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arXiv:1704.02289 · Journal of the Optical Society of America B

Levitated nanoparticle as a classical two-level atom [Invited]

Martin Frimmer, Jan Gieseler, Thomas Ihn, Lukáš Novotný

Published May 24, 2017• 7 citations
arXivHTMLPDF

Abstract

The center-of-mass motion of a single optically levitated nanoparticle resembles three uncoupled harmonic oscillators. We show how a suitable modulation of the optical trapping potential can give rise to a coupling between two of these oscillators, such that their dynamics are governed by a classical equation of motion that resembles the Schrödinger equation for a two-level system. Based on experimental data, we illustrate the dynamics of this parametrically coupled system both in the frequency and in the time domain. We discuss the limitations and differences of the mechanical analogue in comparison to a true quantum mechanical system.

DOI
10.1364/josab.34.000c52

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The center-of-mass motion of a single optically levitated nanoparticle resembles three uncoupled harmonic oscillators. We show how a suitable modulation of the optical trapping potential can give rise to a coupling between two of these oscillators, such that their dynamics are governed by a classical equation of motion that resembles the Schrödinger equation for a two-level system. Based on experimental data, we illustrate the dynamics of this parametrically coupled system both in the frequency and in the time domain. We discuss the limitations and differences of the mechanical analogue in comparison to a true quantum mechanical system.
ABSTRACT Levitodynamics, i.e., the levitation of objects of mesoscopic size has made huge progress in the last decade allowing to address some questions of fundamental physics for the first time. It has become possible to cool a levitated particle of mesoscopic size down to its motional ground state and to observe its motion driven by quantum fluctuations. This defines a quantum system that is ideally suited for an analysis within Nelson's stochastic mechanics approach to quantum mechanics, which allows for a dynamic description of individual particle paths. In good approximation, a levitated nanoparticle is a quantum harmonic oscillator. The coherent states of such an oscillator are superpositions of classical paths and the stochastic ground state process. They are exact solutions not only of the Schrödinger equation but also of the quantum Hamilton equations of Nelson's stochastic mechanics, and they are amenable to path simulations. All model parameters are typically available from experiment. Analyzing the quantum motion of the levitated nanoparticle in terms of the coherent states of a quantum harmonic oscillator allows for a quantitative prediction of the experimentally measured power spectral density of its position fluctuations and predicts new experimentally accessible measures for the mean number of phonons present in the center of mass motion. It also explains the observed phase space trajectory of the nano‐particle during cooling.
We develop the theory describing the quantum coupled dynamics of the center-of-mass motion of a nanoparticle and an ensemble of ions co-trapped in a dual-frequency linear Paul trap. We first derive analytical expressions for the motional frequencies and classical trajectories of both nanoparticle and ions. We then derive a quantum master equation for the ion-nanoparticle system and quantify the sympathetic cooling of the nanoparticle motion enabled by its Coulomb coupling to a continuously Doppler-cooled ion. We predict that motional cooling down to sub-kelvin temperatures is achievable in state-of-the-art experiments even in the absence of motional feedback and in the presence of micromotion. We then extend our analysis to an ensemble of NNN ions, predicting a linear increase of the cooling rate as a function of NNN and motional cooling of the nanoparticle down to tenths of millikelvin in current experimental platforms. Our work establishes the theoretical toolbox needed to explore the ion-assisted preparation of non-Gaussian motional states of levitated nanoparticles.
Optically levitated nanoparticles have recently emerged as versatile platforms for investigating macroscopic quantum mechanics and enabling ultrasensitive metrology. In this paper we theoretically consider two damping regimes of an optically levitated nanoparticle cooled by cavityless parametric feedback. Our treatment is based on a generalized Fokker-Planck equation derived from the quantum master equation presented recently and shown to agree very well with experiment [B. Rodenburg, L. P. Neukirch, A. N. Vamivakas, and M. Bhattacharya, Quantum model of cooling and force sensing with an optically trapped nanoparticle, Optica 3, 318 (2016)]. For low damping, we find that the resulting Wigner function yields the single-peaked oscillator position distribution and recovers the appropriate energy distribution derived earlier using a classical theory and verified experimentally [J. Gieseler, R. Quidant, C. Dellago, and L. Novotny, Dynamic relaxation of a levitated nanoparticle from a non-equilibrium steady state, Nat. Nano. 9, 358 (2014)]. For high damping, in contrast, we predict a double-peaked position distribution, which we trace to an underlying bistability induced by feedback. Unlike in cavity-based optomechanics, stochastic processes play a major role in determining the bistable behavior. To support our conclusions, we present analytical expressions as well as numerical simulations using the truncated Wigner function approach. Our work opens up the prospect of developing bistability-based devices, characterization of phase-space dynamics, and investigation of the quantum-classical transition using levitated nanoparticles.
Abstract Tests of quantum mechanics on a macroscopic scale require extreme control over mechanical motion and its decoherence [1-4]. Quantum control of mechanical motion has been achieved by engineering the radiation pressure coupling between a micromechanical oscillator and the electromagnetic field in a resonator [5-8]. Furthermore, measurement-based feedback control relying on cavity-enhanced detection schemes has been used to cool micromechanical oscillators to their quantum ground states [9]. In contrast to mechanically tethered systems, optically levitated nanoparticles are particularly promising candidates for matter-wave experiments with massive objects [10,11], since their trapping potential is fully controllable. In this work, we optically levitate a femto-gram dielectric particle in cryogenic free space, which suppresses thermal effects sufficiently to make the measurement backaction the dominant decoherence mechanism. With an efficient quantum measurement, we exert quantum control over the dynamics of the particle. We cool its center-of-mass motion by measurement-based feedback to an average occupancy of 0.65 motional quanta, corresponding to a state purity of 43%. The absence of an optical resonator and its bandwidth limitations holds promise to transfer the full quantum control available for electromagnetic fields to a mechanical system. Together with the fact that the optical trapping potential is highly controllable, our experimental platform offers a route to investigating quantum mechanics at macroscopic scales [12,13].
The motion control of a levitated nanoparticle plays a central role in optical levitation for fundamental studies and practical applications. Here, we presented digital parametric feedback cooling based on square wave modulation by switching trapping laser intensity between two levels. The effects of the modulation depth and modulation signal phase on the cooling result were investigated in detail. Using such a digital parametric feedback method, the center-of-mass temperature of all three motional degrees of freedom can be cooled to dozens of millikelvin. The flexibility and agility of the digital feedback control pave the way for a variety of motion control modes.
Levitated nanoparticles are a forerunner as an experimental platform to test the limits of quantum mechanics at a macroscopic scale. Some important initial steps have been made towards preparing a macroscopic quantum state of a relatively massive (femtogram) particle. Specifically, the community has achieved ground-state cooling of the center-of-mass motion of a nanoparticle levitated in an optical trap. One crucial further step is now to expand the wavefunction of the particle. This step should happen in the presence of a minimum of decoherence, which makes evolution in an optical trap (inevitably exerting measurement backaction) unsuitable.