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arXiv:1608.05049

The driven Dicke Model: time-dependent mean field and quantum fluctuations in a non-equilibrium quantum many-body system

Gianluca Francica, Simone Montangero, Mauro Paternostro, Francesco Plastina

Published Aug 17, 2016• 1 citation
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Abstract

We establish a new theoretical framework, based on a time-dependent mean field approach, to address the dynamics of the driven Dicke model. The joint evolution of both mean fields and quantum fluctuations gives rise to a rich and generally non-linear dynamics, featuring a normal (stable) regime and an unstable, super-radiant one. Various dynamical phenomena emerge, such as the spontaneous amplification of vacuum fluctuations, or the appearance of special points around which the mean-field amplitudes rotate during driven time evolution, signalling a dynamical symmetry breaking. We also provide a characterization of the driving-induced photon production in terms of the work done by the driving agent, of the non-adiabaticity of the process and of the entanglement generated between the atomic system and the cavity mode.

DOI
10.48550/arxiv.1608.05049

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Present-day experiments have started to couple traditional simulations of ultracold atom experiments with quantum light-fields in cavities. This has provided a wealth of op- portunities to enlarge the number of interaction potentials: cavity mediated long-range interactions compete with kinetic energies, longitudinal fields, short-ranged collisional or magnetic spin-spin interactions. The intracavity many-body lattice models often have to be maintained far from equilibrium through the presence of external driving lasers that help to boost and engineer the various interaction potentials. The steady influx of energy is compensated by a steady stream of energy out of the atom-cavity system for example by photon losses or atomic spontaneous emission. 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As the generic model for atom-light interactions, it has been experimen- tally realized in a variety of modern quantum optical systems, highlighting its relevance for present-day research. The Dicke model is also highly versatile itself. It has been extended into the dissipative realm, was promoted to account for multiple optical light modes and was used to describe multiple, coupled single-mode cavity structures. It was adapted to treat spin-selective coupling to a cavity to describe superradiance phase tran- sitions in multi-level atomic systems. Moreover, it was realised in electronic circuits where the dipole coupling of real atoms to single mode fields is replaced by a capacitive cou- pling of artificial atoms to a resonator mode. This illustrates that the Dicke model and its extended variants are ’future-proof’ and continue to be of relevance for fundamental light-matter interactions and for driven-dissipative phase transitions. \nIn this thesis, we investigate magnetic phase transitions in driven-dissipative atomic en- sembles interacting with quantum light. We present three research projects on variants of cooperative radiation of an ensemble of laser driven two-level atoms in a single mode optical cavity, as described by the Dicke model. \nThroughout the chapters 2,3 and 4 that contain the main body of research of this thesis, we investigate phase transitions between non-equilibrium stationary states in engineered quantum-optical systems each of which extends the conventional Dicke model physics. As a starting point, we map the quantum equations of motion onto a set of semiclassical nonlinear stochastic equations and analyse their stationary states and instabilities with master equations for atomic spin and photon mean-field amplitudes. These are used to obtain experimentally relevant parameters such as critical atom-light couplings for phase transitions, phase diagrams and properties of stationary non-equilibrium states in addition to cavity output spectra that identify the imprint of magnetic correlations in the light-field. \nIn chapter 2, we help resolve a discrepancy between earlier experimental investigations of the critical atom-light coupling strength for the superradiance transition in the Dicke model: higher external pumping strengths than theoretically predicted were needed to observe a coherent, superradiant state of the light field in an optical cavity. By including incoherent spontaneous emission of atomic excitations, we extend the dissipative Dicke model to a two loss channel variant containing both photon leakage and atomic decay that reproduces the experimentally observed critical atom-light coupling. \nRecent experiments have started to interface quantum many body lattice models with coherent cavity fields, thereby allowing to realize new quantum phases through competing atom-cavity and atom-atom interactions. In chapter 3, we consider a simplified model for such a set-up where a single quantized mode of the light-field interacts with an ensemble of Rydberg-dressed atoms inside a high finesse optical cavity. This model provides a base case for further studies of quantum magnets in optical cavities. At the heart of this model is a competition of short- (dipolar atom-atom) and long-range (atom-light) interactions at the Hamiltonian level in the presence of both spontaneous emission and photon leak- age through the cavity mirrors. We show that different magnetic phases can coexist with coherent atomic radiation and provide clear experimental signatures to identify the mag- netic structure and intra-cavity dynamics. We suggest an experimental level-scheme for a quantum optical implementation of our model. \nIn chapter 4 we consider a generic, collective decay for many-body excitations in the paradigmatic Dicke model. This extension drastically enriches the dynamics as it induces a bicritical point and a bistable regime dominated by true non-equilibrium fluctuations that induce a dissipative first-order phase transition that can only be resolved by including finite fluctuation corrections with the help of stochastic Langevin equations. We investigate the hysteretic response to time-dependent ramps of the atom-light coupling. Discontinuous first-order phase transitions where metastable states coexist in a hysteresis domain have been investigated in recent dissipative quantum-optical experiments. We review noise- activation far from thermal equilibrium in chapter 5.

