We study the non-equilibrium dynamics of a spinful single-orbital quantum dot with an incorporated quantum mechanical spin-1/2 magnetic impurity. Due to the spin degeneracy, double occupancy is allowed, and Coulomb interaction together with the exchange coupling of the magnetic impurity influence the dynamics. By extending the iterative summation of real-time path integrals (ISPI) to this coupled system, we monitor the time-dependent non-equilibrium current and the impurity spin polarization to determine features of the time-dependent non-equilibrium dynamics. We particulary focus on the deep quantum regime, where all time and energy scales are of the same order of magnitude and no small parameter is available. We observe a significant influence of the non-equilibrium decay of the impurity spin polarization both in the presence and in the absence of Coulomb interaction. The exponential relaxation is faster for larger bias voltages, electron–impurity interactions and temperatures. We show that the exact relaxation rate deviates from the corresponding perturbative result. In addition, we study in detail the impurity's back action on the charge current and find a reduction of the stationary current for increasing coupling to the impurity. Moreover, our approach allows us to systematically distinguish mean-field Coulomb and impurity effects from the influence of quantum fluctuations and flip-flop scattering, respectively. In fact, we find a local maximum of the current for a finite Coulomb interaction due to the presence of the impurity.
We develop a generic method in Liouville space to describe the dissipative dynamics of coherent interacting quantum dots with adiabatic time dependence beyond linear response. We show how the adiabatic response can be related to effective quantities known from real-time renormalization group methods for stationary quantities. We propose the study of a delay time as a characteristic time scale. We apply the method to the interacting resonant level model and calculate the nonlinear adiabatic charge response to time-dependent gate voltages, tunneling barriers and Coulomb interaction. The dot charge delay time is found to be given by a unique expression in all cases, in contrast to the capacitance and the charge relaxation resistance. We discuss the observability of the effects in molecular systems and cold-atom setups.
We investigate the quench dynamics of a quantum dot strongly coupled to spin-polarized ferromagnetic leads. The real-time evolution is calculated by means of the time-dependent density-matrix numerical renormalization group method implemented within the matrix product states framework. We examine the system's response to a quench in the spin-dependent coupling strength to ferromagnetic leads as well as in the position of the dot's orbital level. The spin dynamics is analyzed by calculating the time-dependent expectation values of the quantum dot's magnetization and occupation. Based on these, we determine the time dependence of a ferromagnetic-contact-induced exchange field and predict its nonmonotonic buildup. In particular, two timescales are identified, describing the development of the exchange field and the dot's magnetization sign change. Finally, we study the effects of finite temperature on the dynamical behavior of the system.
We develop a general approach to the nonequilibrium dynamics of quantum-impurity systems for arbitrary coupling strength. The numerical renormalization group is used to generate a complete basis set necessary for the correct description of the time evolution. We benchmark our method with the exact analytical solution for the resonant-level model. As a first application, we investigate the equilibration of an ultrasmall quantum dot subject to a sudden change of gate voltage and external magnetic field. Two distinct relaxation times are identified for the spin and charge dynamics.
We have developed a numerically exact approach to compute real‐time path integral expressions for quantum transport problems out of equilibrium. The scheme is based on a deterministic iterative summation of the path integral (ISPI) for the generating function of nonequilibrium observables of interest. We apply the scheme to compute the charge current or dynamical quantities of small strongly correlated quantum systems as a quantum dot or molecules that are tunnel coupled to leads. Self‐energies due to the leads, being nonlocal in time, are fully taken into account within a finite memory time, thereby including non‐Markovian effects. Numerical results are extrapolated first to vanishing (Trotter) time discretization and, second, to infinite memory time. The method is applied to nonequilibrium transport through a single‐impurity Anderson dot in the first place. We benchmark our results in various regimes of the rich parameter space. In the respective regime of validity, iterative summation of real‐time path integrals (ISPI) results are shown to match those of other state‐of‐the art methods. Especially, we have chosen the mixed valence regime of the Anderson model to compare ISPI to time dependent density matrix renormalization group (tDMRG) and functional RG calculations. Secondly, we determine the nonequilibrium current through a molecular junction in presence of a vibrational mode. We have found an exact mapping of the single impurity Anderson–Holstein model to an effective spin‐1 problem. In analytically tractable regimes, as the adiabatic phonon or weak molecule‐lead coupling regime, we reproduce known perturbative results. Studying the crossover regime between those limits shows that the Franck–Condon blockade persists in the quantum limit. At low temperature, the Franck–Condon steps in the characteristics are smeared due to nonequilibrium conditions. The third system under investigation here is the magnetic Anderson model which consists of a spinful single‐orbital quantum dot with an incorporated quantum mechanical spin–1/2 magnetic impurity. Coulomb interaction together with the exchange coupling of the magnetic impurity with the electron spins strongly influence the dynamics. We investigate the nonequilibrium tunneling current through the system as a function of exchange and Coulomb interaction as well as the real‐time impurity polarization. From the real‐time evolution of physical observables, we are able to determine characteristics of the time‐dependent nonequilibrium current and the relaxation dynamics of the impurity. These examples illustrate that the ISPI technique is particularly well suited for the quantum regime, when all time and energy scales are of the same order of magnitude.
We study charge and spin transport through an interacting quantum wire, caused by backscattering of electrons off an effective impurity potential with a periodic time dependence. The adiabatic regime of this pump for charge and spin is shown to depend on the presence of interactions in the wire. For the noninteracting case, the transported quantities in a period are calculated and found to be adiabatic (independent of the pumping frequency) for all frequencies $\ensuremath{\Omega}\ensuremath{\ll}{v}_{F}/\mathcal{l},$ where
l is the range of the scattering potential and
vF is the Fermi velocity; this result is along the lines of adiabatic pumping in mesoscopic systems. On the other hand, we show that for a wire with repulsive electron-electron interactions, the adiabatic regime is confined to $\ensuremath{\Elzxh}\ensuremath{\Omega}\ensuremath{\ll}{\ensuremath{\omega}}_{\ensuremath{\Gamma}},$ where ${\ensuremath{\omega}}_{\ensuremath{\Gamma}}$ is an energy scale set by the backscattering potential. Using symmetry and scaling properties of the quantum wire Hamiltonian, we relate the charge Q and spin S transported through the wire in a period $2\ensuremath{\pi}/\ensuremath{\Omega}$ to an integral involving quasistatic backscattering conductances. We also show that the pumped charge Q (or the spin
S) is quantized in the adiabatic limit if the conductance of the system is zero at the stable fixed point of the renormalization-group (RG) transformations. The quanta transported are given by the winding number of a complex coupling $\ensuremath{\Gamma}(\ensuremath{\Omega}t)$ as it traverses a closed path
C enclosing the origin $\ensuremath{\Gamma}=0.$ No adiabatic charge or spin is transported when the RG fixed point corresponds to a perfectly conducting wire, or if the path
C does not enclose the point $\ensuremath{\Gamma}=0.$ By contrast, for a RG marginal conductance---which is the case for noninteracting electrons---the charge transported in a cycle is not quantized, rather it is proportional to the area enclosed by the path or circuit
C, in agreement with previous studies of noninteracting mesoscopic systems. Finite size, temperature, and frequency effects on the transported quantities follow from the relation between adiabatic transport coefficients (backscattering conductances) and the quasistatic conductance of the system.