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arXiv:1609.06411 · Scientific Reports

Paramagnetic resonance in spin-polarized disordered Bose-Einstein condensates

V. M. Kovalev, Ivan G. Savenko

Published May 11, 2017• 10 citations
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Abstract

We study the pseudo-spin density response of a disordered two-dimensional spin-polarized Bose gas to weak alternating magnetic field, assuming that one of the spin states of the doublet is macroscopically occupied and Bose-condensed while the occupation of the other state remains much smaller. We calculate spatial and temporal dispersions of spin susceptibility of the gas taking into account spin-flip processes due to the transverse-longitudinal splitting, considering microcavity exciton polaritons as a testbed. Further, we use the Bogoliubov theory of weakly-interacting gases and show that the time-dependent magnetic field power absorption exhibits double resonance structure corresponding to two particle spin states (contrast to paramagnetic resonance in regular spin-polarized electron gas). We analyze the widths of these resonances caused by scattering on the disorder and show that, in contrast with the ballistic regime, in the presence of impurities, the polariton scattering on them is twofold: scattering on the impurity potential directly and scattering on the spatially fluctuating condensate density caused by the disorder. As a result, the width of the resonance associated with the Bose-condensed spin state can be surprisingly narrow in comparison with the width of the resonance associated with the non-condensed state.

