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arXiv:0711.4632 · Physical Review A

Collisional properties of weakly bound heteronuclear dimers

Bout Marcelis, S. J. J. M. F. Kokkelmans, Georgy V. Shlyapnikov, Dmitry S. Petrov

Published Mar 13, 2008• 47 citations
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Abstract

We consider collisional properties of weakly bound heteronuclear molecules (dimers) formed in a two-species mixture of atoms with a large mass difference. We focus on dimers containing light fermionic atoms as they manifest collisional stability due to an effective dimer-dimer repulsion originating from the exchange of the light atoms. In order to solve the dimer-dimer scattering problem we develop a theoretical approach, which provides a physically transparent and quantitative description of this four-atom system in terms of three- and two-body observables. We calculate the elastic scattering amplitude and the rates of inelastic processes such as the trimer formation and the relaxation of dimers into deeply bound molecular states. Irrespective of whether the heavy atoms are bosons or fermions, the inelastic rate can be significantly lower than the rate of elastic collisions. Moreover, the measurement of the inelastic rate which is a four-body observable, can be an efficient and precise tool for determining three-body observables such as the three-body parameter, positions of Efimov states, and their lifetimes.

DOI
10.1103/physreva.77.032707

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We consider weakly bound bosonic and fermionic heteronuclear molecules (dimers) in ultracold atomic gases, where the interspecies interaction is characterized by a large positive scattering length. We develop a new theoretical approach to solve the four-body scattering problem, which is valid when the mass ratio between the constituent atoms is sufficiently large. This approach is then used to study elastic and inelastic dimer- dimer scattering processes in the case that the light constituent atoms are fermions, while the heavy atoms can be either fermions or bosons. Due to the Fermi statistics of the light atoms, the heavy atoms experience a strong repulsion at large intermolecular distances. This leads to suppression of the collisional relaxation to universal trimer (Efimov) states and/or deeply bound molecular states. We present the formation rate of Efimov trimers as a function of the three-body parameter for several experimentally interesting systems. The competition between the formation of trimers and relaxation to deeply bound molecules is analyzed, and prospects for future studies of these systems are discussed.
We consider weakly bound diatomic molecules (dimers) formed in a two-component atomic Fermi gas with a large positive scattering length for the interspecies interaction. We develop a theoretical approach for calculating atom-dimer and dimer-dimer elastic scattering and for analyzing the inelastic collisional relaxation of the molecules into deep bound states. This approach is based on the single-channel zero-range approximation, and we find that it is applicable in the vicinity of a wide two-body Feshbach resonance. Our results draw prospects for various interesting manipulations of weakly bound dimers of fermionic atoms.
We calculate the universal spectrum of trimer and tetramer states in heteronuclear mixtures of ultracold atoms with different masses in the vicinity of the heavy-light dimer threshold. To extract the energies, we solve the three- and four-body problem for simple two- and three-body potentials tuned to the universal region using the Gaussian expansion method. We focus on the case of one light particle of mass mmm and two or three heavy bosons of mass MMM with resonant heavy-light interactions. We find that trimer and tetramer cross into the heavy-light dimer threshold at almost the same point and that as the mass ratio M/mM/mM/m decreases, the distance between the thresholds for trimer and tetramer states becomes smaller. We also comment on the possibility of observing exotic three-body states consisting of a dimer and two atoms in this region and compare with previous work.
Few-body effects play an important role for the understanding of ultracold quantum gases. We make use of an effective field theory approach to investigate various aspects of universal few-body physics close to a Feshbach resonance. That is the regime where the scattering length is large compared to all other length scales of the system and thus determines the observables. It is also the regime where the Efimov effect whose main characteristic is the occurrence of a sequence of three-body bound states becomes important. At unitarity, i.e., for diverging scattering length, the ratio of binding energies of neighboring states approaches a constant. The existence of those trimers can be captured by a single three-body parameter and influences observables such as recombination rates. Starting from adequate Lagrangians, we derive atom-dimer scattering amplitudes that contain all information of interest about the three-particle systems. With this method, we first investigate the scattering of atoms and dimers at finite temperature in the presence of the Efimov effect. We calculate the dimer relaxation rate and obtain good agreement with available experimental data. Furthermore, heteronuclear mixtures exhibiting large interspecies scattering length are studied in detail. If bosons are the majority species, the Efimov effect occurs in an S-wave channel and we are able to compute three-body recombination and dimer relaxation rates. The results are compared to the outcome of two existing experiments. For mainly fermionic systems, the Efimov effect is only present in an overall P-wave and three-body recombination at threshold vanishes. However, in mixtures of atoms and dimers, scattering cross sections and dimer relaxation show the typical Efimov behavior of log-periodicity. We also consider two-dimensional Bose gases, where the Efimov effect does not occur. For those systems, we derive an equation including the first non-universal corrections and deduce three-body observables such as binding energies and atom-dimer scattering parameters.
We consider a heteronuclear fermionic mixture on the molecular side of an interspecies Feshbach resonance and discuss atom-dimer scattering properties in uniform space and in the presence of an external confining potential, restricting the system to a quasi-two-dimensional geometry. We find that there is a peculiar atom-dimer p-wave resonance which can be tuned by changing the frequency of the confinement. Our results have implications for the ongoing experiments on lithium-potassium mixtures, where this mechanism allows for switching the p-wave interaction between a K atom and Li-K dimer from attractive to repulsive, and forming a weakly bound trimer with unit angular momentum. We show that such trimers are long lived and the atom-dimer resonance does not enhance inelastic relaxation in the mixture, making it an outstanding candidate for studies of p-wave resonance effects in a many-body system.
Four-body system of 4He{}^4\mathrm{He}4He atoms: Dimer-dimer scattering
The strong short-range repulsion, characteristic to realistic interatomic potentials, complicates the description of weakly-bound few-body systems such as those of \He atoms. The present work proposes an approach for solving this problem and applies it to a realistic system of four 4He{}^4\mathrm{He}4He atoms. The potential is gradually softened such that rigorous four-body equations for bound and scattering tates can be accurately solved in the momentum-space framework, and the results are extrapolated back to the limit of the original potential. Linear correlations between three- and four body quantities are observed, and the accuracy of the procedure is improved by extrapolating in one of the three-body quantities. Results for the 4He{}^4\mathrm{He}4He tetramer ground and excited state binding energies and atom-trimer scattering agree well with at least some of earlier determinations and shed light on the existing disagreements. An additional case of the Phillips correlation line is established for the dimer-dimer scattering length. The trimer production rate via the ultracold two-dimer collisions is estimated, it exhibits significant finite-range effects despite the weak binding of the dimer.