•Aug 1, 2018•0 citations
We establish a new theoretical framework, based on a time-dependent mean field approach, to address the dynamics of the driven Dicke model. The joint evolution of both mean fields and quantum fluctuations gives rise to a rich and generally non-linear dynamics, featuring a normal (stable) regime and an unstable, super-radiant one. Various dynamical phenomena emerge, such as the spontaneous amplification of vacuum fluctuations, or the appearance of special points around which the mean-field amplitudes rotate during driven time evolution, signalling a dynamical symmetry breaking. We also provide a characterization of the driving-induced photon production in terms of the work done by the driving agent, of the non-adiabaticity of the process and of the entanglement generated between the atomic system and the cavity mode.
We establish a new theoretical framework, based on a time-dependent mean field approach, to address the dynamics of the driven Dicke model, describing, e.g., an atomic sample of N teo-level systems coupled to a cavity field, and driven by an external pump. We provide a description of the dynamics that also includes the effects of quantum fluctuations. The joint evolution of both mean fields and quantum fluctuations gives rise to a rich and generally non-linear dynamics, featuring a normal and a super radiant regime, which are the dynamical counterpart of the two static quantum phases. Various dynamical phenomena emerge, such as the spontaneous amplification of vacuum fluctuations, or the appearance of three stable points around which the mean field amplitudes rotate during time evolution. We also provide a characterization of the driving induced photon production by analyzing the average photon number, the Mandel parameter, the work done by the driving agent, and the non-adiabaticity of the process, evaluated in terms of the inner friction. Finally, we discuss the squeezing and the entanglement between the atomic system and the cavity mode.
Control and manipulation of quantum engineered systems allows for the utilization of time-dependent parametric modulations for accessing novel out-of-equilibrium phenomena. In the absence of such driving, the dissipative Dicke model exhibits a fascinating out-of-equilibrium many-body phase transition as a function of a coupling between a driven photonic cavity and numerous two-level atoms. We study the effect of a parametric modulation of this coupling and discover a rich phase diagram as a function of the modulation strength. We find that in addition to the established normal and super-radiant phases, a new phase with pulsed superradiance, which we term dynamical normal phase, appears when the system is parametrically driven. Employing different methods, we characterize the different phases and the transitions between them. Specific heed is paid to the role of dissipation in determining the phase boundaries. Our analysis paves the road for the experimental study of dynamically stabilized phases of interacting light and matter.
Abstract The Dicke model—a paradigmatic example of superradiance in quantum optics—describes an ensemble of atoms which are collectively coupled to a leaky cavity mode. As a result of the cooperative nature of these interactions, the system’s dynamics is captured by the behavior of a single mean-field, collective spin. In this mean-field limit, it has recently been shown that the interplay between photon losses and periodic driving of light–matter coupling can lead to time-crystalline-like behavior of the collective spin (Gong et al 2018 Phys. Rev. Lett. 120 040404). In this work, we investigate whether such a Dicke time crystal (TC) is stable to perturbations that explicitly break the mean-field solvability of the conventional Dicke model. In particular, we consider the addition of short-range interactions between the atoms which breaks the collective coupling and leads to complex many-body dynamics. In this context, the interplay between periodic driving, dissipation and interactions yields a rich set of dynamical responses, including long-lived and metastable Dicke-TCs, where losses can cool down the many-body heating resulting from the continuous pump of energy from the periodic drive. Specifically, when the additional short-range interactions are ferromagnetic, we observe time crystalline behavior at non-perturbative values of the coupling strength, suggesting the possible existence of stable dynamical order in a driven-dissipative quantum many-body system. These findings illustrate the rich nature of novel dynamical responses with many-body character in quantum optics platforms.
