This thesis offers novel strategies for the measurement of quantum correlations present in controllable quantum systems, as well as for a full-fledged implementation of the models of light-matter interaction through which these correlations can be generated. We propose the use of an ancillary qubit to efficiently access both time-correlation functions and entanglement monotones, and we provide two experimental demonstrations of our methods, measuring time correlations in an NMR setup and entanglement monotones in a photonic system. Moreover, we explain how time-correlation functions could be exploited for the quantum simulation of open quantum dynamics, and we provide an experimental recipe for the measurement of entanglement monotones in trapped ion technologies. On the other hand, we explore the quantum simulation of quantum optical models of light-matter interaction for inaccessible coupling regimes, providing experimental proposals for their implementation, both in ions and superconducting circuits. Finally, we also provide an experimental proposal for the quantum simulation of spin models in trapped ions following a digital-analog simulation scheme.
This thesis offers novel strategies for the measurement of quantum correlations present in controllable quantum systems, as well as for a full-fledged implementation of the models of light-matter interaction through which these correlations can be generated. We propose the use of an ancillary qubit to efficiently access both time-correlation functions and entanglement monotones, and we provide two experimental demonstrations of our methods, measuring time correlations in an NMR setup and entanglement monotones in a photonic system. Moreover, we explain how time-correlation functions could be exploited for the quantum simulation of open quantum dynamics, and we provide an experimental recipe for the measurement of entanglement monotones in trapped ion technologies. On the other hand, we explore the quantum simulation of quantum optical models of light-matter interaction for inaccessible coupling regimes, providing experimental proposals for their implementation, both in ions and superconducting circuits. Finally, we also provide an experimental proposal for the quantum simulation of spin models in trapped ions following a digital-analog simulation scheme.
Quantum simulation platforms such as cold atoms, superconducting circuits, and trapped ions enable the experimental investigation of quantum many-body systems, with important implications for quantum technologies. In this thesis, we investigate how entanglement and correlations develop in such systems and how they can be harnessed both for the theoretical study of models relevant to condensed matter physics and for practical applications in quantum metrology. We begin by focusing on the adiabatic preparation of quantum many-body ground states. In particular, we show that quantum simulators can probe the link between spectral degeneracy and Spontaneous Symmetry Breaking, as pioneered by P.W. Anderson. We prove that odd-sized spin-½ systems exhibiting time-reversal symmetry sustain a net magnetization even away from the thermodynamic limit, thanks to an exact spectral degeneracy. Moreover, the symmetry-broken state exhibits scalable spin squeezing, a key resource for quantum metrology. We then turn to a different paradigm of evolution: quench dynamics. In particular, we show that monitoring the real-time evolution of correlations allows for the experimental measurement of the dispersion relation of fundamental excitations. In the case of two-dimensional long-range ordered systems, such as the dipolar XY model, these excitations are spin waves, leading to sharp features in the evolution of two-point correlation functions. Conversely, in one-dimensional systems, fundamental excitations have a fermionic nature, and their detection requires the measurement of non-local correlation functions. The latter, while inaccessible in condensed matter, are instead well suited to quantum simulators with individually addressable degrees of freedom.
Abstract Light-matter interactions are an established field that is experiencing a renaissance in recent years due to the introduction of exotic coupling regimes. These include the ultrastrong and deep-strong coupling regimes, where the coupling constant is smaller and of the order of the frequency of the light mode, or larger than this frequency, respectively. In the past few years, quantum simulations of light-matter interactions in all possible coupling regimes have been proposed and experimentally realized, in quantum platforms such as trapped ions, superconducting circuits, cold atoms, and quantum photonics. We review this fledgling field, illustrating the benefits and challenges of the quantum simulations of light-matter interactions with quantum technologies.
In this Thesis we design radiation patterns capable of creating effective light-matter interactions suited to applications in quantum computing, quantum simulation and quantum sensing. On the one hand, we have used dynamical decoupling techniques to design quantum operations that are robust against errors in environmental and control fields, achieving high-fidelity quantum logic in trapped ions and energy-efficient nuclear magnetic resonance at the nanoscale with nitrogen-vacancy centers in diamond. On the other hand, we have studied generalised models of light-matter interaction, leading to the discovery of selective multi-photon interactions in the Rabi-Stark model and a proposal for preparing non-classical quantum states using the nonlinear quantum Rabi model. Finally, we have shown how the appropriate tailoring of interactions among ultracold atoms in optical lattices could lead to solve the boson sampling problem faster than the best supercomputers, thus demonstrating quantum supremacy. In this manner, we believe the results presented here significantly expand our knowledge on the control of light-matter interactions, and provide optimal scenarios for current quantum devices to generate the next-generation of quantum applications.
