Abstract The Dicke model—a paradigmatic example of superradiance in quantum optics—describes an ensemble of atoms which are collectively coupled to a leaky cavity mode. As a result of the cooperative nature of these interactions, the system’s dynamics is captured by the behavior of a single mean-field, collective spin. In this mean-field limit, it has recently been shown that the interplay between photon losses and periodic driving of light–matter coupling can lead to time-crystalline-like behavior of the collective spin (Gong et al 2018 Phys. Rev. Lett. 120 040404). In this work, we investigate whether such a Dicke time crystal (TC) is stable to perturbations that explicitly break the mean-field solvability of the conventional Dicke model. In particular, we consider the addition of short-range interactions between the atoms which breaks the collective coupling and leads to complex many-body dynamics. In this context, the interplay between periodic driving, dissipation and interactions yields a rich set of dynamical responses, including long-lived and metastable Dicke-TCs, where losses can cool down the many-body heating resulting from the continuous pump of energy from the periodic drive. Specifically, when the additional short-range interactions are ferromagnetic, we observe time crystalline behavior at non-perturbative values of the coupling strength, suggesting the possible existence of stable dynamical order in a driven-dissipative quantum many-body system. These findings illustrate the rich nature of novel dynamical responses with many-body character in quantum optics platforms.
Abstract The Dicke model—a paradigmatic example of superradiance in quantum optics—describes an ensemble of atoms which are collectively coupled to a leaky cavity mode. As a result of the cooperative nature of these interactions, the system’s dynamics is captured by the behavior of a single mean-field, collective spin. In this mean-field limit, it has recently been shown that the interplay between photon losses and periodic driving of light–matter coupling can lead to time-crystalline-like behavior of the collective spin (Gong et al 2018 Phys. Rev. Lett. 120 040404). In this work, we investigate whether such a Dicke time crystal (TC) is stable to perturbations that explicitly break the mean-field solvability of the conventional Dicke model. In particular, we consider the addition of short-range interactions between the atoms which breaks the collective coupling and leads to complex many-body dynamics. In this context, the interplay between periodic driving, dissipation and interactions yields a rich set of dynamical responses, including long-lived and metastable Dicke-TCs, where losses can cool down the many-body heating resulting from the continuous pump of energy from the periodic drive. Specifically, when the additional short-range interactions are ferromagnetic, we observe time crystalline behavior at non-perturbative values of the coupling strength, suggesting the possible existence of stable dynamical order in a driven-dissipative quantum many-body system. These findings illustrate the rich nature of novel dynamical responses with many-body character in quantum optics platforms.
The interplay between many-body interactions and controlled dissipation provides a rich setting for nonequilibrium quantum phases. We explore the superradiant phase transitions in a Rydberg-interacting open Dicke model with cavity loss and local dissipation. We find that the nonlinear feedback from atomic interactions stabilizes the atomic collective excited state and induces resonant collective motion, which can be further converted into robust superradiant oscillations with the inclusion of local dissipation. Beyond the mean-field approximation, we prove this system can support the finite-size local dissipative temporal order, i.e., continuous time crystal, from evidences of the decreasing damping of a finite-frequency Liouvillian mode and the linear-size scaling of quantum fluctuations. The correlation between the atomic colletive dynamics and the cavity photon number makes our findings easy to detect from output optical signal. By bridging interacting atomic matter and driven-dissipative cavity QED, our Rydberg-interacting Dicke model provides a unique spin-1/2 platform for exploring dynamical phase transitions and macroscopic temporal order in open quantum matter.
