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arXiv:1611.09106 · Journal of Physics Condensed Matter

Three-electron spin qubits

Maximilian Rimbach-Russ, Guido Burkard

Published May 31, 2017• 95 citations
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Abstract

The goal of this article is to review the progress of three-electron spin qubits from their inception to the state of the art. We direct the main focus towards the exchange-only qubit (Bacon et al 2000 Phys. Rev. Lett. 85 1758-61, DiVincenzo et al 2000 Nature 408 339) and its derived versions, e.g. the resonant exchange (RX) qubit, but we also discuss other qubit implementations using three electron spins. For each three-spin qubit we describe the qubit model, the envisioned physical realization, the implementations of single-qubit operations, as well as the read-out and initialization schemes. Two-qubit gates and decoherence properties are discussed for the RX qubit and the exchange-only qubit, thereby completing the list of requirements for quantum computation for a viable candidate qubit implementation. We start by describing the full system of three electrons in a triple quantum dot, then discuss the charge-stability diagram, restricting ourselves to the relevant subsystem, introduce the qubit states, and discuss important transitions to other charge states (Russ et al 2016 Phys. Rev. B 94 165411). Introducing the various qubit implementations, we begin with the exchange-only qubit (DiVincenzo et al 2000 Nature 408 339, Laird et al 2010 Phys. Rev. B 82 075403), followed by the RX qubit (Medford et al 2013 Phys. Rev. Lett. 111 050501, Taylor et al 2013 Phys. Rev. Lett. 111 050502), the spin-charge qubit (Kyriakidis and Burkard 2007 Phys. Rev. B 75 115324), and the hybrid qubit (Shi et al 2012 Phys. Rev. Lett. 108 140503, Koh et al 2012 Phys. Rev. Lett. 109 250503, Cao et al 2016 Phys. Rev. Lett. 116 086801, Thorgrimsson et al 2016 arXiv:1611.04945). The main focus will be on the exchange-only qubit and its modification, the RX qubit, whose single-qubit operations are realized by driving the qubit at its resonant frequency in the microwave range similar to electron spin resonance. Two different types of two-qubit operations are presented for the exchange-only qubits which can be divided into short-ranged and long-ranged interactions. Both of these interaction types are expected to be necessary in a large-scale quantum computer. The short-ranged interactions use the exchange coupling by placing qubits next to each other and applying exchange-pulses (DiVincenzo et al 2000 Nature 408 339, Fong and Wandzura 2011 Quantum Inf. Comput. 11 1003, Setiawan et al 2014 Phys. Rev. B 89 085314, Zeuch et al 2014 Phys. Rev. B 90 045306, Doherty and Wardrop 2013 Phys. Rev. Lett. 111 050503, Shim and Tahan 2016 Phys. Rev. B 93 121410), while the long-ranged interactions use the photons of a superconducting microwave cavity as a mediator in order to couple two qubits over long distances (Russ and Burkard 2015 Phys. Rev. B 92 205412, Srinivasa et al 2016 Phys. Rev. B 94 205421). The nature of the three-electron qubit states each having the same total spin and total spin in z-direction (same Zeeman energy) provides a natural protection against several sources of noise (DiVincenzo et al 2000 Nature 408 339, Taylor et al 2013 Phys. Rev. Lett. 111 050502, Kempe et al 2001 Phys. Rev. A 63 042307, Russ and Burkard 2015 Phys. Rev. B 91 235411). The price to pay for this advantage is an increase in gate complexity. We also take into account the decoherence of the qubit through the influence of magnetic noise (Ladd 2012 Phys. Rev. B 86 125408, Mehl and DiVincenzo 2013 Phys. Rev. B 87 195309, Hung et al 2014 Phys. Rev. B 90 045308), in particular dephasing due to the presence of nuclear spins, as well as dephasing due to charge noise (Medford et al 2013 Phys. Rev. Lett. 111 050501, Taylor et al 2013 Phys. Rev. Lett. 111 050502, Shim and Tahan 2016 Phys. Rev. B 93 121410, Russ and Burkard 2015 Phys. Rev. B 91 235411, Fei et al 2015 Phys. Rev. B 91 205434), fluctuations of the energy levels on each dot due to noisy gate voltages or the environment. Several techniques are discussed which partly decouple the qubit from magnetic noise (Setiawan et al 2014 Phys. Rev. B 89 085314, West and Fong 2012 New J. Phys. 14 083002, Rohling and Burkard 2016 Phys. Rev. B 93 205434) while for charge noise it is shown that it is favorable to operate the qubit on the so-called '(double) sweet spots' (Taylor et al 2013 Phys. Rev. Lett. 111 050502, Shim and Tahan 2016 Phys. Rev. B 93 121410, Russ and Burkard 2015 Phys. Rev. B 91 235411, Fei et al 2015 Phys. Rev. B 91 205434, Malinowski et al 2017 arXiv: 1704.01298), which are least susceptible to noise, thus providing a longer lifetime of the qubit.

