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arXiv:1701.01454 · Physical review. B./Physical review. B

Many-body interferometry of magnetic polaron dynamics

Yuto Ashida, Richard Schmidt, Leticia Tarruell, Eugene Demler

Published Feb 20, 2018• 42 citations
arXivHTMLPDF

Abstract

The physics of quantum impurities coupled to a many-body environment is among the most important paradigms of condensed-matter physics. In particular, the formation of polarons, quasiparticles dressed by the polarization cloud, is key to the understanding of transport, optical response, and induced interactions in a variety of materials. Despite recent remarkable developments in ultracold atoms and solid-state materials, the direct measurement of their ultimate building block, the polaron cloud, has remained a fundamental challenge. We propose and analyze a platform to probe time-resolved dynamics of polaron-cloud formation with an interferometric protocol. We consider an impurity atom immersed in a two-component Bose-Einstein condensate where the impurity generates spin-wave excitations that can be directly measured by the Ramsey interference of surrounding atoms. The dressing by spin waves leads to the formation of magnetic polarons and reveals a unique interplay between few- and many-body physics that is signified by single- and multi-frequency oscillatory dynamics corresponding to the formation of many-body bound states. Finally, we discuss concrete experimental implementations in ultracold atoms.

DOI
10.1103/physrevb.97.060302

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The physics of quantum impurities coupled to a many-body environment is among the most important paradigms of condensed-matter physics. In particular, the formation of polarons, quasiparticles dressed by the polarization cloud, is key to the understanding of transport, optical response, and induced interactions in a variety of materials. Despite recent remarkable developments in ultracold atoms and solid-state materials, the direct measurement of their ultimate building block, the polaron cloud, has remained a fundamental challenge. We propose and analyze a platform to probe time-resolved dynamics of polaron-cloud formation with an interferometric protocol. We consider an impurity atom immersed in a two-component Bose-Einstein condensate where the impurity generates spin-wave excitations that can be directly measured by the Ramsey interference of surrounding atoms. The dressing by spin waves leads to the formation of magnetic polarons and reveals a unique interplay between few- and many-body physics that is signified by single- and multi-frequency oscillatory dynamics corresponding to the formation of many-body bound states. Finally, we discuss concrete experimental implementations in ultracold atoms.
In recent years, Rydberg excitations in atomic quantum gases have become a successful platform to explore quantum impurity problems. A single impurity immersed in a Fermi gas leads to the formation of a polaron, a quasiparticle consisting of the impurity being dressed by the surrounding medium. With a radius of about the Fermi wavelength, the density profile of a polaron cannot be explored using in situ optical imaging techniques. In this Letter, we propose a new experimental measurement technique that enables the in situ imaging of the polaron cloud in ultracold quantum gases. The impurity atom induces the formation of a polaron cloud and is then excited to a Rydberg state. Because of the mesoscopic interaction range of Rydberg excitations, which can be tuned by the principal numbers of the Rydberg state, atoms extracted from the polaron cloud form dimers with the impurity. By performing first principle calculations of the absorption spectrum based on a functional determinant approach, we show how the occupation of the dimer state can be directly observed in spectroscopy experiments and can be mapped onto the density profile of the gas particles, hence providing a direct, real-time, and in situ measure of the polaron cloud.
Advancing our understanding of non-equilibrium phenomena in quantum many-body systems remains one of the greatest challenges in physics. Here we report on the experimental observation of a paradigmatic many-body problem, namely the non-equilibrium dynamics of a quantum impurity immersed in a bosonic environment1,2. We use an interferometric technique to prepare coherent superposition states of atoms in a Bose–Einstein condensate with a small impurity-state component, and monitor the evolution of such quantum superpositions into polaronic quasiparticles. These results offer a systematic picture of polaron formation3–7 from weak to strong impurity interactions. They reveal three distinct regimes of evolution with dynamical transitions that provide a link between few-body processes and many-body dynamics. Our measurements reveal universal dynamical behaviour in interacting many-body systems and demonstrate new pathways to study non-equilibrium quantum phenomena. Quantum impurities immersed in a bosonic environment can evolve into polaronic quasiparticles, so-called polarons. Interferometric measurement reveals this transition, which involves three different regimes dominated by few-body and many-body dynamics.