Present-day experiments have started to couple traditional simulations of ultracold atom experiments with quantum light-fields in cavities. This has provided a wealth of op- portunities to enlarge the number of interaction potentials: cavity mediated long-range interactions compete with kinetic energies, longitudinal fields, short-ranged collisional or magnetic spin-spin interactions. The intracavity many-body lattice models often have to be maintained far from equilibrium through the presence of external driving lasers that help to boost and engineer the various interaction potentials. The steady influx of energy is compensated by a steady stream of energy out of the atom-cavity system for example by photon losses or atomic spontaneous emission. Several experiments have demonstrated that such environments can give rise to new competing quantum phases. \nBut this long-standing ambition to push for models with tailorable interaction potentials can bring with it also considerable challenges in their theoretical description, since sponta- neous symmetry breaking transitions in many body lattice systems coupled to dynamical light-fields with single-photon character occur in the presence of drive and dissipation for the photonic force carriers. This clearly calls for model systems where the above men- tioned interplay of interactions, drive, dissipation and cooperative many-body behaviour can be theoretically studied to provide simple, experimentally verifiable predictions. \nThe Dicke model is, through its simplicity (an exactly solved ferromagnet with infinite range atom-atom interactions mediated by a single cavity mode), an exceptionally well- suited candidate. As the generic model for atom-light interactions, it has been experimen- tally realized in a variety of modern quantum optical systems, highlighting its relevance for present-day research. The Dicke model is also highly versatile itself. It has been extended into the dissipative realm, was promoted to account for multiple optical light modes and was used to describe multiple, coupled single-mode cavity structures. It was adapted to treat spin-selective coupling to a cavity to describe superradiance phase tran- sitions in multi-level atomic systems. Moreover, it was realised in electronic circuits where the dipole coupling of real atoms to single mode fields is replaced by a capacitive cou- pling of artificial atoms to a resonator mode. This illustrates that the Dicke model and its extended variants are ’future-proof’ and continue to be of relevance for fundamental light-matter interactions and for driven-dissipative phase transitions. \nIn this thesis, we investigate magnetic phase transitions in driven-dissipative atomic en- sembles interacting with quantum light. We present three research projects on variants of cooperative radiation of an ensemble of laser driven two-level atoms in a single mode optical cavity, as described by the Dicke model. \nThroughout the chapters 2,3 and 4 that contain the main body of research of this thesis, we investigate phase transitions between non-equilibrium stationary states in engineered quantum-optical systems each of which extends the conventional Dicke model physics. As a starting point, we map the quantum equations of motion onto a set of semiclassical nonlinear stochastic equations and analyse their stationary states and instabilities with master equations for atomic spin and photon mean-field amplitudes. These are used to obtain experimentally relevant parameters such as critical atom-light couplings for phase transitions, phase diagrams and properties of stationary non-equilibrium states in addition to cavity output spectra that identify the imprint of magnetic correlations in the light-field. \nIn chapter 2, we help resolve a discrepancy between earlier experimental investigations of the critical atom-light coupling strength for the superradiance transition in the Dicke model: higher external pumping strengths than theoretically predicted were needed to observe a coherent, superradiant state of the light field in an optical cavity. By including incoherent spontaneous emission of atomic excitations, we extend the dissipative Dicke model to a two loss channel variant containing both photon leakage and atomic decay that reproduces the experimentally observed critical atom-light coupling. \nRecent experiments have started to interface quantum many body lattice models with coherent cavity fields, thereby allowing to realize new quantum phases through competing atom-cavity and atom-atom interactions. In chapter 3, we consider a simplified model for such a set-up where a single quantized mode of the light-field interacts with an ensemble of Rydberg-dressed atoms inside a high finesse optical cavity. This model provides a base case for further studies of quantum magnets in optical cavities. At the heart of this model is a competition of short- (dipolar atom-atom) and long-range (atom-light) interactions at the Hamiltonian level in the presence of both spontaneous emission and photon leak- age through the cavity mirrors. We show that different magnetic phases can coexist with coherent atomic radiation and provide clear experimental signatures to identify the mag- netic structure and intra-cavity dynamics. We suggest an experimental level-scheme for a quantum optical implementation of our model. \nIn chapter 4 we consider a generic, collective decay for many-body excitations in the paradigmatic Dicke model. This extension drastically enriches the dynamics as it induces a bicritical point and a bistable regime dominated by true non-equilibrium fluctuations that induce a dissipative first-order phase transition that can only be resolved by including finite fluctuation corrections with the help of stochastic Langevin equations. We investigate the hysteretic response to time-dependent ramps of the atom-light coupling. Discontinuous first-order phase transitions where metastable states coexist in a hysteresis domain have been investigated in recent dissipative quantum-optical experiments. We review noise- activation far from thermal equilibrium in chapter 5.