DOI
10.1038/s41598-017-01125-4

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We study the pseudo-spin density response of a disordered two-dimensional spin-polarized Bose gas to weak alternating magnetic field, assuming that one of the spin states of the doublet is macroscopically occupied and Bose-condensed while the occupation of the other state remains much smaller. We calculate spatial and temporal dispersions of spin susceptibility of the gas taking into account spin-flip processes due to the transverse-longitudinal splitting, considering microcavity exciton polaritons as a testbed. Further, we use the Bogoliubov theory of weakly-interacting gases and show that the time-dependent magnetic field power absorption exhibits double resonance structure corresponding to two particle spin states (contrast to paramagnetic resonance in regular spin-polarized electron gas). We analyze the widths of these resonances caused by scattering on the disorder and show that, in contrast with the ballistic regime, in the presence of impurities, the polariton scattering on them is twofold: scattering on the impurity potential directly and scattering on the spatially fluctuating condensate density caused by the disorder. As a result, the width of the resonance associated with the Bose-condensed spin state can be surprisingly narrow in comparison with the width of the resonance associated with the non-condensed state.
We study the pseudo-spin density response of a disordered two-dimensional spin-polarized Bose gas of exciton polaritons to weak alternating magnetic field, assuming that one of the spin states of the doublet is macroscopically occupied and Bose-condensed while the occupation of the other state remains much smaller. We calculate spatial and temporal dispersions of spin susceptibility of the gas taking into account spin-flip processes due to the transverse-longitudinal splitting. Further, we use the Bogoliubov theory of weakly-interacting gases and show that the time-dependent magnetic field power absorption exhibits double resonance structure corresponding to two particle spin states (contrast to paramagnetic resonance in regular spin-polarized electron gas). We analyze the widths of these resonances caused by scattering on the disorder and show that, in contrast with the ballistic regime, in the presence of impurities, the polariton scattering on them is twofold: scattering on the impurity potential directly and scattering on the spatially fluctuating condensate density caused by the disorder. As a result, the width of the resonance associated with the Bose-condensed spin state can be surprizingly narrow in comparison with the width of the resonance associated with the non-condensed state.
We present an analytic Bogoliubov description of a Bose-Einstein condensate of polar molecules trapped in a quasi-two-dimensional geometry and interacting via internal state-dependent dipole-dipole interactions. We derive the mean-field ground-state energy functional, and we derive analytic expressions for the dispersion relations, Bogoliubov amplitudes, and static structure factors. This method can be applied to any homogeneous, two-component system with linear coupling and direct, momentum-dependent interactions. The properties of the mean-field ground state, including polarization and stability, are investigated, and we identify three distinct instabilities: a density-wave rotonization that occurs when the gas is fully polarized, a spin-wave rotonization that occurs near zero polarization, and a mixed instability at intermediate fields. The nature of these instabilities is clarified by means of the real-space density-density correlation functions, which characterize the spontaneous fluctuations of the ground state, and the momentum-space structure factors, which characterize the response of the system to external perturbations. We find that the gas is susceptible to both density-wave and spin-wave responses in the polarized limit but only a spin-wave response in the zero-polarization limit. These results are relevant for experiments with rigid rotor molecules such as RbCs, $\mathrm{\ensuremath{\Lambda}}$-doublet molecules such as ThO that have an anomalously small zero-field splitting, and doublet-$\mathrm{\ensuremath{\Sigma}}$ molecules such as SrF where two low-lying opposite-parity states can be tuned to zero splitting by an external magnetic field.
The effect of a magnetic field on a spinor exciton-polariton condensate has been investigated. A quenching of a polariton Zeeman splitting and an elliptical polarization of the condensate have been observed at low magnetic fields B<2 T. The effects are attributed to a competition between the magnetic field induced circular polarization buildup and the spin-anisotropic polariton-polariton interaction which favors a linear polarization. The sign of the circular polarization of the condensate emission at B<3 T is negative, suggesting that a dynamic condensation in the excited spin state rather than the ground spin state takes place in this magnetic field range. From about 2T on, the Zeeman splitting opens and from then on the slope of the circular polarization degree changes its sign. For magnetic fields larger than the 3 T, the upper spin state occupation is energetically suppressed and circularly polarized condensation takes place in the ground state.
The suppression of Zeeman energy splitting due to spin-dependent interactions (the spin Meissner effect) was predicted to occur within a Bose-Einstein condensate. We report a clear observation of this effect in semimagnetic microcavities which exhibit a giant Zeeman energy splitting between two spin-polarized polariton states as high as 2 meV and demonstrate that a partial suppression of the energy difference occurs already in the uncondensed phase in a striking similarity to the behavior of up-critical superconductors in the fluctuation-dominated regime. These observations are explained quantitatively by a kinetic model accounting for both the condensed and uncondensed polaritons and taking into account the nonequilibrium character of the system.
The polaronic system consisting of an impurity in a dilute Bose-Einstein condensate is considered in the presence of a narrow Feshbach resonance. For this purpose a coupled-channel model is used, which at the mean field level predicts the formation of quasiparticles that are a superposition of the impurity and the molecular states. The impurity-boson interactions and the coupling between the open and closed channels are then considered weak and a perturbative calculation of the corrections to the mean field results is presented. This allows to examine the properties of the quasiparticles, such as the lifetime and the effective mass. The model is applied to two physical systems: an impurity atom in a Bose-condensed atomic gas in 3D and a spin down lower polariton in a Bose-Einstein condensate of spin up lower polaritons in 2D. The model parameters are linked to the physical parameters by identifying the low energy T-matrix and applying a proper renormalization scheme.
We consider coherent states of weakly interacting bosons under the conditions of external resonant excitation, with a focus on a two-dimensional polariton fluid driven by a plane electromagnetic wave near the ground state. The coherent driving breaks the U(1) symmetry explicitly, which prevents the occurrence of quantum vortices in a uniform scalar condensate. Surprisingly, a spinor (two-component) system of the same kind admits topological excitations, such as domain walls of relative phase or confined half-vortex molecules, typical of a freely evolving spinor Bose system. Opposite-phase domains arise from the spontaneous breakdown of the spin symmetry (Z2)(\mathbb{Z}_2)(Z2​). Domain walls form with time even when the initial state of the system is uniform or completely disordered; they fall into different topological types distinguished by the total phase variation in the transverse direction. One type of domain walls is similar to ``magnetic'' solitons in Bose-Einstein condensates and exhibits nonzero spin polarization whose sign depends on the direction of motion. Domain walls of the second type, by contrast, behave like monopoles with broken spatiotemporal symmetry and tend to move in certain preferred directions. The interaction of vortices and domain walls results in a long-range ordering of the system.