The dissipative quantum phase transitions experienced by a driven optical system are studied in order to understand the underlying light-matter coupling. The primary system under study is composed of a cavity mode coupled to a two-level system with dissipation being introduced through the interaction with a surrounding environment; an external coherent field is included to drive the system out of the ground state. The coupling is given by a generalized Rabi Hamiltonian, where rotating, gr, and counter-rotating, ngr, couplings are both present and can be adjusted independently. A comprehensive study of the different phases the system can exhibit as gr and n are varied is presented. From this, we construct a bridge between two limiting scenarios: (i) the Jaynes-Cummings limit (n = 0), where the system undergoes a phase transition by means of the breakdown of the photon blockade, and (ii) the driven Dicke limit ( = 1 ), where the normal to super-radiant phase transition is found. Novel behaviour encountered in an intermediate regime (1 > n > 0) is discussed. Attention is drawn towards the strong coupling regime, where changes at the one-photon level induce nonlinear effects and behaviour reminiscent of phase transitions is encountered with just a few photons present. A comparison between weak and strong coupling regimes, and, thus, an exploration of the effect of fluctuations over quantum phase transitions of light, is given through a survey of the phases an auxiliary optical system exhibits. This system is composed of two coupled nonlinear cavities that are driven coherently and damped through the interaction with the environment; it is seen to exhibit three phases. Two phases present high-correlation between the cavities and are differentiated by the photon statistics, transitioning from classical to quantum. The third phase is characterized by a highly localized field in one of the cavities. The departure from mean-field results is highlighted and a new way to characterize the possible phases of the system is proposed. Finally, the crucial role of quantum fluctuations is quantified and used to define the phases at hand.
In this thesis, we study the nonequilibrium dynamics of the time dependent single mode Dicke model in the thermodynamic limit in the context of the Liouville-von Neumann canonical method. We report an exact solution for this model under a non-equilibrium situation, generated by time dependent control parameters. We compute the correlations: in the atom-field ground state by means of the density operator for the pure state of the universe, and the corresponding reduced density operator for the atoms when the field is in resonance with the atomic ensemble. We obtain a closed relationship between the correlations in the ground state, the localisation of the atom¿s Wigner function in phase space, and the localisation of the wave function of the universe. As a measure of bipartite entanglement, we calculate the linear entropy from which we study the atom-field entanglement dynamics. In particular, we find a strong relationship between the stability of the auxiliary dynamical parameters, the reported entanglement, and the dynamics of certain physical observables. Furthermore, we use the Liouville-von Neumann technique to study the influence of quantum and thermal fluctuations on the dynamics of the normal and the superradiant phase. In addition, we calculate the density matrix for the quantum mechanical evolution of an initial thermal equilibrium state in the case of an instantaneous atom-field coupling and time independent ω and ω0.
Present-day experiments have started to couple traditional simulations of ultracold atom experiments with quantum light-fields in cavities. This has provided a wealth of op- portunities to enlarge the number of interaction potentials: cavity mediated long-range interactions compete with kinetic energies, longitudinal fields, short-ranged collisional or magnetic spin-spin interactions. The intracavity many-body lattice models often have to be maintained far from equilibrium through the presence of external driving lasers that help to boost and engineer the various interaction potentials. The steady influx of energy is compensated by a steady stream of energy out of the atom-cavity system for example by photon losses or atomic spontaneous emission. Several experiments have demonstrated that such environments can give rise to new competing quantum phases. \nBut this long-standing ambition to push for models with tailorable interaction potentials can bring with it also considerable challenges in their theoretical description, since sponta- neous symmetry breaking transitions in many body lattice systems coupled to dynamical light-fields with single-photon character occur in the presence of drive and dissipation for the photonic force carriers. This clearly calls for model systems where the above men- tioned interplay of