Spectroscopic and interferometric measurements complement each other in extracting the fundamental properties of quantum many-body systems. While spectroscopy provides precise measurements of equilibrated energies, interferometry can elucidate the dynamical evolution of the system. For an impurity immersed in a bosonic medium, both are equally important for understanding the quasiparticle physics of the Bose polaron. Here, we compare the interferometric and spectroscopic timescales to the underlying dynamical regimes of the impurity dynamics and the polaron lifetime, highlighting the capability of the interferometric approach to clearly resolve polaron dynamics. In particular, interferometric measurements of the coherence amplitude at strong interactions reveal faster quantum dynamics at large repulsive interaction strengths than at unitarity. These observations are in excellent agreement with a short-time theoretical prediction including both the continuum and the attractive polaron branch. For longer times, qualitative agreement with a many-body theoretical prediction which includes both branches is obtained. Moreover, the polaron energy is extracted from interferometric measurements of the observed phase velocity in agreement with previous spectroscopic results from weak to strong attractive interactions. Finally, the phase evolution allows for the measurement of an energetic equilibration timescale, describing the initial approach of the phase velocity to the polaron energy. Theoretically, this is shown to lie within the regime of universal dynamics revealing a fast initial evolution towards the formation of polarons. Our results give a comprehensive picture of the many-body physics governing the Bose polaron and thus validates the quasiparticle framework for further studies.
Important properties of complex quantum many-body systems and their phase diagrams can often already be inferred from the impurity limit. The Bose polaron problem describing an impurity atom immersed in a Bose-Einstein condensate is a paradigmatic example. The interplay between the impurity-mediated attraction between the bosons and their intrinsic repulsion makes this model rich and interesting, but also complex to describe theoretically. To tackle this challenge, we develop a quantum chemistry-inspired computational technique and compare two variational methods that fully include both the boson-impurity and interboson interactions. We find one regime where the impurity-mediated interactions overcome the repulsion between the bosons, so that a sweep of the boson-impurity interaction strength leads to an instability of the polaron due to the formation of many-body clusters. If instead the interboson interactions dominate, the impurity will experience a crossover from a polaron into a few-body bound state. We achieve a unified understanding incorporating both of these regimes and show that they are experimentally accessible. Moreover, we develop an analytical model that allows us to interpret these phenomena in the Landau framework of phase transitions, revealing a deep connection of the Bose polaron model to both few- and many-body physics.
Abstract Lattice polarons, quasiparticles arising from the interaction between an impurity and its surrounding bosonic environment confined to a lattice system, have emerged as a platform for generating complex few-body states, probing many-body phenomena, and addressing long-standing problems in physics. In this study, we employ a variational ansatz to investigate the quasiparticle and spectral properties of an impurity coupled to a condensate gas of hard-core bosons in a two-dimensional optical lattice. Our findings demonstrate that the polaron features can be tuned by adjusting the filling factor of the bath, revealing intriguing polaron characteristics in the strongly interacting regime. These results offer valuable insights for lattice polaron experiments with ultracold gases and can serve as a guide for new experiments in emergent quantum devices, such as moiré materials, where optical excitations can be described in terms of hard-core bosons.
The physics of impurities in a bosonic quantum environment is a paradigmatic and challenging many-body problem. Here, this problem is investigated for impurities with strong repulsive interactions based on Ramsey interferometry in a quantum degenerate gas of K 39 atoms. We observe revivals in the amplitude of the interferometric signal and identify them as beat signals between two coexisting quasiparticle branches, the attractive and repulsive polarons. The interferometric signal allows for an extraction of their energies for a wide range of interaction strengths, thus resolving outstanding discrepancies in earlier spectroscopic measurements. Furthermore, we identify several dynamical regimes in the formation of the repulsive Bose polaron. Our results improve the understanding of quantum impurities interacting strongly with a bosonic environment and show how short-lived nonequilibrium many-body states can be probed using quantum beat spectroscopy.