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arXiv:1703.04165 · Physical Review Letters

Suppression of Multiphoton Resonances in Driven Quantum Systems via Pulse Shape Optimization

Denis Gagnon, François Fillion‐Gourdeau, Joey Dumont, Catherine Lefebvre, Steve G. MacLean

Published Aug 3, 2017• 17 citations
arXivHTMLPDF

Abstract

This Letter demonstrates control over multiphoton absorption processes in driven two-level systems, which include, for example, superconducting qubits or laser-irradiated graphene, through spectral shaping of the driving pulse. Starting from calculations based on Floquet theory, we use differential evolution, a general purpose optimization algorithm, to find the Fourier coefficients of the driving function that suppress a given multiphoton resonance in the strong field regime. We show that the suppression of the transition probability is due to the coherent superposition of high-order Fourier harmonics which closes the dynamical gap between the Floquet states of the two-level system.

DOI
10.1103/physrevlett.119.053203

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This Letter demonstrates control over multiphoton absorption processes in driven two-level systems, which include, for example, superconducting qubits or laser-irradiated graphene, through spectral shaping of the driving pulse. Starting from calculations based on Floquet theory, we use differential evolution, a general purpose optimization algorithm, to find the Fourier coefficients of the driving function that suppress a given multiphoton resonance in the strong field regime. We show that the suppression of the transition probability is due to the coherent superposition of high-order Fourier harmonics which closes the dynamical gap between the Floquet states of the two-level system.
We consider the dynamics of a two-level system (qubit) driven by strong and short resonant pulses in the framework of Floquet theory. First we derive analytical expressions for the quasienergies and Floquet states of the driven system. If the pulse amplitude varies very slowly, the system adiabatically follows the instantaneous Floquet states, which acquire dynamical phases that depend on the evolution of the quasienergies over time. The difference between the phases acquired by the two Floquet states corresponds to a qubit state rotation, generalizing the notion of Rabi oscillations to the case of large driving amplitudes. If the pulse amplitude changes very fast, the evolution is nonadiabatic, with transitions taking place between the Floquet states. We quantify and analyze the nonadiabatic transitions during the pulse by employing adiabatic perturbation theory and exact numerical simulations. We find that, for certain combinations of pulse rise and fall times and maximum driving amplitude, a destructive interference effect leads to a remarkably strong suppression of transitions between the Floquet states. This effect provides the basis of a quantum control protocol, which we name Floquet interference efficient suppression of transitions in the adiabatic basis (FIESTA), that can be used to design ultrafast high-fidelity single-qubit quantum gates.
We extend the many-mode Floquet theorem (MMFT) for the investigation of multiphoton resonance dynamics driven by intense frequency-comb laser fields. The frequency comb structure generated by a train of short laser pulses can be exactly represented by a combination of the main frequency and the repetition frequency. MMFT allows non-perturbative and exact treatment of the interaction of a quantum system with the frequency-comb laser fields. We observe simultaneous multiphoton resonance processes between a two-level system and frequency-comb laser. The multiphoton processes can be coherently controlled by tuning the laser parameters such as the carrier-envelope phase (CEP) shift. In particular, high-order harmonic generation shows immense enhancement by tuning the CEP shift, due to simultaneous multiphoton resonances.
Using the Floquet formalism and the adiabatic approximation we develop a theory for optimal control of a multilevel quantum system interacting with an external electric field under multiphoton resonance conditions. Optimal solutions for the case of control over a time interval are presented. We derive a differential equation to determine the shape of the optimal pulse, and show how the order of the multiphoton resonance affects the solution. In particular, we demonstrate that optimal control in the case of two-photon resonance and using only adiabatically shaped control pulses represents a special degenerate case, for which the shape of the pulse cannot be optimized. Thus, for this particular case the final state of the controlled system is completely determined by the pulse energy.
Synopsis High-order nonlinear multiphoton dynamics of closed and open periodically driven quantum systems are studied within the semiclassical Floquet formalism. Multiphoton up/down frequency conversion in a super-conducting circuit is realized and faithfully reproduced with calculations. The absorption spectra are suppressed at sharp avoided crossings of the Floquet states. We include the effect of coupling to cavity by time evolving the master equation. The characteristics of the time-averaged absorption spectra are investigated by probing details near and around the exceptional points where suppression occurs.
We present a theoretical investigation of the multiphoton resonance dynamics driven by intense frequency-comb and cavity-mode fields inside a femtosecond enhancement cavity (fsEC). The many-mode Floquet theorem is employed to provide a nonperturbative and exact treatment of the interaction between a quantum system and laser fields. The quasienergy structure driven by the frequency-comb laser field is modified by coupling the cavity-mode field and the multiphoton resonance processes between modified quasienergy states, resulting in the generation of even-order harmonics. The high-order harmonic generation (HHG) from a two-level system driven by the laser fields can be coherently controlled by tuning the laser parameters. In particular, the tuning intensity of the cavity-mode field allows one to coherently control the HHG power spectra without changing the absolute positions of comb frequencies.
We present a Floquet treatment of multiphoton quantum interference in a strongly driven superconducting flux qubit. The periodically time-dependent Schr\"odinger equation can be reduced to an equivalent time-independent infinite-dimensional Floquet matrix eigenvalue problem. For resonant or nearly resonant multiphoton transitions, we extend the generalized Van Vleck (GVV) nearly degenerate high-order perturbation theory for the treatment of the Floquet Hamiltonian, allowing the reduction of the infinite-dimensional Floquet matrix to an $N\ifmmode\times\else\texttimes\fi{}N$ effective Hamiltonian, where NNN is the number of eigenstates under consideration. The GVV approach allows accurate treatment of ac Stark shift, power broadening, time-dependent and time-averaged transition probability, etc., well beyond the rotating wave approximation. We extend the Floquet and GVV approaches for numerical and analytical studies of the multiphoton resonance processes and quantum interference phenomena for the superconducting flux qubit system (N=2)(N=2)(N=2) driven by intense ac fields.