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arXiv:2310.18183 · Physical Review Research

Quantum beat spectroscopy of repulsive Bose polarons

Andreas M. Morgen, S. S. Balling, K. Knakkergaard Nielsen, Thomas Pohl, Georg M. Bruun, J. Arlt

Published Apr 2, 2025• 6 citations
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Abstract

The physics of impurities in a bosonic quantum environment is a paradigmatic and challenging many-body problem. Here, this problem is investigated for impurities with strong repulsive interactions based on Ramsey interferometry in a quantum degenerate gas of K 39 atoms. We observe revivals in the amplitude of the interferometric signal and identify them as beat signals between two coexisting quasiparticle branches, the attractive and repulsive polarons. The interferometric signal allows for an extraction of their energies for a wide range of interaction strengths, thus resolving outstanding discrepancies in earlier spectroscopic measurements. Furthermore, we identify several dynamical regimes in the formation of the repulsive Bose polaron. Our results improve the understanding of quantum impurities interacting strongly with a bosonic environment and show how short-lived nonequilibrium many-body states can be probed using quantum beat spectroscopy.

DOI
10.1103/physrevresearch.7.l022002

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The physics of impurities in a bosonic quantum environment is a paradigmatic and challenging many-body problem. Here, this problem is investigated for impurities with strong repulsive interactions based on Ramsey interferometry in a quantum degenerate gas of K 39 atoms. We observe revivals in the amplitude of the interferometric signal and identify them as beat signals between two coexisting quasiparticle branches, the attractive and repulsive polarons. The interferometric signal allows for an extraction of their energies for a wide range of interaction strengths, thus resolving outstanding discrepancies in earlier spectroscopic measurements. Furthermore, we identify several dynamical regimes in the formation of the repulsive Bose polaron. Our results improve the understanding of quantum impurities interacting strongly with a bosonic environment and show how short-lived nonequilibrium many-body states can be probed using quantum beat spectroscopy.
Spectroscopic and interferometric measurements complement each other in extracting the fundamental properties of quantum many-body systems. While spectroscopy provides precise measurements of equilibrated energies, interferometry can elucidate the dynamical evolution of the system. For an impurity immersed in a bosonic medium, both are equally important for understanding the quasiparticle physics of the Bose polaron. Here, we compare the interferometric and spectroscopic timescales to the underlying dynamical regimes of the impurity dynamics and the polaron lifetime, highlighting the capability of the interferometric approach to clearly resolve polaron dynamics. In particular, interferometric measurements of the coherence amplitude at strong interactions reveal faster quantum dynamics at large repulsive interaction strengths than at unitarity. These observations are in excellent agreement with a short-time theoretical prediction including both the continuum and the attractive polaron branch. For longer times, qualitative agreement with a many-body theoretical prediction which includes both branches is obtained. Moreover, the polaron energy is extracted from interferometric measurements of the observed phase velocity in agreement with previous spectroscopic results from weak to strong attractive interactions. Finally, the phase evolution allows for the measurement of an energetic equilibration timescale, describing the initial approach of the phase velocity to the polaron energy. Theoretically, this is shown to lie within the regime of universal dynamics revealing a fast initial evolution towards the formation of polarons. Our results give a comprehensive picture of the many-body physics governing the Bose polaron and thus validates the quasiparticle framework for further studies.
Advancing our understanding of non-equilibrium phenomena in quantum many-body systems remains one of the greatest challenges in physics. Here we report on the experimental observation of a paradigmatic many-body problem, namely the non-equilibrium dynamics of a quantum impurity immersed in a bosonic environment1,2. We use an interferometric technique to prepare coherent superposition states of atoms in a Bose–Einstein condensate with a small impurity-state component, and monitor the evolution of such quantum superpositions into polaronic quasiparticles. These results offer a systematic picture of polaron formation3–7 from weak to strong impurity interactions. They reveal three distinct regimes of evolution with dynamical transitions that provide a link between few-body processes and many-body dynamics. Our measurements reveal universal dynamical behaviour in interacting many-body systems and demonstrate new pathways to study non-equilibrium quantum phenomena. Quantum impurities immersed in a bosonic environment can evolve into polaronic quasiparticles, so-called polarons. Interferometric measurement reveals this transition, which involves three different regimes dominated by few-body and many-body dynamics.
Important properties of complex quantum many-body systems and their phase diagrams can often already be inferred from the impurity limit. The Bose polaron problem describing an impurity atom immersed in a Bose-Einstein condensate is a paradigmatic example. The interplay between the impurity-mediated attraction between the bosons and their intrinsic repulsion makes this model rich and interesting, but also complex to describe theoretically. To tackle this challenge, we develop a quantum chemistry-inspired computational technique and compare two variational methods that fully include both the boson-impurity and interboson interactions. We find one regime where the impurity-mediated interactions overcome the repulsion between the bosons, so that a sweep of the boson-impurity interaction strength leads to an instability of the polaron due to the formation of many-body clusters. If instead the interboson interactions dominate, the impurity will experience a crossover from a polaron into a few-body bound state. We achieve a unified understanding incorporating both of these regimes and show that they are experimentally accessible. Moreover, we develop an analytical model that allows us to interpret these phenomena in the Landau framework of phase transitions, revealing a deep connection of the Bose polaron model to both few- and many-body physics.
When an impurity is immersed in a Bose-Einstein condensate, impurity-boson interactions are expected to dress the impurity into a quasiparticle, the Bose polaron. We superimpose an ultracold atomic gas of ^{87}Rb with a much lower density gas of fermionic ^{40}K impurities. Through the use of a Feshbach resonance and radio-frequency spectroscopy, we characterize the energy, spectral width, and lifetime of the resultant polaron on both the attractive and the repulsive branches in the strongly interacting regime. The width of the polaron in the attractive branch is narrow compared to its binding energy, even as the two-body scattering length diverges.
The problem of an impurity particle moving through a bosonic medium plays a fundamental role in physics.However, the canonical scenario of a mobile impurity immersed in a Bose-Einstein condensate (BEC) has not yet been realized.Here, we use radio frequency spectroscopy of ultracold bosonic 39 K atoms to experimentally demonstrate the existence of a well-defined quasiparticle state of an impurity interacting with a BEC.We measure the energy of the impurity both for attractive and repulsive interactions, and find excellent agreement with theories that incorporate three-body correlations, both in the weak-coupling limits and across unitarity.The spectral response consists of a well-defined quasiparticle peak at weak coupling, while for increasing interaction strength, the spectrum is strongly broadened and becomes dominated by the many-body continuum of excited states.Crucially, no significant effects of three-body decay are observed.Our results open up exciting prospects for studying mobile impurities in a bosonic environment and strongly interacting Bose systems in general.
The problem of an impurity particle moving through a bosonic medium plays a fundamental role in physics. However, the canonical scenario of a mobile impurity immersed in a Bose-Einstein condensate (BEC) has not yet been realized. Here, we use radio frequency spectroscopy of ultracold bosonic ^{39}K atoms to experimentally demonstrate the existence of a well-defined quasiparticle state of an impurity interacting with a BEC. We measure the energy of the impurity both for attractive and repulsive interactions, and find excellent agreement with theories that incorporate three-body correlations, both in the weak-coupling limits and across unitarity. The spectral response consists of a well-defined quasiparticle peak at weak coupling, while for increasing interaction strength, the spectrum is strongly broadened and becomes dominated by the many-body continuum of excited states. Crucially, no significant effects of three-body decay are observed. Our results open up exciting prospects for studying mobile impurities in a bosonic environment and strongly interacting Bose systems in general.