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arXiv:1109.6148 · Europhysics Letters (EPL)

Nonlinear adiabatic response of interacting quantum dots

Oleksiy Kashuba, Herbert Schoeller, Janine Splettstoesser

Published Jun 1, 2012• 26 citations
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Abstract

We develop a generic method in Liouville space to describe the dissipative dynamics of coherent interacting quantum dots with adiabatic time dependence beyond linear response. We show how the adiabatic response can be related to effective quantities known from real-time renormalization group methods for stationary quantities. We propose the study of a delay time as a characteristic time scale. We apply the method to the interacting resonant level model and calculate the nonlinear adiabatic charge response to time-dependent gate voltages, tunneling barriers and Coulomb interaction. The dot charge delay time is found to be given by a unique expression in all cases, in contrast to the capacitance and the charge relaxation resistance. We discuss the observability of the effects in molecular systems and cold-atom setups.

DOI
10.1209/0295-5075/98/57003

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Using a real-time renormalization group method we study the minimal model of a quantum dot dominated by charge fluctuations, the two-lead interacting resonant level model, at finite bias voltage. We develop a set of RG equations to treat the case of weak and strong charge fluctuations, together with the determination of power-law exponents up to second order in the Coulomb interaction. We derive analytic expressions for the charge susceptibility, the steady-state current, and the conductance in the situation of arbitrary system parameters, in particular away from the particle-hole symmetric point and for asymmetric Coulomb interactions. In the asymmetric situation we find that power laws can be observed for the current only as a function of the level position (gate voltage) but in general not as a function of the voltage except for extremely large voltages. Furthermore, we study the quench dynamics after sudden switch-on of the level-lead couplings. The time evolution of the dot occupation and current is governed by exponential relaxation accompanied by voltage-dependent oscillations and characteristic algebraic decay.
We formulate a general theory to study the time-dependent charge and energy transport of an adiabatically driven interacting quantum dot in contact with a reservoir for arbitrary amplitudes of the driving potential. We study within this framework the Anderson impurity model with a local ac gate voltage. We show that the exact adiabatic quantum dynamics of this system is fully determined by the behavior of the charge susceptibility of the frozen problem. At T=0T=0T=0, we evaluate the dynamic response functions with the numerical renormalization group (NRG). The time-resolved heat production exhibits a pronounced feature described by an instantaneous Joule law characterized by a universal B\"uttiker resistance quantum R0=h/(2e2){R}_{0}=h/(2{e}^{2})R0​=h/(2e2) for each spin channel. We show that this law holds in the noninteracting as well as in the interacting system and also when the system is spin polarized. In addition, in the presence of a static magnetic field, the interplay between many-body interactions and spin polarization leads to a nontrivial energy exchange between electrons with different spin components.
We introduce a real time version of the functional renormalization group, which allows us to study correlation effects on nonequilibrium transport through quantum dots. Our method is equally capable to address (i) the relaxation out of a nonequilibrium initial state into a (potentially) steady state driven by a bias voltage and (ii) the dynamics governed by an explicitly time-dependent Hamiltonian. All time regimes from transient to asymptotic can be tackled; the only approximation is the consistent truncation of the flow equations at a given order. As an application we investigate the relaxation dynamics of the interacting resonant level model, which describes a fermionic quantum dot dominated by charge fluctuations. Moreover, we study incoherence and relaxation phenomena within the ohmic spin-boson model by mapping the latter to the interacting resonant level model.
We develop a general approach to the nonequilibrium dynamics of quantum-impurity systems for arbitrary coupling strength. The numerical renormalization group is used to generate a complete basis set necessary for the correct description of the time evolution. We benchmark our method with the exact analytical solution for the resonant-level model. As a first application, we investigate the equilibration of an ultrasmall quantum dot subject to a sudden change of gate voltage and external magnetic field. Two distinct relaxation times are identified for the spin and charge dynamics.
We study the relaxation dynamics of a quantum dot with local Coulomb correlations coupled to two noninteracting leads which are held in grand-canonical equilibrium. Only charge degrees of freedom are considered and the dot is described by a model which in the scaling limit becomes equivalent to the interacting resonant level model. We examine the time evolution of the current and the dot occupancy resulting from changes in the dot-lead coupling, the dots' on-site energy, or the charging energy. Abrupt and smooth parameter changes as well as setups with and without driving bias voltage are considered. For biased dots, we investigate the often studied response after turning on the dot-lead coupling but also the experimentally more relevant case in which the voltage is turned on. We identify and explain a variety of interesting many-body effects, and we clarify the role of initial correlations.