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arXiv:1611.03198 · Physical Review A

Observation of resonant scattering between ultracold heteronuclear Feshbach molecules

Fudong Wang, Xin Ye, Mingyang Guo, D. Blume, Dajun Wang

Published Oct 14, 2019• 16 citations
arXivHTMLPDF

Abstract

We report the observation of a dimer-dimer inelastic collision resonance for ultracold Feshbach molecules made of bosonic sodium and rubidium atoms. This resonance, which we attribute to the crossing of the dimer-dimer threshold with a heteronuclear tetramer state, manifests itself as a pronounced inelastic loss peak of dimers when the interspecies scattering length between the constituent atoms is tuned. Near this resonance, a strong modification of the temperature dependence of the dimer-dimer scattering is observed. Our result provides insight into the heteronuclear four-body system consisting of heavy and light bosons and offers the possibility of investigating ultracold molecules with tunable interactions.

DOI
10.1103/physreva.100.042706

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We report the observation of a dimer-dimer inelastic collision resonance for ultracold Feshbach molecules made of bosonic sodium and rubidium atoms. This resonance, which we attribute to the crossing of the dimer-dimer threshold with a heteronuclear tetramer state, manifests itself as a pronounced inelastic loss peak of dimers when the interspecies scattering length between the constituent atoms is tuned. Near this resonance, a strong modification of the temperature dependence of the dimer-dimer scattering is observed. Our result provides insight into the heteronuclear four-body system consisting of heavy and light bosons and offers the possibility of investigating ultracold molecules with tunable interactions.
We study inelastic collisions in a pure, trapped sample of Feshbach molecules made of bosonic cesium atoms in the quantum halo regime. We measure the relaxation rate coefficient for decay to lower-lying molecular states and study the dependence on scattering length and temperature. We identify a pronounced loss minimum with varying scattering length along with a further suppression of loss with decreasing temperature. Our observations provide insight into the physics of a few-body quantum system that consists of four identical bosons at large values of the two-body scattering length.
We consider weakly bound bosonic and fermionic heteronuclear molecules (dimers) in ultracold atomic gases, where the interspecies interaction is characterized by a large positive scattering length. We develop a new theoretical approach to solve the four-body scattering problem, which is valid when the mass ratio between the constituent atoms is sufficiently large. This approach is then used to study elastic and inelastic dimer- dimer scattering processes in the case that the light constituent atoms are fermions, while the heavy atoms can be either fermions or bosons. Due to the Fermi statistics of the light atoms, the heavy atoms experience a strong repulsion at large intermolecular distances. This leads to suppression of the collisional relaxation to universal trimer (Efimov) states and/or deeply bound molecular states. We present the formation rate of Efimov trimers as a function of the three-body parameter for several experimentally interesting systems. The competition between the formation of trimers and relaxation to deeply bound molecules is analyzed, and prospects for future studies of these systems are discussed.
We study collisions in an optically trapped, pure sample of ultracold Cs 2 molecules in various internal states. The molecular gas is created by Feshbach association from a near-degenerate atomic gas, with adjustable temperatures in the nanokelvin range. We identify several narrow loss resonances, which point to the coupling to more complex molecular states and may be interpreted as Feshbach resonances in dimerdimer interactions. Moreover, in some molecular states we observe a surprising temperature dependence in collisional loss. This shows that the situation cannot be understood in terms of the usual simple threshold behavior for inelastic two-body collisions. We interpret this observation as further evidence for a more complex molecular structure beyond the well-understood dimer physics.
We consider collisional properties of weakly bound heteronuclear molecules (dimers) formed in a two-species mixture of atoms with a large mass difference. We focus on dimers containing light fermionic atoms as they manifest collisional stability due to an effective dimer-dimer repulsion originating from the exchange of the light atoms. In order to solve the dimer-dimer scattering problem we develop a theoretical approach, which provides a physically transparent and quantitative description of this four-atom system in terms of three- and two-body observables. We calculate the elastic scattering amplitude and the rates of inelastic processes such as the trimer formation and the relaxation of dimers into deeply bound molecular states. Irrespective of whether the heavy atoms are bosons or fermions, the inelastic rate can be significantly lower than the rate of elastic collisions. Moreover, the measurement of the inelastic rate which is a four-body observable, can be an efficient and precise tool for determining three-body observables such as the three-body parameter, positions of Efimov states, and their lifetimes.
Atom loss resonances in ultracold trapped atoms have been observed at scattering lengths near atom-dimer resonances, at which Efimov trimers cross the atom-dimer threshold, and near two-dimer resonances, at which universal tetramers cross the dimer-dimer threshold. We propose a new mechanism for these loss resonances in a Bose-Einstein condensate of atoms. As the scattering length is ramped to the large final value at which the atom loss rate is measured, the time-dependent scattering length generates a small condensate of shallow dimers coherently from the atom condensate. The coexisting atom and dimer condensates can be described by a low-energy effective field theory with universal coefficients that are determined by matching exact results from few-body physics. The classical field equations for the atom and dimer condensates predict narrow enhancements in the atom loss rate near atom-dimer resonances and near two-dimer resonances due to inelastic dimer collisions.
In the absence of inelastic scattering, Feshbach resonances produce poles in scattering lengths and very large peaks in elastic cross-sections. However, inelastic scattering removes the poles. Whenever the resonant state is coupled comparably to the elastic and inelastic channels, the scattering length exhibits only a small oscillation and peaks in cross-sections are significantly suppressed. A resonant scattering length is defined to characterize the amplitude of the oscillation, and is shown to be small for many collisions of ultracold molecules. The results suggest that cross-sections for some ultracold collision processes will be much less sensitive to details of the potential than has been expected.