First observation of the quantized exciton-polariton field and effect of interactions on a single polariton
Álvaro Cuevas, Juan Camilo López Carreño, Blanca Silva, Milena De Giorgi, D. G. Suárez-Forero, Carlos Sánchez Muñoz, Antonio Fieramosca, Filippo Cardano, Lorenzo Marrucci, Vittorianna Tasco, G. Biasiol, Elena del Valle, Lorenzo Dominici, Dario Ballarini, Giuseppe Gigli, Paolo Mataloni, Fabrice P. Laussy, Fabio Sciarrino, D. Sanvitto
Polaritons are quasi-particles that originate from the coupling of light with matter and that demonstrate quantum phenomena at the many-particle mesoscopic level, such as Bose-Einstein condensation and superfluidity. A highly sought and long-time missing feature of polaritons is a genuine quantum manifestation of their dynamics at the single-particle level. Although they are conceptually perceived as entangled states and theoretical proposals abound for an explicit manifestation of their single-particle properties, so far their behavior has remained fully accounted for by classical and mean-field theories. We report the first experimental demonstration of a genuinely quantum state of the microcavity polariton field, by swapping a photon for a polariton in a two-photon entangled state generated by parametric downconversion. When bringing this single-polariton quantum state in contact with a polariton condensate, we observe a disentangling with the external photon. This manifestation of a polariton quantum state involving a single quantum unlocks new possibilities for quantum information processing with interacting bosons.
Polaritons are quasi-particles that originate from the coupling of light with matter and that demonstrate quantum phenomena at the many-particle mesoscopic level, such as Bose-Einstein condensation and superfluidity. A highly sought and long-time missing feature of polaritons is a genuine quantum manifestation of their dynamics at the single-particle level. Although they are conceptually perceived as entangled states and theoretical proposals abound for an explicit manifestation of their single-particle properties, so far their behavior has remained fully accounted for by classical and mean-field theories. We report the first experimental demonstration of a genuinely quantum state of the microcavity polariton field, by swapping a photon for a polariton in a two-photon entangled state generated by parametric downconversion. When bringing this single-polariton quantum state in contact with a polariton condensate, we observe a disentangling with the external photon. This manifestation of a polariton quantum state involving a single quantum unlocks new possibilities for quantum information processing with interacting bosons.
Polaritons are quasi-particles originating from the coupling of light with matter and that demonstrated quantum phenomena at the many-particle mesoscopic level, such as BEC and superuidity. A highly sought and long-time missing feature of polaritons is a genuine quantum manifestation of their dynamics at the single-particle level. Although they are conceptually perceived as entangled states and theoretical proposals abound for an explicit manifestation of their single-particle properties, so far their behaviour remained fully accountable for by classical and mean-field theories. In this Article, we report the first experimental demonstration of a genuinely-quantum manifestation of microcavity polaritons, by swapping the entanglement between a polariton and an external photon from a photon pair generated by parametric down-conversion. Moreover we demonstrate how interactions manifest at a single polariton level by perturbing the entangled state with a rarefied polariton condensate. Our results open the page of quantum polaritonics and implement the first application of quantum spectroscopy.
Bose-Einstein condensation (BEC) is a thermodynamic phase transition of an interacting Bose gas. Its key signatures are remarkable quantum effects like superfluidity and a phonon-like Bogoliubov excitation spectrum, which have been verified for atomic BECs. In the solid state, BEC of exciton-polaritons has been reported. Polaritons are strongly coupled light-matter quasiparticles in semiconductor microcavities and composite bosons. However, they are subject to dephasing and decay and need external pumping to reach a steady state. Accordingly the polariton BEC is a nonequilibrium process of a degenerate polariton gas in self-equilibrium, but out of equilibrium with the baths it is coupled to and therefore deviates from the thermodynamic phase transition seen in atomic BECs. Here we show that key signatures of BEC can even be observed without fulfilling the self-equilibrium condition in a highly photonic quantum degenerate nonequilibrium system.
