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arXiv:1611.05230 · Molecular Physics

Towards laser control of open quantum systems: memory effects

Raiju Puthumpally-Joseph, Osman Atabek, Étienne Mangaud, Michèle Desouter-Lecomte, Dominique Sugny

Published Apr 27, 2017• 6 citations
arXivHTMLPDF

Abstract

Laser control of open quantum systems (OQS) is a challenging issue as compared to its counterpart in isolated small size molecules, basically due to very large numbers of degrees of freedom to be accounted for. Such a control aims at appropriately optimising decoherence processes of a central two-level system (a given vibrational mode, for instance) towards its environmental bath (including, for instance, all other normal modes). A variety of applications could potentially be envisioned, either to preserve the central system from decaying (long duration molecular alignment or orientation, qubit decoherence protection) or, to speed up the information flow towards the bath (efficient charge or proton transfers in long chain organic compounds). Achieving such controls requires some quantitative measures of decoherence in relation with memory effects in the bath response, actually given by the degree of non-Markovianity. Characteristic decoherence rates of a Spin-Boson model are calculated using a Nakajima–Zwanzig type master equation with converged hierarchical equations of motion expansion for the memory kernel. It is shown that, by adequately tuning the two-level transition frequency through a controlled Stark shift produced by an external laser field, non-Markovianity can be enhanced in a continuous way leading to a first attempt towards the control of OQS.