interactions, drive, dissipation and cooperative many-body behaviour can be theoretically studied to provide simple, experimentally verifiable predictions. \nThe Dicke model is, through its simplicity (an exactly solved ferromagnet with infinite range atom-atom interactions mediated by a single cavity mode), an exceptionally well- suited candidate. As the generic model for atom-light interactions, it has been experimen- tally realized in a variety of modern quantum optical systems, highlighting its relevance for present-day research. The Dicke model is also highly versatile itself. It has been extended into the dissipative realm, was promoted to account for multiple optical light modes and was used to describe multiple, coupled single-mode cavity structures. It was adapted to treat spin-selective coupling to a cavity to describe superradiance phase tran- sitions in multi-level atomic systems. Moreover, it was realised in electronic circuits where the dipole coupling of real atoms to single mode fields is replaced by a capacitive cou- pling of artificial atoms to a resonator mode. This illustrates that the Dicke model and its extended variants are ’future-proof’ and continue to be of relevance for fundamental light-matter interactions and for driven-dissipative phase transitions. \nIn this thesis, we investigate magnetic phase transitions in driven-dissipative atomic en- sembles interacting with quantum light. We present three research projects on variants of cooperative radiation of an ensemble of laser driven two-level atoms in a single mode optical cavity, as described by the Dicke model. \nThroughout the chapters 2,3 and 4 that contain the main body of research of this thesis, we investigate phase transitions between non-equilibrium stationary states in engineered quantum-optical systems each of which extends the conventional Dicke model physics. As a starting point, we map the quantum equations of motion onto a set of semiclassical nonlinear stochastic equations and analyse their stationary states and instabilities with master equations for atomic spin and photon mean-field amplitudes. These are used to obtain experimentally relevant parameters such as critical atom-light couplings for phase transitions, phase diagrams and properties of stationary non-equilibrium states in addition to cavity output spectra that identify the imprint of magnetic correlations in the light-field. \nIn chapter 2, we help resolve a discrepancy between earlier experimental investigations of the critical atom-light coupling strength for the superradiance transition in the Dicke model: higher external pumping strengths than theoretically predicted were needed to observe a coherent, superradiant state of the light field in an optical cavity. By including incoherent spontaneous emission of atomic excitations, we extend the dissipative Dicke model to a two loss channel variant containing both photon leakage and atomic decay that reproduces the experimentally observed critical atom-light coupling. \nRecent experiments have started to interface quantum many body lattice models with coherent cavity fields, thereby allowing to realize new quantum phases through competing atom-cavity and atom-atom interactions. In chapter 3, we consider a simplified model for such a set-up where a single quantized mode of the light-field interacts with an ensemble of Rydberg-dressed atoms inside a high finesse optical cavity. This model provides a base case for further studies of quantum magnets in optical cavities. At the heart of this model is a competition of short- (dipolar atom-atom) and long-range (atom-light) interactions at the Hamiltonian level in the presence of both spontaneous emission and photon leak- age through the cavity mirrors. We show that different magnetic phases can coexist with coherent atomic radiation and provide clear experimental signatures to identify the mag- netic structure and intra-cavity dynamics. We suggest an experimental level-scheme for a quantum optical implementation of our model. \nIn chapter 4 we consider a generic, collective decay for many-body excitations in the paradigmatic Dicke model. This extension drastically enriches the dynamics as it induces a bicritical point and a bistable regime dominated by true non-equilibrium fluctuations that induce a dissipative first-order phase transition that can only be resolved by including finite fluctuation corrections with the help of stochastic Langevin equations. We investigate the hysteretic response to time-dependent ramps of the atom-light coupling. Discontinuous first-order phase transitions where metastable states coexist in a hysteresis domain have been investigated in recent dissipative quantum-optical experiments. We review noise- activation far from thermal equilibrium in chapter 5.