DOI
10.1088/1361-648x/aa761f

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The goal of this article is to review the progress of three-electron spin qubits from their inception to the state of the art. We direct the main focus towards the exchange-only qubit (Bacon et al 2000 Phys. Rev. Lett. 85 1758-61, DiVincenzo et al 2000 Nature 408 339) and its derived versions, e.g. the resonant exchange (RX) qubit, but we also discuss other qubit implementations using three electron spins. For each three-spin qubit we describe the qubit model, the envisioned physical realization, the implementations of single-qubit operations, as well as the read-out and initialization schemes. Two-qubit gates and decoherence properties are discussed for the RX qubit and the exchange-only qubit, thereby completing the list of requirements for quantum computation for a viable candidate qubit implementation. We start by describing the full system of three electrons in a triple quantum dot, then discuss the charge-stability diagram, restricting ourselves to the relevant subsystem, introduce the qubit states, and discuss important transitions to other charge states (Russ et al 2016 Phys. Rev. B 94 165411). Introducing the various qubit implementations, we begin with the exchange-only qubit (DiVincenzo et al 2000 Nature 408 339, Laird et al 2010 Phys. Rev. B 82 075403), followed by the RX qubit (Medford et al 2013 Phys. Rev. Lett. 111 050501, Taylor et al 2013 Phys. Rev. Lett. 111 050502), the spin-charge qubit (Kyriakidis and Burkard 2007 Phys. Rev. B 75 115324), and the hybrid qubit (Shi et al 2012 Phys. Rev. Lett. 108 140503, Koh et al 2012 Phys. Rev. Lett. 109 250503, Cao et al 2016 Phys. Rev. Lett. 116 086801, Thorgrimsson et al 2016 arXiv:1611.04945). The main focus will be on the exchange-only qubit and its modification, the RX qubit, whose single-qubit operations are realized by driving the qubit at its resonant frequency in the microwave range similar to electron spin resonance. Two different types of two-qubit operations are presented for the exchange-only qubits which can be divided into short-ranged and long-ranged interactions. Both of these interaction types are expected to be necessary in a large-scale quantum computer. The short-ranged interactions use the exchange coupling by placing qubits next to each other and applying exchange-pulses (DiVincenzo et al 2000 Nature 408 339, Fong and Wandzura 2011 Quantum Inf. Comput. 11 1003, Setiawan et al 2014 Phys. Rev. B 89 085314, Zeuch et al 2014 Phys. Rev. B 90 045306, Doherty and Wardrop 2013 Phys. Rev. Lett. 111 050503, Shim and Tahan 2016 Phys. Rev. B 93 121410), while the long-ranged interactions use the photons of a superconducting microwave cavity as a mediator in order to couple two qubits over long distances (Russ and Burkard 2015 Phys. Rev. B 92 205412, Srinivasa et al 2016 Phys. Rev. B 94 205421). The nature of the three-electron qubit states each having the same total spin and total spin in z-direction (same Zeeman energy) provides a natural protection against several sources of noise (DiVincenzo et al 2000 Nature 408 339, Taylor et al 2013 Phys. Rev. Lett. 111 050502, Kempe et al 2001 Phys. Rev. A 63 042307, Russ and Burkard 2015 Phys. Rev. B 91 235411). The price to pay for this advantage is an increase in gate complexity. We also take into account the decoherence of the qubit through the influence of magnetic noise (Ladd 2012 Phys. Rev. B 86 125408, Mehl and DiVincenzo 2013 Phys. Rev. B 87 195309, Hung et al 2014 Phys. Rev. B 90 045308), in particular dephasing due to the presence of nuclear spins, as well as dephasing due to charge noise (Medford et al 2013 Phys. Rev. Lett. 111 050501, Taylor et al 2013 Phys. Rev. Lett. 111 050502, Shim and Tahan 2016 Phys. Rev. B 93 121410, Russ and Burkard 2015 Phys. Rev. B 91 235411, Fei et al 2015 Phys. Rev. B 91 205434), fluctuations of the