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arXiv:1609.07336 · Scientific Reports

Entanglement and nonclassicality in four-mode Gaussian states generated via parametric down-conversion and frequency up-conversion

Ievgen I. Arkhipov, Jan Peřina, Ondřej Haderka, Alessia Allevi, Maria Bondani

Published Sep 23, 2016• 5 citations
arXivHTMLPDF

Abstract

Multipartite entanglement and nonclassicality of four-mode Gaussian states generated in two simultaneous nonlinear processes involving parametric down-conversion and frequency up-conversion are analyzed assuming the vacuum as the initial state. Suitable conditions for the generation of highly entangled states are found. Transfer of the entanglement from the down-converted modes into the up-converted ones is also suggested. The analysis of the whole set of states reveals that sub-shot-noise intensity correlations between the equally-populated down-converted modes, as well as the equally-populated up-converted modes, uniquely identify entangled states. They represent a powerful entanglement identifier also in other cases with arbitrarily populated modes.

DOI
10.1038/srep33802

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Multipartite entanglement and nonclassicality of four-mode Gaussian states generated in two simultaneous nonlinear processes involving parametric down-conversion and frequency up-conversion are analyzed assuming the vacuum as the initial state. Suitable conditions for the generation of highly entangled states are found. Transfer of the entanglement from the down-converted modes into the up-converted ones is also suggested. The analysis of the whole set of states reveals that sub-shot-noise intensity correlations between the equally-populated down-converted modes, as well as the equally-populated up-converted modes, uniquely identify entangled states. They represent a powerful entanglement identifier also in other cases with arbitrarily populated modes.
We use a versatile model to evaluate the multipartite entanglement and the nonclassical light generation in optical parametric oscillators, exploring the differences between doubly and triply resonant cavity configurations. We demonstrate the entanglement of the pump mode with converted fields in both situations, and the fundamental differences of oscillators using parametric down conversion and four wave mixing processes as the intracavity amplification technique. The strong correlations involving the sidebands of the pump and converted fields give the signatures of a rich dynamic of multipartite entanglement.
In a recent paper [I. I. Arkhipov, Phys. Rev. A 98, 021803 (2018)], it was shown that one can completely identify the nonclassicality of single- and two-mode Gaussian states by means of certain nonclassicality witnesses which are based on intensity moments up to the third order of optical fields, provided that an appropriate coherent displacement is applied to a given Gaussian state. Here, we utilize a mathematical equivalence between the description of the coherent displaced Gaussian states generated in the spontaneous parametric processes and the Gaussian states generated in the corresponding stimulated parametric processes. Resorting to that equivalence, we study and compare the power of those nonclassicality witnesses in the detection of the nonclassicality of the two-mode Gaussian states generated in both the spontaneous and stimulated second subharmonic and down-conversion processes and which are subsequently subject to a beam splitter. We demonstrate that by means of an appropriate induced stimulated emission, one can completely identify the nonclassicality of the considered Gaussian states in comparison to the case of the spontaneous emission. This is important from the experimental point of view, as the stimulated emission can be easily implemented in running optical experiments, and such method can exploit just simple linear detectors.
The behavior of general nonclassical two-mode Gaussian states at a beam splitter is investigated. Single-mode nonclassicality as well as two-mode entanglement of both input and output states are analyzed suggesting their suitable quantifiers. These quantifiers are derived from local and global invariants of linear unitary two-mode transformations such that the sum of input (or output) local nonclassicality measures and entanglement measure gives a global invariant. This invariant quantifies the global nonclassicality resource. Mutual transformations of local nonclassicalities and entanglement induced by the beam splitter are analyzed considering incident noisy twin beams, single-mode noisy squeezed vacuum states, and states encompassing both squeezed states and twin beams. A rich tapestry of interesting nonclassical output states is predicted.
We investigate the performance of a certain nonclassicality identifier, expressed via integrated second-order intensity moments of optical fields, in revealing bipartite entanglement of quantum-optical frequency combs (QOFCs), which are generated in both spontaneous and stimulated parametric down-conversion processes. We show that, by utilizing that nonclassicality identifier, one can well identify the entanglement of the QOFC directly from the experimentally measured intensity moments without invoking any state reconstruction techniques or homodyne detection. Moreover, we demonstrate that the stimulated generation of the QOFC improves the entanglement detection of these fields with the nonclassicality identifier. Additionally, we show that the nonclassicality identifier can be expressed in a factorized form of detectors quantum efficiencies and the number of modes, if the QOFC consists of many copies of the same two-mode twin beam. As an example, we apply the nonclassicality identifier to two specific types of QOFC, where: (i) the QOFC consists of many independent two-mode twin beams with non-overlapped spatial frequency modes, and (ii) the QOFC contains entangled spatial frequency modes which are completely overlapped, i.e., each mode is entangled with all the remaining modes in the system. We show that, in both cases, the nonclassicality identifier can reveal bipartite entanglement of the QOFC including noise, and that it becomes even more sensitive for the stimulated processes.
An analysis is conducted of the multipartite entanglement for Gaussian states generated by the parametric down-conversion of a femtosecond frequency comb. Using a recently introduced method for constructing optimal entanglement criteria, a family of tests is formulated for mode decompositions that extends beyond the traditional bipartition analyses. A numerical optimization over this family is performed to achieve maximal significance of entanglement verification. For experimentally prepared 4-, 6-, and 10-mode states, full entanglement is certified for all of the 14, 202, and 115 974 possible nontrivial partitions, respectively.