We investigate the emergence of a time crystal (TC) in a driven dissipative many-body spin array. In this system the interplay between incoherent spin pumping and collective emission stabilizes a synchronized non-equilibrium steady state which in the thermodynamic limit features a self-generated time-periodic pattern imposed by collective elastic interactions. In contrast to prior realizations where the time symmetry is already broken by an external drive, here it is only spontaneously broken by the elastic exchange interactions and manifest in the two-time correlation spectrum. Employing a combination of exact numerical calculations and a second-order cumulant expansion, we investigate the impact of many-body correlations on the TC formation and establish a connection between the regime where it is stable and where the system features a slow growth rate of the mutual information. This observation allows us to conclude that the TC studied here is an emergent semi-classical out-of-equilibrium state of matter. We also confirm the rigidity of the TC to single-particle dephasing. Finally, we discuss an experimental implementation using long lived dipoles in an optical cavity.
We elucidate the role that the dissipation in a bosonic channel plays in the prevalence and stability of time crystals (TCs) in a periodically driven spin-boson system described by the Dicke model. Here, the bosons are represented by photons, and they mediate the infinite-range interactions between the spin systems. For strong dissipation, we study the dynamics using an effective atom-only description and the closed Lipkin-Meshkov-Glick model. By mapping out the phase diagrams for varying dissipation strengths, ranging from zero to infinitely strong, we demonstrate that the area in the phase diagram, where a TC exists, grows with the dissipation strength but only up to an optimal point, beyond which most of the TCs become unstable. We find TCs in both closed-system and dissipative regimes, but dissipative TCs are shown to be more robust against random noise in the drive and are only weakly affected by the choice of initial state. We present the finite-sized behavior and the scaling of the lifetime of the TCs with respect to the number of spins and the interaction strength within a fully quantum mechanical description.
The Dicke model is a paradigmatic quantum-optical model describing the interaction of a collection of two-level systems with a single bosonic mode. Effective implementations of this model made it possible to observe the emergence of superradiance, i.e., cooperative phenomena arising from the collective nature of light-matter interactions. Via reservoir engineering and analogue quantum simulation techniques, current experimental platforms allow us not only to implement the Dicke model but also to design more exotic interactions, such as the two-photon Dicke model. In the Hamiltonian case, this model presents an interesting phase diagram characterized by two quantum criticalities: a superradiant phase transition and a spectral collapse, that is, the coalescence of discrete energy levels into a continuous band. Here, we investigate the effects of both qubit and photon dissipation on the phase transition and on the instability induced by the spectral collapse. Using a mean-field decoupling approximation, we analytically obtain the steady-state expectation values of the observables signaling a symmetry breaking, identifying a first-order phase transition from the normal to the superradiant phase. Our stability analysis unveils a very rich phase diagram, which features stable, bistable, and unstable phases depending on the dissipation rate.
We investigate the emergence of a time crystal in a driven-dissipative many-body spin array. In this system the interplay between incoherent spin pumping and collective emission stabilizes a synchronized non-equilibrium steady state which in the thermodynamic limit features a self-generated time-periodic pattern imposed by collective elastic interactions. In contrast to prior realizations where the time symmetry is already broken by an external drive, here it is only spontaneously broken by the elastic exchange interactions and manifest in the two-time correlation spectrum. Employing a combination of exact numerical calculations and a second-order cumulant expansion, we investigate the impact of many-body correlations on the time crystal formation and establish a connection between the regime where it is stable and a slow growth rate of the mutual information, signalling that the time crystal studied here is an emergent semi-classical out-of-equilibrium state of matter. We also confirm the rigidity of the time crystal to single-particle dephasing. Finally, we discuss an experimental implementation using long-lived dipoles in an optical cavity