energy levels on each dot due to noisy gate voltages or the environment. Several techniques are discussed which partly decouple the qubit from magnetic noise (Setiawan et al 2014 Phys. Rev. B 89 085314, West and Fong 2012 New J. Phys. 14 083002, Rohling and Burkard 2016 Phys. Rev. B 93 205434) while for charge noise it is shown that it is favorable to operate the qubit on the so-called '(double) sweet spots' (Taylor et al 2013 Phys. Rev. Lett. 111 050502, Shim and Tahan 2016 Phys. Rev. B 93 121410, Russ and Burkard 2015 Phys. Rev. B 91 235411, Fei et al 2015 Phys. Rev. B 91 205434, Malinowski et al 2017 arXiv: 1704.01298), which are least susceptible to noise, thus providing a longer lifetime of the qubit.
Quantum information processing in semiconductor quantum dots using single and multi-spin qubitsThe idea of a quantum computer, a device capable of processing information using quantum bits (qubit) instead of classical bits that outperforms classical computer in terms of computation speed, is still science ction. However, recent advances in quantum information processing showed that this ction may come true faster than anticipated. A promising platform for the physical realization of a qubit are spin qubits where the information is encoded in the quantum mechanical spin of an electron con ned in a semiconductor quantum dot. There are a variety of di erent implementations how the logical qubit is physically encoded, the use of a single electron spin or the use of the spins of multi electrons. This thesis focuses on the implementation of the spin- 1/2 qubit using the spin of a single electron in a single quantum dot, the exchangeonly (EO) qubit using three electron spins distributed in three quantum dots, and the novel quadrupolar exchange-only (QUEX) qubit using four electron spins distributed in three quantum dots. In this thesis we investigate several theoretical aspects of the physical implementation of the aforementioned qubit encodings. Since all three qubit encodings are allelectric controlled these implementations su er decoherence, the loss of information, from electric uctuations of the environment commonly called charge noise. Typically, the use of more quantum dots increases the decoherence due to charge noise while it decreases the decoherence due to magnetic noise. The rst main aspect investigated in this thesis is the protection of the quantum information encoded in the di erent qubit implementations against charge noise. Special attention is paid to the multi-electron spin implementations where high-symmetry points of operation are discovered which are less sensitive to the charge noise. Protection against charge noise is even better by increasing the number of electrons while keeping the number of quantum dots making the QUEX qubit superior to the EO qubit. So far the main direction in this thesis is the reduction of the qubit sensitivity to electric uctuations. However, coherent electromagnetic elds in form of microwaves v can be used to interconnect qubits. In this thesis also a high-performance coupling between two spin-1/2 is investigated. The use of a resonator, subsequently, allows for a coupling of qubits over macroscopic distances as well as to extract valuable information about the physical system. Because of the larger susceptibility of multi-spin qubits to the electric eld of the resonator, this thesis focuses on the coupling between an EO or a QUEX qubit and a microwave resonator. Points of operations are discovered for both qubit implementations which o er a strong coupling towards a microwave resonator while maintaining their protection against charge noise. Subsequently, a series of measurements are proposed to extract information about the microscopic structure of the quantum dots. Finally, a promising high-performance protocol for coupling two qubits remotely via the resonator is investigated in detail.
