Decoherence due to charge noise is one of the central challenges in using spin qubits in semiconductor quantum dots as a platform for quantum information processing. Recently, it has been experimentally demonstrated in both Si and GaAs singlet-triplet qubits that the effects of charge noise can be suppressed if qubit operations are implemented using symmetric barrier control instead of the standard tilt control. Here, we investigate the key issue of whether the benefits of barrier control persist over the entire set of single-qubit gates by performing randomized benchmarking simulations. We find the surprising result that the improvement afforded by barrier control depends sensitively on the amount of spin noise: for the minimal nuclear spin noise levels present in Si, the coherence time improves by more than 2 orders of magnitude whereas in GaAs, by contrast the coherence time is essentially the same for barrier and tilt control. However, we establish that barrier control becomes beneficial if qubit operations are performed using a new family of composite pulses that reduce gate times by up to 90%. With these optimized pulses, barrier control is the best way to achieve high-fidelity quantum gates in singlet-triplet qubits.
Decoherence due to charge noise is one of the central challenges in using spin qubits in semiconductor quantum dots as a platform for quantum information processing. Recently, it has been experimentally demonstrated in both Si and GaAs singlet-triplet qubits that the effects of charge noise can be suppressed if qubit operations are implemented using symmetric barrier control instead of the standard tilt control. Here, we investigate the key issue of whether the benefits of barrier control persist over the entire set of single-qubit gates by performing randomized benchmarking simulations. We find the surprising result that the improvement afforded by barrier control depends sensitively on the amount of spin noise: for the minimal nuclear spin noise levels present in Si, the coherence time improves by more than 2 orders of magnitude whereas in GaAs, by contrast the coherence time is essentially the same for barrier and tilt control. However, we establish that barrier control becomes beneficial if qubit operations are performed using a new family of composite pulses that reduce gate times by up to 90%. With these optimized pulses, barrier control is the best way to achieve high-fidelity quantum gates in singlet-triplet qubits.
It has been recently demonstrated that a singlet-triplet spin qubit in semiconductor double quantum dots can be controlled by changing the height of the potential barrier between the two dots (``barrier control''), which has led to a considerable reduction of charge noises as compared with the traditional tilt control method. In this paper we show, through a molecular-orbital-theoretic calculation of double quantum dots influenced by a charged impurity, that the relative charge noise for a system under the barrier control not only is smaller than that for the tilt control but actually decreases as a function of an increasing exchange interaction. This is understood as a combined consequence of the greatly suppressed detuning noise when the two dots are symmetrically operated, as well as an enhancement of the interdot hopping energy of an electron when the barrier is lowered which in turn reduces the relative charge noise at large exchange interaction values. We have also studied the response of the qubit to charged impurities at different locations and found that the improvement of barrier control is least for impurities equidistant from the two dots due to the small detuning noise they cause but is otherwise significant along other directions.
It has been recently demonstrated that a singlet-triplet spin qubit in semiconductor double quantum dots can be controlled by changing the height of the potential barrier between the two dots (barrier control), which has led to a considerable reduction of charge noises as compared to the traditional tilt control method. In this paper we show, through a molecular-orbital-theoretic calculation of double quantum dots influenced by a charged impurity, that the relative charge noise for a system under the barrier control not only is smaller than that for the tilt control, but actually decreases as a function of an increasing exchange interaction. This is understood as a combined consequence of the greatly suppressed detuning noise when the two dots are symmetrically operated, as well as an enhancement of the inter-dot hopping energy of an electron when the barrier is lowered which in turn reduces the relative charge noise at large exchange interaction values. We have also studied the response of the qubit to charged impurities at different locations, and found that the improvement of barrier control is least for impurities equidistant from the two dots due to the small detuning noise they cause, but is otherwise significant along other directions.
