties [1]. Quantum networks utilize static (matter) quantum bits (qubits) to store and process quantum information at local nodes, and photons as flying qubits for long-distance quantum state transmission between different nodes. To realize a quantum network, it is crucial to achieve light-matter entanglement and reversible quantum-state transfer between light and matter, i.e., the light-matter quantum interface, and the quantum repeater for large-scale quantum communications [2]. Recent experiments have shown that both electrons and holes confined in semiconductor quantum dots (QDs) have long spin relaxation time (T1e, T1h ~ ms) and long spin coherence time (T2e ~ s, T2h > 100 ns). Moreover, fast spin cooling and ultra-fast spin manipulation as well as spin echoes to preserve the spin coherence have also been demonstrated. Undoubtedly these rapid progresses imply that the QD spin is a good candidate for matter qubit in quantum information processing. Furthermore, QD-based single photon sources have been also developed. Therefore, semiconductor QDs offer a good platform for solid-state quantum networking. Here we present two types of conditional quantum gates, i.e., the photon-spin entangling gates [3-4] using a single QD spin in a single-sided or double-sided optical microcavity. Both gates are universal and deterministic (if they are optimized). The spin-selective coherent photon-spin interaction enhanced by the cavity QED lead to giant circular birefringence, which allows us to build these gates. We will show some of the key applications [3-5], including: (i) single-shot quantum non-demolition measurement of spin; (ii) single-photon based spin manipulations and spin echoes to preserve the spin coherence; (iii) photon-spin, spin-spin and photon-photon entanglement generation with high fidelity and high efficiency; (iv) deterministic photon-spin interface and perfect spin memory; (v) complete and loss-resistant Bell-state analyzer, which could increase the distance of state-of-the-art quantum communications by one order of magnitude (from current 100 km to over 1000 km) [5]; (vi) the full quantum repeater combining quantum memory, entanglement swapping and purifications for arbitrary long distance communications [5]; (vii) spin-controlled single photon sources. All these schemes are feasible with current semiconductor technology [6], and we have recently seen conditional phase shifts in uncharged QD-cavity systems [7]. The versatile spin-cavity systems can be applied in all aspects of quantum information science and technology, not only for large-scale quantum communication networks, but also for scalable quantum computing with either photons or spins as qubits. References [1] H.J. Kimble, Nature (London) 453, 1023 (2008). [2] H.-J. Briegel et al., Phys. Rev. Lett. 81, 5932 (1998). [3] C.Y. Hu et al., Phys. Rev. B 78, 085307 (2008); ibid. 78, 125318 (2008). [4] C.Y. Hu et al., Phys. Rev. B 80, 205326 (2009). [5] C.Y. Hu and J.G. Rarity, ArXiv: quant-ph 1005.5545 (2010). [6] S. Reitzenstein et al., Appl. Phys. Lett. 90, 251109 (2007). [7] A.B. Young et al., ArXiv: quant-ph 1011.0384 (2010).