A two-level quantum system is the building block of a quantum computer. This pair of quantum states defines the computational unit of a quantum computer, and it is called a quantum bit or qubit in analogy to the bit that is the binary unit of a classical computer. The spin of a single electron naturally defines such a two-level quantum system. A quantum dot can be tuned to the single-electron regime, and an array of singly occupied quantum dots provides a multi-qubit register. This thesis describes the multielectron encoding of a spin qubit using a pair or a trio of quantum dots, and it analyzes the coherence properties and manipulation protocols of this system. The singlet-triplet qubit, coded using the singlet state and the spinless triplet state of a pair of singly occupied quantum dots, can be controlled all electrically when applying voltages to gates close to the quantum dot structure. Rapid, subnanosecond modifications of the double quantum dot's charge configuration have been realized successfully. A small magnetic field gradient across the double quantum dot enables universal qubit control. Two modifications of the normal singlet-triplet encoding are introduced. (1) The six-electron configuration of a double quantum dot encodes a singlet-triplet qubit in the same way as for the two-electron double quantum dot. Two electrons at each quantum dot are irrelevant for the qubit manipulations because they are paired in a singlet state; the remaining two electrons encode the qubit. The qubit's wave function is immune to charge noise at moderate out-of-plane magnetic fields. (2) A singlet-triplet qubit encoded using two quantum dots of different sizes has an orbital state degeneracy of the singlet state and the spinless triplet state at finite out-of-plane magnetic fields. Spin-orbit interactions lift this state degeneracy, while the magnitude of the state coupling is determined by the size difference of the QDs. This setup enables the manipulations of singlet-triplet qubits without the need for magnetic field gradients. Finally, two-qubit gates between singlet-triplet qubits are proposed that use mediated exchange interactions via one quantum state. These operations are well controlled and highly noise insensitive. Orbital interactions alone can control spin qubits coded in a three electron Hilbert space. For example, the exchange-only qubit is encoded using three singly occupied quantum dots. The exchange interactions of two quantum dot pairs need to be modified to manipulate this qubit. The noise sensitivity of the exchange-only qubit is discussed. Alternatively, a three-electron qubit at a double quantum dot can be operated when single electrons are transferred between the quantum dots. Fast, subnanosecond manipulations of the double quantum dot's charge configuration are required to realize single-qubit gates. A novel two-qubit pulse gate for the three-electron double quantum dot qubit is proposed.
We report on our recent progress in applying semiconductor quantum dots for spin-based quantum computation, as proposed by Loss and DiVincenzo (1998 Phys. Rev. A 57 120). For the purpose of single-electron spin resonance, we study different types of single quantum dot devices that are designed for the generation of a local ac magnetic field in the vicinity of the dot. We observe photon-assisted tunnelling as well as pumping due to the ac voltage induced by the ac current driven through a wire in the vicinity of the dot, but no evidence for ESR so far. Analogue concepts for a double quantum dot and the hydrogen molecule are discussed in detail. Our experimental results in laterally coupled vertical double quantum dot device show that the Heitler–London model forms a good approximation of the two-electron wavefunction. The exchange coupling constant J is estimated. The relevance of this system for two-qubit gates, in particular the SWAP operation, is discussed. Density functional calculations reveal the importance of the gate electrode geometry in lateral quantum dots for the tunability of J in realistic two-qubit gates.
