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arXiv:1701.07812 · Nano Letters

Phonon-Assisted Two-Photon Interference from Remote Quantum Emitters

Marcus Reindl, Klaus D. Jöns, Daniel Huber, Christian Schimpf, Yong-Heng Huo, Val Zwiller, Armando Rastelli, Rinaldo Trotta

Published May 30, 2017• 117 citations
arXivHTMLPDF

Abstract

Photonic quantum technologies are on the verge of finding applications in everyday life with quantum cryptography and quantum simulators on the horizon. Extensive research has been carried out to identify suitable quantum emitters and single epitaxial quantum dots have emerged as near-optimal sources of bright, on-demand, highly indistinguishable single photons and entangled photon-pairs. In order to build up quantum networks, it is essential to interface remote quantum emitters. However, this is still an outstanding challenge, as the quantum states of dissimilar "artificial atoms" have to be prepared on-demand with high fidelity and the generated photons have to be made indistinguishable in all possible degrees of freedom. Here, we overcome this major obstacle and show an unprecedented two-photon interference (visibility of 51 ± 5%) from remote strain-tunable GaAs quantum dots emitting on-demand photon-pairs. We achieve this result by exploiting for the first time the full potential of a novel phonon-assisted two-photon excitation scheme, which allows for the generation of highly indistinguishable (visibility of 71 ± 9%) entangled photon-pairs (fidelity of 90 ± 2%), enables push-button biexciton state preparation (fidelity of 80 ± 2%) and outperforms conventional resonant two-photon excitation schemes in terms of robustness against environmental decoherence. Our results mark an important milestone for the practical realization of quantum repeaters and complex multiphoton entanglement experiments involving dissimilar artificial atoms.

DOI
10.1021/acs.nanolett.7b00777

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Photonic quantum technologies are on the verge of finding applications in everyday life with quantum cryptography and quantum simulators on the horizon. Extensive research has been carried out to identify suitable quantum emitters and single epitaxial quantum dots have emerged as near-optimal sources of bright, on-demand, highly indistinguishable single photons and entangled photon-pairs. In order to build up quantum networks, it is essential to interface remote quantum emitters. However, this is still an outstanding challenge, as the quantum states of dissimilar "artificial atoms" have to be prepared on-demand with high fidelity and the generated photons have to be made indistinguishable in all possible degrees of freedom. Here, we overcome this major obstacle and show an unprecedented two-photon interference (visibility of 51 ± 5%) from remote strain-tunable GaAs quantum dots emitting on-demand photon-pairs. We achieve this result by exploiting for the first time the full potential of a novel phonon-assisted two-photon excitation scheme, which allows for the generation of highly indistinguishable (visibility of 71 ± 9%) entangled photon-pairs (fidelity of 90 ± 2%), enables push-button biexciton state preparation (fidelity of 80 ± 2%) and outperforms conventional resonant two-photon excitation schemes in terms of robustness against environmental decoherence. Our results mark an important milestone for the practical realization of quantum repeaters and complex multiphoton entanglement experiments involving dissimilar artificial atoms.
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Entanglement swapping is a protocol that details how to create entanglement between previously uncorrelated particles. Its all-photonic version - mediated by the interference of photon pairs generated by separate quantum systems-finds disparate applications in quantum networks. So far, all-photonic entanglement swapping between remote systems has been implemented only using sources that operate probabilistically. However, the scaling up of quantum networks requires deterministic quantum emitters that do not suffer from a trade-off between degree of entanglement and photonpair generation rate. Here, we demonstrate all-photonic entanglement swapping using photon-pairs generated by two separate GaAs quantum dots. The emitters are deterministically embedded in hybrid semiconductor-piezoelectric devices that make the entangled-photons from two dissimilar quantum dots nearly identical. Entanglement swapping is demonstrated with a fidelity as high as 0.71(2), more than 10 standard deviations above the classical limit. The experimental data are quantitatively explained by a theoretical model that also suggests how to boost the protocol performances. Our work opens the path to the exploitation of quantum dot entangled-photon sources in quantum repeater networks.
High Resolution Image Download MS PowerPoint Slide Entangled photons are an integral part in quantum optics experiments and a key resource in quantum imaging, quantum communication, and photonic quantum information processing. Making this resource available on-demand has been an ongoing scientific challenge with enormous progress in recent years. Of particular interest is the potential to transmit quantum information over long distances, making photons the only reliable flying qubit. Entangled photons at the telecom C-band could be directly launched into single-mode optical fibers, enabling worldwide quantum communication via existing telecommunication infrastructure. However, the on-demand generation of entangled photons at this desired wavelength window has been elusive. Here, we show a photon pair generation efficiency of 69.9 ± 3.6% in the telecom C-band by an InAs/GaAs semiconductor quantum dot on a metamorphic buffer layer. Using a robust phonon-assisted two-photon excitation scheme we measure a maximum concurrence of 91.4 ± 3.8% and a peak fidelity to the Φ + state of 95.2 ± 1.1%, verifying on-demand generation of strongly entangled photon pairs and marking an important milestone for interfacing quantum light sources with our classical fiber networks.
All-optical quantum teleportation lies at the heart of quantum communication science and technology. This quantum phenomenon is built up around the nonlocal properties of entangled states of light that, in the perspective of real-life applications, should be encoded on photon pairs generated on demand. Despite recent advances, however, the exploitation of deterministic quantum light sources in push-button quantum teleportation schemes remains a major open challenge. Here, we perform an important step toward this goal and show that photon pairs generated on demand by a GaAs quantum dot can be used to implement a teleportation protocol whose fidelity violates the classical limit (by more than 5 SDs) for arbitrary input states. Moreover, we develop a theoretical framework that matches the experimental observations and that defines the degree of entanglement and indistinguishability needed to overcome the classical limit independently of the input state. Our results emphasize that on-demand solid-state quantum emitters are one of the most promising candidates to realize deterministic quantum teleportation in practical quantum networks.
We report on the observation of nearly maximally entangled photon pairs from semiconductor quantum dots, without resorting to postselection techniques. We use GaAs quantum dots integrated on a patterned piezoelectric actuator capable of suppressing the exciton fine structure splitting. By using a resonant two-photon excitation, we coherently drive the biexciton state and demonstrate experimentally that our device generates polarization-entangled photons with a fidelity of 0.978(5) and a concurrence of 0.97(1) taking into account the nonidealities stemming from the experimental setup. By combining fine-structure-dependent fidelity measurements and a theoretical model, we identify an exciton spin-scattering process as a possible residual decoherence mechanism. We suggest that this imperfection may be overcome using a modest Purcell enhancement so as to achieve fidelities >0.99, thus making quantum dots evenly matched with the best probabilistic entangled photon sources.