A key ingredient for fault-tolerant quantum computers are sufficiently accurate logic gates on single and multiple qubits in the presence of decohering noise. In this thesis, we theoretically develop and experimentally demonstrate such high-fidelity quantum gates for semiconductor-based quantum computing. Specifically, we consider a qubit encoded in the singlet and one triplet state of two electron spins in GaAs. While its potential for optical coupling makes GaAs an attractive material, highly auto-correlated magnetic field noise from fluctuating nuclear spins leads to considerably lower coherence times than for Si-based devices, where nuclear spins can be removed by isotopic purification. In addition to noise, the control methods used in earlier experiments are based on unrealistic approximations. For these reasons, fidelities well above 99 %, as required by current quantum error correction (QEC) schemes, have not been obtained before this thesis. To tackle these issues, we extend the filter function formalism to describe quantum gates and processes in the presence of experimentally relevant non-Markovian noise. Since this formalism can consider all relevant noise sources in a computationally efficient manner, it can be used to find optimal control pulses by numerical optimization, leading to predicted single-qubit gate fidelities of 99.9 %. Furthermore, we deal with the considerable control challenges associated with this qubit type by experimental calibration of the optimized control pulses. To this end, we extend our previous experimental gate set calibration (GSC) routine to remove systematic gate errors on an arbitrary number of qubits. We apply the numerically optimized single-qubit control pulses to our GaAs sample and experimentally calibrate them with GSC. This procedure yields an average gate fidelity of 99.50 ± 0.04 % and a low leakage rate of 0.13 ± 0.03 % out of the computational subspace, characterized by randomized benchmarking. We also optimize realistic two-qubit control pulses, considering current control hardware as well as interqubit Coulomb and exchange coupling that cannot be fully turned off. Using measured noise spectra, we show that two-qubit gate fidelities of 99.90 % can be reached in GaAs, while 99.99 % can be achieved in Si. These results demonstrate that high-fidelity gates can be realized even in the presence of nuclear spins as in GaAs.
In order to enable semiconductor-based quantum computing with many qubits, issues like residual interqubit coupling and constraints from scalable control hardware need to be tackled to retain the high gate fidelities demonstrated in current single-qubit devices. Here we focus on two exchange-coupled singlet-triplet spin qubits, considering realistic control hardware as well as Coulomb and exchange coupling that cannot be fully turned off. Using measured noise spectra, we optimize realistic control pulses and show that two-qubit (single-qubit) gate fidelities of 99.90% ($\ensuremath{\ge}99.69%$) can be reached in GaAs, while 99.99% ($\ensuremath{\ge}99.95%$) can be achieved in Si.
We analyze a simple exchange-based two-qubit gate for singlet-triplet qubits in gate-defined semiconductor quantum dots that can be implemented in a single exchange pulse. Excitations from the logical subspace are suppressed by a magnetic field gradient that causes spin-flip transitions to be non-energy-conserving. We show that the use of adiabatic pulses greatly reduces leakage processes comapred to square pulses. We also characterize the effect of charge noise on the entanglement fidelity of the gate both analytically and in simulations; demonstrating high entanglement fidelities for physically realistic experimental parameters. Specifically we find that it is possible to achieve fidelities and gate times that are comparable to single-qubit states using realistic magnetic field gradients.
Electron spins confined in semiconductor quantum dots are emerging as a promising system to study quantum information science and to perform sensitive metrology. Their weak interaction with the environment leads to long coherence times and robust storage for quantum information, and the intrinsic tunability of semiconductors allows for controllable operations, initialization, and readout of their quantum state. These spin qubits are also promising candidates for the building block for a scalable quantum information processor due to their prospects for scalability and miniaturization. owever, several obstacles limit the performance of quantum information experiments in these systems. For example, the weak coupling to the environment makes inter-qubit operations challenging, and a fluctuating nuclear magnetic field limits the performance of single-qubit operations.\n\n\n\nThe focus of this thesis will be several experiments which address some of the outstanding problems in semiconductor spin qubits, in particular, singlet-triplet (S-T0) qubits. We use these qubits to probe both the electric field and magnetic field noise that limit the performance of these qubits. The magnetic noise bath is probed with high bandwidth and precision using novel techniques borrowed from the field of Hamiltonian learning, which are effective due to the rapid control and readout available in S-T0 qubits. These findings allow us to effectively undo the undesired effects of the fluctuating nuclear magnetic field by tracking them in real-time, and we demonstrate a 30-fold improvement in the coherence time T2*.\n\n\n\nWe probe the voltage noise environment of the qubit using coherent qubit oscillations, which is partially enabled by control of the nuclear magnetic field. We find that the voltage noise bath is frequency- dependent, even at frequencies as high as 1MHz, and it shows surprising and, as of yet, unexplained temperature dependence. We leverage this knowledge of the voltage noise environment, the nuclear magnetic field control, as well as new techniques for calibrated measurement of the density matrix in a singlet-triplet qubit to entangle two adjacent single-triplet qubits. We fully characterize the generated entangled states and prove that they are, indeed, entangled.\n\n\n\nThis work opens new opportunities to use qubits as sensors for improved metrological capabilities, as well as for improved quantum information processing. The singlet-triplet qubit is unique in that it can be used to probe two fundamentally different noise baths, which are important for a large variety of solid state qubits. More specifically, this work establishes the singlet-triplet qubit as a viable candidate for the building block of a scalable quantum information processor.