Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1612.07225 · Physical Review A

Quantum spectroscopy of single spins assisted by a classical clock

Tuvia Gefen, Maxim Khodas, Liam Paul McGuinness, Fedor Jelezko, Alex Retzker

Published Jul 27, 2018• 20 citations
arXivHTMLPDF

Abstract

Quantum spectroscopy with single two-level systems has considerably improved our ability to detect weak signals. Recently it was realized that for classical signals, precision and resolution of quantum spectroscopy is limited mainly by coherence of the signal and the stability of the clock used to measure time. The coherence time of the quantum probe, which can be significantly shorter, is not a major limiting factor in resolution measurements. Here, we address a similar question for spectroscopy of quantum signals, for example, a quantum sensor is used to detect a single nuclear spin. We present and analyze a novel correlation spectroscopy technique with performance that is limited by the coherence time of the target spins and the stability of the clock.

DOI
10.1103/physreva.98.013844

Related papers

Classical memory assisted correlation spectroscopy of quantum signals

Maxim Khodas, Tuvia Gefen, Liam Paul McGuinness +2 more

Quantum spectroscopy with single qubits has improved considerably our ability to detect weak signals arising from classical and quantum sources. Recently, the use of additional memory qubits in quantum spectroscopy has allowed a resolution beyond the sensor coherence time to be reached. Alternatively, combining a classical clock allows for spectroscopy of classical fields with a resolution given by the clock coherence time. We present a novel correlation spectroscopy technique with resolution that is limited by the coherence time of the classical clock. This method is capable of screening the classical signal while still being able to detect the quantum one.

•Dec 21, 2016•0 citations

High-resolution spectroscopy of single nuclear spins via sequential weak measurements

Matthias Pfender, Ping Wang, Hitoshi Sumiya +8 more

Abstract Nuclear magnetic resonance (NMR) of single spins have recently been detected by quantum sensors. However, the spectral resolution has been limited by the sensor’s relaxation to a few kHz at room temperature. This can be improved by using quantum memories, at the expense of sensitivity. In contrast, classical signals can be measured with exceptional spectral resolution by using continuous measurement techniques, without compromising sensitivity. When applied to single-spin NMR, it is critical to overcome the impact of back action inherent of quantum measurement. Here we report sequential weak measurements on a single 13C nuclear spin. The back-action causes the spin to undergo a quantum dynamics phase transition from coherent trapping to coherent oscillation. Single-spin NMR at room-temperature with a spectral resolution of 3.8 Hz is achieved. These results enable the use of measurement-correlation schemes for the detection of very weakly coupled single spins.

arXiv:1806.02181•Nature Communications•Feb 5, 2019•94 citations

Precise Spectroscopy of High-Frequency Oscillating Fields with a Single-Qubit Sensor

Yaoming Chu, Pengcheng Yang, Musang Gong +5 more

Precise spectroscopy of oscillating fields plays a significant role in many fields. Here, we propose an experimentally feasible scheme to measure the frequency of a fast-oscillating field using a single-qubit sensor. By invoking a stable classical clock, the signal phase correlations between successive measurements enable us to extract the target frequency with extremely high precision. In addition, we integrate dynamical decoupling technique into the framework to suppress the influence of slow environmental noise. Our framework is feasible with a variety of atomic and single solid-state spin systems within the state-of-the-art experimental capabilities as a versatile tool for quantum spectroscopy.

arXiv:2009.05458•Physical Review Applied•Jan 19, 2021•16 citations

Enhancing quantum sensing sensitivity by a quantum memory

Sebastian Zaiser, Torsten Rendler, Ingmar Jakobi +7 more

In quantum sensing, precision is typically limited by the maximum time interval over which phase can be accumulated. Memories have been used to enhance this time interval beyond the coherence lifetime and thus gain precision. Here, we demonstrate that by using a quantum memory an increased sensitivity can also be achieved. To this end, we use entanglement in a hybrid spin system comprising a sensing and a memory qubit associated with a single nitrogen-vacancy centre in diamond. With the memory we retain the full quantum state even after coherence decay of the sensor, which enables coherent interaction with distinct weakly coupled nuclear spin qubits. We benchmark the performance of our hybrid quantum system against use of the sensing qubit alone by gradually increasing the entanglement of sensor and memory. We further apply this quantum sensor-memory pair for high-resolution NMR spectroscopy of single (13)C nuclear spins.

Nature Communications•Aug 10, 2016•180 citations

Precise Spectroscopy of High-Frequency Oscillating Fields with a Single-Qubit Sensor

Yaoming Chu, Pengcheng Yang, Musang Gong +5 more

Precise spectroscopy of oscillating fields plays a significant role in many fields. Here, we propose an experimentally feasible scheme to measure the frequency of a fast-oscillating field using a single-qubit sensor. By invoking a stable classical clock, the signal phase correlations between successive measurements enable us to extract the target frequency with extremely high precision. In addition, we integrate dynamical decoupling technique into the framework to suppress the influence of slow environmental noise. Our framework is feasible with a variety of atomic and single solid-state spin systems within the state-of-the-art experimental capabilities as a versatile tool for quantum spectroscopy.