Simulation of the interaction of light with matter, including at the few-photon level, is important for understanding the optical and optoelectronic properties of materials and for modeling next-generation nonlinear spectroscopies that use entangled light. At the few-photon level the quantum properties of the electromagnetic field must be accounted for with a quantized treatment of the field, and then such simulations quickly become intractable, especially if the matter subsystem must be modeled with a large number of degrees of freedom, as can be required to accurately capture many-body effects and quantum noise sources. Motivated by this we develop a quantum simulation framework for simulating such light-matter interactions on platforms with controllable bosonic degrees of freedom, such as vibrational modes in the trapped ion platform. The key innovation in our work is a scheme for simulating interactions with a continuum field using only a few discrete bosonic modes, which is enabled by a Green's function (response function) formalism. We develop the simulation approach, sketch how the simulation can be performed using trapped ions, and then illustrate the method with numerical examples. Our work expands the reach of quantum simulation to important light-matter interaction models and illustrates the advantages of extracting dynamical quantities such as response functions from quantum simulations.
Quantum networks are composed of quantum nodes which coherently interact by way of quantum channels. They offer powerful capabilities for quantum computation, communication, and metrology. A generic requirement for these realizations is the capability to generate and store quantum states among multiple quantum nodes, and to disseminate these resources throughout the network via the quantum channels. In this thesis, I describe a series of experiments whereby single excitations in atomic ensembles are strongly coupled to optical modes and provide efficient means for the coherent control of entangled states between matter and light. By following the seminal proposal by Duan et al., we have generated measurement-induced entanglement of an excitation between two cold atomic ensembles. Using this system, we investigated the relationship for the global bipartite entanglement and local correlations in its subsystems. In addition, we achieved functional quantum nodes for entanglement distribution. Two pairs of remote ensembles at two quantum nodes were prepared into entangled states in a heralded and asynchronous fashion by the conditional controls of the entanglement. The quantum states of the ensembles were then distributed into polarization entangled states of photons. We also prepared an analogous quantum state and transferred the nonlocal coherence between two pairs of heralded entangled atomic ensembles, providing a step towards entanglement connection. Beyond such probabilistic approaches, we demonstrated an experiment where entanglement between two quantum memories is created by the reversible and deterministic mapping of an entangled state of light via dynamic electromagnetically induced transparency. This experiment opens novel prospects of integrating hybrid quantum systems by way of reversible quantum interfaces between light and matter. Then, we extended our work to multipartite quantum systems. We theoretically investigated the characterization of multipartite mode-entangled states by way of quantum uncertainty relations, and introduced theoretical tools to verify the entanglement orders in multipartite systems. In particular, we achieved entanglement for one delocalized photon among multiple optical modes (N > 2). Finally, we have achieved measurement-induced entanglement of spin waves among four quantum memories. The individual atomic components for the entangled W state of the four ensembles were then coherently converted into four propagating entangled beams of light via superradiant emissions. We observed the statistical and dynamic transitions for the multipartite entangled spin waves. Experiments described in this thesis thereby represent significant advances of experimental and theoretical capabilities to generate, store, transfer, and characterize entanglement of matter and light over quantum networks.
Although quantum mechanics has been able to explain a wide range of physical, chemical, and even biological events with unprecedented accuracy, fundamental problems remain. For instance, the problem of quantum measurement and quantum entanglement, which are the most perplexing problems that have persisted since the foundation of quantum mechanics. Both are crucial quantum resources with broad applications in quantum information science, quantum computing and quantum optics. For this reason, this thesis is devoted to research the quantum measurement from the weakest regime to the strongest one as well as the dynamics of entanglement of different quantum systems. In this work, we study the measurement transition for a coherent-squeezed pointer state through a transition factor Γ that involves a system-pointer coupling by using an arbitrary measured observable A. In addition, we show that the shift in the pointer’s position and momentum establishes a relationship with a new value defined as the transition value, which generalizes the weak value as well as the conditional expectation value. Furthermore, a new strategy is introduced to achieve different measurement regimes by just adjusting the r and ϕξ parameters of the coherent-squeezed pointer state, opening an interesting way to test quantum mechanics foundations. Our scheme has been theoretically applied in a trapped ion illuminated by a bichromatic laser beam, with a high potential to be implemented in future experimental setups. Besides, we propose a method to regulate the quantum entanglement in the system mentioned before as well as a dispersive-hybrid system where a qubit is directly coupled to a cavity and a mechanical resonator. Entanglement can be controlled by only tuning the squeezing parameters associated with the vibrational mode. As the squeezing amplitude becomes larger, the maximal entanglement abruptly falls to zero at specific squeezing phases. For the hybrid system, it is also possible to generate entanglement for bipartitions from the qubit-cavity-resonator system after applying this strategy. Entangled qubit-cavity states are created through squeezing, even though there is no direct interaction between them. We also analyze the effect of atomic, optical, and vibrational losses on the quantum entanglement. We finally discuss our schemes to be implemented in future experimental setups and promote further studies to generalize the concept of “monogamy of entanglement” in tripartite systems outside qubit-composite states, in particular, (2 ⊗ 2 ⊗ n)-dimensional systems.