The main scope of this thesis is the investigation of quantum properties of nonlinear, dissipative, optical and condensed matter systems. Compared with previous studies on this subjects, we reached several milestone of general interests for the theoretical and experimental community. \nThe main experimental platform we refer to in this thesis is microcavity polaritons: polaritons arise from the coupling of light with excitons in a quantum well, i.e., a 2D semiconductor material embedded in the microcavity. They have attracted the interest of the scientific community for their rich physics. Polaritons can form out-of-equilibrium Bose-Einstein condensates, they can experience superfluid phase transition and, due to their interaction via the excitonic component, they show a variety of phenomena which are typical of nonlinear physics, such as bistability and parametric scattering. \nIn particular, motivated by recent proposals about the generation of single photons from weakly nonlinear system, like the unconventional photon blockade, and by the production of squeezed states in polariton systems, we studied the possibility of obtaining antibunched light and other quantum states (like squeezed states and entangled states), when the nonlinear system shows some peculiar features: in particular we consider polariton soliton and cascade systems. \nFinally, when considering nonlinear incoherent processes, we investigate the effect of the PT-symmetry and the PT-symmetry breaking on the quantum state of the emitted light. \nHence, this research work has two main objectives: first, from the fundamental physics point of view, to understand the interplay between nonlinear phenomena and quantum optics, second to provide useful tools for future technological applications. Specifically, for the latter case, we demonstrate a theorem that links the measurement of intensity correlations with the occurrence of certain phase transitions, and we propose a setup to maximize the non-classicality of the light emitted by weakly non-linear systems via a cascade configuration. \n \n \n
Summary form only given. Semiconductor microcavities can be engineered to produce strong coupling between photons and quantum well excitons leading to the formation of new eigenstates called polaritons. Due to their peculiar dispersion, enabling non-equilibrium Bose-Einstein condensation [1], and their straightforward experimental accessibility, microcavity polaritons have gained considerable interest in recent years. Polariton states can be selectively populated by choosing the excitation angle and the wavelength of the excitation laser. After a lifetime of a few picoseconds the polariton decays and a photon is emitted from the cavity, carrying the complete information on the underlying polariton state. Several theoretical works [2-3] suggest that polariton-polariton interactions can be a source of non-classical photon correlations, producing photon pairs that are entangled in either the energy, the polarization, or the momentum degree of freedom. One appeal of such a system is that many parameters such as the polariton-polariton interaction strength are tunable [4] and multipartite entangled states can be created in a single device [5]. However, due to the lack of high-quality samples, experimental realisations of these schemes have been elusive so far. In this contribution, we will discuss some of our experimental work on the statistics of polariton-polariton parametric scattering. Excited polaritons can scatter in a four-wave mixing process into signal and idler states lying on a figure-eight shaped curve in k-space, where phase-matching is fulfilled. We make use of a sample with ultra narrow exciton resonances, which allows for the generation and detection of correlated light. We present our measurements of the second order correlation functions using time-correlated photon counting. We discuss in detail, how polariton quantum correlations depend on a number of experimental parameters, such as phase space location and excitation density and find that the results can be understood in the framework of the well known Bogoliubov theory for 2D Bose gases utilised for microcavity polaritons [6]. We find bunching below the parametric threshold and a slow buildup of coherence above the threshold similar to the quantum statistics of a non-degenerate optical parametric oscillator, which is well known for its nonclassical properties [7]. We discuss in particular the influence of strong background processes on the observed photon statistics.
We review, aiming at an audience of final year undergraduates, the phenomena observed in, and properties of, microcavity exciton–polariton condensates. These are condensates of mixed light and matter, consisting of superpositions of photons in semiconductor microcavities and excitons in quantum wells. Because of the imperfect confinement of the photon component, exciton–polaritons have a finite lifetime, and have to be continuously re-populated. Therefore, exciton–polariton condensates lie somewhere between equilibrium Bose–Einstein condensates and lasers. We review in particular the evidence for condensation, the coherence properties studied experimentally, and the wide variety of spatial structures either observed or predicted to exist in exciton–polariton condensates, including quantised vortices and other coherent structures. We also discuss the question of superfluidity in a non-equilibrium system, reviewing both the experimental attempts to investigate superfluidity to date, and the theoretical suggestions of how it may be further elucidated.
Two-photon absorption (TPA) allows accessing “dark” states of matter that are otherwise inaccessible to light, which serve as important building blocks for quantum information processing. In a semiconductor microcavity, TPA-driven condensation of strongly coupled light-matter exciton–polaritons can enable new solid-state quantum simulations of “dark” state-condensate interactions and was predicted to stimulate THz emission. Here, we report the first observation of two-photon-pumped polariton condensation, demonstrated by angle-resolved photoluminescence in a GaAs-based microcavity. TPA is evidenced in the quadratic emission dependence on pump power below and above the condensation threshold, and second-harmonic generation is ruled out by both this threshold behavior and by the emission peak energy showing no dependence on pump photon energy. Our results pave the way toward novel polariton-based sources and solid-state coherent control of collective quantum states with individual two-level systems.