•Jan 1, 2021•8 citations

Overcoming Frequency Resolution Limits Using a Solid-State Spin Quantum Sensor

Qingyun Cao, Genko T. Genov, Yaoming Chu +4 more

The ability to determine precisely the separation of two frequencies is fundamental to spectroscopy, yet the resolution limit poses a critical challenge: distinguishing two incoherent signals becomes impossible when their frequencies are sufficiently close. Here, we demonstrate a simple and powerful approach, dubbed superresolution quantum sensing, which experimentally resolves two nearly identical incoherent signals using a solid-state spin quantum sensor. By carefully choosing interrogation times that satisfy the superresolution condition, we eliminate quantum projection noise, overcoming the vanishing distinguishability of signals with near-identical frequencies. This leads to improved resolution, which scales as t^{-2} in comparison to the standard t^{-1} scaling. Together with a greatly reduced classical readout noise assisted by a nuclear spin, we are able to achieve sub-kHz resolution with a signal detection time of 80 μs. Our results highlight the potential of quantum sensing to overcome conventional frequency resolution limitations, with broad implications for precision measurements.

arXiv:2506.20416•Physical Review Letters•Nov 24, 2025•0 citations
Quantum spectroscopy with single two-level systems has considerably improved our ability to detect weak signals. Recently it was realized that for classical signals, precision and resolution of quantum spectroscopy is limited mainly by coherence of the signal and the stability of the clock used to measure time. The coherence time of the quantum probe, which can be significantly shorter, is not a major limiting factor in resolution measurements. Here, we address a similar question for spectroscopy of quantum signals, for example, a quantum sensor is used to detect a single nuclear spin. We present and analyze a novel correlation spectroscopy technique with performance that is limited by the coherence time of the target spins and the stability of the clock.
Quantum spectroscopy with single qubits has improved considerably our ability to detect weak signals arising from classical and quantum sources. Recently, the use of additional memory qubits in quantum spectroscopy has allowed a resolution beyond the sensor coherence time to be reached. Alternatively, combining a classical clock allows for spectroscopy of classical fields with a resolution given by the clock coherence time. We present a novel correlation spectroscopy technique with resolution that is limited by the coherence time of the classical clock. This method is capable of screening the classical signal while still being able to detect the quantum one.
Abstract Nuclear magnetic resonance (NMR) of single spins have recently been detected by quantum sensors. However, the spectral resolution has been limited by the sensor’s relaxation to a few kHz at room temperature. This can be improved by using quantum memories, at the expense of sensitivity. In contrast, classical signals can be measured with exceptional spectral resolution by using continuous measurement techniques, without compromising sensitivity. When applied to single-spin NMR, it is critical to overcome the impact of back action inherent of quantum measurement. Here we report sequential weak measurements on a single 13C nuclear spin. The back-action causes the spin to undergo a quantum dynamics phase transition from coherent trapping to coherent oscillation. Single-spin NMR at room-temperature with a spectral resolution of 3.8 Hz is achieved. These results enable the use of measurement-correlation schemes for the detection of very weakly coupled single spins.
Precise spectroscopy of oscillating fields plays a significant role in many fields. Here, we propose an experimentally feasible scheme to measure the frequency of a fast-oscillating field using a single-qubit sensor. By invoking a stable classical clock, the signal phase correlations between successive measurements enable us to extract the target frequency with extremely high precision. In addition, we integrate dynamical decoupling technique into the framework to suppress the influence of slow environmental noise. Our framework is feasible with a variety of atomic and single solid-state spin systems within the state-of-the-art experimental capabilities as a versatile tool for quantum spectroscopy.
In quantum sensing, precision is typically limited by the maximum time interval over which phase can be accumulated. Memories have been used to enhance this time interval beyond the coherence lifetime and thus gain precision. Here, we demonstrate that by using a quantum memory an increased sensitivity can also be achieved. To this end, we use entanglement in a hybrid spin system comprising a sensing and a memory qubit associated with a single nitrogen-vacancy centre in diamond. With the memory we retain the full quantum state even after coherence decay of the sensor, which enables coherent interaction with distinct weakly coupled nuclear spin qubits. We benchmark the performance of our hybrid quantum system against use of the sensing qubit alone by gradually increasing the entanglement of sensor and memory. We further apply this quantum sensor-memory pair for high-resolution NMR spectroscopy of single (13)C nuclear spins.
Precise spectroscopy of oscillating fields plays a significant role in many fields. Here, we propose an experimentally feasible scheme to measure the frequency of a fast-oscillating field using a single-qubit sensor. By invoking a stable classical clock, the signal phase correlations between successive measurements enable us to extract the target frequency with extremely high precision. In addition, we integrate dynamical decoupling technique into the framework to suppress the influence of slow environmental noise. Our framework is feasible with a variety of atomic and single solid-state spin systems within the state-of-the-art experimental capabilities as a versatile tool for quantum spectroscopy.
The ability to determine precisely the separation of two frequencies is fundamental to spectroscopy, yet the resolution limit poses a critical challenge: distinguishing two incoherent signals becomes impossible when their frequencies are sufficiently close. Here, we demonstrate a simple and powerful approach, dubbed superresolution quantum sensing, which experimentally resolves two nearly identical incoherent signals using a solid-state spin quantum sensor. By carefully choosing interrogation times that satisfy the superresolution condition, we eliminate quantum projection noise, overcoming the vanishing distinguishability of signals with near-identical frequencies. This leads to improved resolution, which scales as t^{-2} in comparison to the standard t^{-1} scaling. Together with a greatly reduced classical readout noise assisted by a nuclear spin, we are able to achieve sub-kHz resolution with a signal detection time of 80 μs. Our results highlight the potential of quantum sensing to overcome conventional frequency resolution limitations, with broad implications for precision measurements.