DOI
10.1080/00268976.2017.1319085

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Laser control of open quantum systems (OQS) is a challenging issue as compared to its counterpart in isolated small size molecules, basically due to very large numbers of degrees of freedom to be accounted for. Such a control aims at appropriately optimising decoherence processes of a central two-level system (a given vibrational mode, for instance) towards its environmental bath (including, for instance, all other normal modes). A variety of applications could potentially be envisioned, either to preserve the central system from decaying (long duration molecular alignment or orientation, qubit decoherence protection) or, to speed up the information flow towards the bath (efficient charge or proton transfers in long chain organic compounds). Achieving such controls requires some quantitative measures of decoherence in relation with memory effects in the bath response, actually given by the degree of non-Markovianity. Characteristic decoherence rates of a Spin-Boson model are calculated using a Nakajima–Zwanzig type master equation with converged hierarchical equations of motion expansion for the memory kernel. It is shown that, by adequately tuning the two-level transition frequency through a controlled Stark shift produced by an external laser field, non-Markovianity can be enhanced in a continuous way leading to a first attempt towards the control of OQS.
Referring to a Fano-type model qualitative analogy we develop a comprehensive basic mechanism for the laser control of the non-Markovian bath response and fully implement it in a realistic control scheme, in strongly coupled open quantum systems. Converged hierarchical equations of motion are worked out to numerically solve the master equation of a spin-boson Hamiltonian to reach the reduced electronic density matrix of a heterojunction in the presence of strong terahertz laser pulses. Robust and efficient control is achieved increasing by a factor of 2 the non-Markovianity measured by the time evolution of the volume of accessible states. The consequences of such fields on the central system populations and coherence are examined, putting the emphasis on the relation between the increase of non-Markovianity and the slowing down of decoherence processes.
The study of entanglement has gained prominence in recent years due to the advent of fields such as Quantum Optics and Quantum Information Theory — advances that have harnessed such counter-intuitive quantum phenomena into elements of everyday life, improving it in the process. Ideal quantum systems, “closed” to the outside world, remain quantum forever and thus manage to retain entanglement. Real quantum systems, however, are “open” to the environment and are therefore susceptible to the phenomenon of decoherence. The resultant loss of entanglement is a major hindrance to the effectiveness of quantum information tasks. In this thesis we have studied the evolution of entanglement in various types of open quantum systems (OQS) coupled in various ways to local baths. We have also studied existing ways and means of controlling the decay of entanglement and have proposed a new method of doing so. We have studied the evolution of entanglement in OQS undergoing Markovian dynamics by using the Lindblad master equation as well as the method of quantum trajectories. We have analyzed the onset of the phenomenon of entanglement sudden death in finite as well as infinite dimensional OQS, connected either locally to a thermal bath or its squeezed variant, or via a quantum non-demolition-type (QND-type) interaction to a local thermal bath. We have found that the QND-type system-bath interaction works best to conserve entanglement in finite dimensional systems, whereas a squeezed thermal bath causes entanglement sudden death even at zero temperature. We have also studied some well-known methods of controlling decoherence in open systems with respect to their ability of preserving entanglement. Some of these procedures include coupling the system to a thermal bath of photonic crystals where the photonic band gap suppresses decoherence, modulation of the systembath frequency in an attempt to contain decoherence, using the method of resonance fluorescence where an external field modulates the transition frequency of the two-qubit systems with each qubit being a two-state atomic system to contain decoherence, and using high-frequency radio waves to decouple the system and bath dynamically and thus reducing decoherence. Our study has revealed a rather startling fact — some of these decoherence control procedures actually result in an elevated rate of loss and a resultant quicker death of entanglement. This is a 6 surprising and extremely counter-intuitive result. Finally, we have proposed a new method of shielding the entanglement in the system from dissipative environmental effects. In this procedure, an ancillary system in a fixed initial state is allowed to interact with the main system through exchange interactions. We have, through numerical computation, showed that an ancilla in the ground state extends the lifespan of entanglement in the main system. Increasing the size of the ancilla, that is, increasing the value of n in an n-qubit ancilla slows down entanglement loss for a two-qubit system connected locally to a thermal bath.
The dynamics of an open quantum system is non-Markovian when memory effect is non-negligible. The quantum memory effect is a very complex issue and presently there is no universally accepted method to quantify it. By examining the memory kernel of the Nakajima-Zwanzig master equation, we study the memory effect in a theoretical model consisting of a spin coupled to an environment of an Ising spin chain subject to a transverse field. We find that it can be dictated by either the time correlation in the environment, or the system-environment correlation, depending on the strength of the transverse field and the state of the environment. We analyze the information loss to the environment and backflow from it, and discover that the information flow is not always a reliable indicator for the nature of the dynamics.
This thesis investigates two thematic lines of research, both underpinned by non-Markovian system-reservoir interactions in quantum optics. The overarching focus is on modelling the open system dynamics in a non-perturbative fashion, broadly on - though not restricted to - instances when the environment is structured. A theory is developed by means of enlarging the open system over environmental degrees of freedom to include memory effects in its dynamics. This is achieved using an established technique that involves mapping a bosonic environment onto a 1D chain of harmonic oscillators. Within this setting, we apply a Heisenberg equation-of-motion approach to derive an exact set coupled differential equations for the open system and a single auxiliary oscillator of the chain. The combined equations are shown to have their interpretation rooted in a quantum Markov stochastic process. Including the auxiliary chain oscillator as part of the original system then enables us to obtain an exact master equation for the enlarged system, avoiding any need for the Born-Markov approximations. Our method is valid for a dissipative two-state system, with cases of multiple excitations and added driving discussed. Separately, we apply the framework of quantum Darwinism to an atom-cavity system, and, subsequently, to a more general multiple-environment model. In both cases, the time-dependent spread of correlations between the open system and fractions of the environment is analysed during the course of the decoherence process. The degree to which information is redundant across different fractions is checked to infer the emergence of classicality. In the second case, we go further and present a decomposition of information in terms of its quantum and classical correlations. A quantitative measure of redundancy is also studied with regard to its ability to witness non-Markovian behaviour. Besides fundamental interest, our results have application to quantum information processing and quantum technologies, keeping in mind the potential beneficial use of non-Markovian effects in reservoir engineering.
The non-Markovian master equation for open quantum systems is obtained by generalization of the standard Zwanzig-Nakajima (ZN) projection technique. To this end, a coupled chain of equations is written for the reduced density matrices of the bath ϱB(t) and of the system ϱS(t). A formal solution of the equation for ϱB(t) in the 2nd approximation in interaction yields a specific extra term related to the intrinsic bath dynamics. This term is nonlinear in the reduced density matrix ϱS(t), and vanishes in the Markovian limit. To verify the consistence and robustness of our approach, we apply the generalized ZN projection scheme to a simple dephasing model. We study the obtained kinetic equation both in the Markovian approximation and beyond it (for the term related to the intrinsic bath dynamics) and compare the results with the exact ones.
An efficient optimal-control theory based on the Krotov method is introduced for a non-Markovian open quantum system with a time-nonlocal master equation in which the control parameter and the bath correlation function are correlated. This optimal-control method is developed via a quantum dissipation formulation that transforms the time-nonlocal master equation to a set of coupled linear time-local equations of motion in an extended auxiliary Liouville space. As an illustration, the optimal-control method is applied to find the control sequences for high-fidelity ZZZ gates and identity gates of a qubit embedded in a non-Markovian bath. ZZZ gates and identity gates with errors less than ${10}^{\ensuremath{-}5}$ for a wide range of bath decoherence parameters can be achieved for the non-Markovian open qubit system with control over only the ${\ensuremath{\sigma}}_{z}$ term. The control-dissipation correlation and the memory effect of the bath are crucial in achieving the high-fidelity gates.