Semiconductor-based spin qubits embedded into a superconducting microwave cavity constitute a fast-progressing and promising platform for realizing fast and fault-tolerant qubit control with long-range two-qubit coupling. The flopping-mode spin qubit consists of a single electron in a double quantum dot; it combines a charge qubit with a spin qubit. With its strong and tunable cavity coupling, the flopping-mode qubit is proven to be well suited for low-power qubit control and cavity-mediated long-range quantum gates. The singlet-triplet (ST) and exchange-only (EO) qubits are multielectron realizations that go without broadband control and are protected from some types of noise, but are challenging to couple to each other and to microwave cavities. We combine the flopping-mode concept with the ST and EO qubits and propose two new flopping-mode qubits that consist of three (four) quantum dots, occupied by two (three) electrons near the ( 1 , 0 , 1 ) ↔ ( 0 , 1 , 1 ) [ ( 1 , 0 , 1 , 1 ) ↔ ( 0 , 1 , 1 , 1 ) ] charge transition. The two-electron system augments the ST 0 spin qubit with a charge qubit that interacts transversally and longitudinally with a cavity. Both couplings are highly tunable, and the longitudinal coupling distinguishes the flopping-mode ST qubit from the regular flopping-mode qubit. The longitudinal coupling allows for nondissipative universal control similar to superconducting transmon qubits. The EO flopping-mode qubit comprises four dots occupied by three electrons and opens a new possibility to perform two-qubit gates for EO qubits that are challenging to perform directly with the exchange coupling. We use input-output theory to provide means of extracting the coupling strengths from cavity transmission data.
Initialization, two-spin coherent manipulation, and readout of a three-spin qubit are demonstrated using a few-electron triple quantum dot. The three-spin qubit is designed to allow all operations for full qubit control to be tuned via nearest-neighbor exchange interaction. Fast readout of charge states takes advantage of multiplexed reflectometry. Decoherence measured in a two-spin subspace is found to be consistent with predictions based on gate voltage noise with a uniform power spectrum. The theory of the exchange-only qubit is developed and it is shown that initialization of only two spins suffices for operation. Requirements for full multiqubit control using only exchange and electrostatic interactions are outlined.
We investigate the behavior of qubits consisting of three electron spins in double and triple quantum dots subject to external electric fields. Our model includes two independent bias parameters, $\ensuremath{\varepsilon}$ and ${\ensuremath{\varepsilon}}_{M}$, which both couple to external electromagnetic fields and can be controlled by gate voltages applied to the quantum dot structures. By varying these parameters, one can switch the qubit type by shifting the energies in the single quantum dots, thus changing the electron occupancy in each dot. Starting from the asymmetric resonant exchange qubit with a (2,0,1) and (1,0,2) charge admixture, one can smoothly cross over to the resonant exchange qubit with a detuned (1,1,1) charge configuration, and to the exchange-only qubit with the same charge configuration but equal energy levels down to the hybrid qubits with (1,2,0) and (0,2,1) charge configurations. Here, (l,m,n)(l,m,n)(l,m,n) describes a configuration with lll electrons in the left dot, mmm electrons in the center dot, and nnn electrons in the right dot. We first focus on random electromagnetic field fluctuations, i.e., ``charge noise,'' at each quantum dot resulting in dephasing of the qubit, and we provide a complete map of the resulting dephasing time as a function of the bias parameters. We pay special attention to the so-called sweet spots and double sweet spots of the system, which are least susceptible to noise. In the second part, we investigate the coupling of the qubit system to the coherent quantized electromagnetic field in a superconducting strip-line cavity, and we also provide a complete map of the coupling strength as a function of the bias parameters. We analyze the asymmetric qubit-cavity coupling via $\ensuremath{\varepsilon}$ and the symmetric coupling via ${\ensuremath{\varepsilon}}_{M}$.