The ability to manipulate single photons is of critical importance for fundamental quantum optics studies and practical implementations of quantum communications. While extraordinary progresses have been made in controlling spatial, temporal, spin and orbit angular momentum degrees of freedom, frequency-domain control of single photons so far relies on nonlinear optical effects, which have faced obstacles such as noise photons, narrow bandwidth and demanding optical filtering. Here we demonstrate the first integrated near-unity efficiency frequency manipulation of single photons, by stretching and compressing a waveguide at 8.3 billion cycles per second. Frequency shift up to 150 GHz at telecom wavelength is realized without measurable added noise and the preservation of quantum coherence is verified through quantum interference between twin photons of different colors. This single photon frequency control approach will be invaluable for increasing the channel capacity of quantum communications and compensating frequency mismatch between quantum systems, paving the road toward hybrid quantum network.
The ability to manipulate single photons is of critical importance for fundamental quantum optics studies and practical implementations of quantum communications. While extraordinary progresses have been made in controlling spatial, temporal, spin and orbit angular momentum degrees of freedom, frequency-domain control of single photons so far relies on nonlinear optical effects, which have faced obstacles such as noise photons, narrow bandwidth and demanding optical filtering. Here we demonstrate the first integrated near-unity efficiency frequency manipulation of single photons, by stretching and compressing a waveguide at 8.3 billion cycles per second. Frequency shift up to 150 GHz at telecom wavelength is realized without measurable added noise and the preservation of quantum coherence is verified through quantum interference between twin photons of different colors. This single photon frequency control approach will be invaluable for increasing the channel capacity of quantum communications and compensating frequency mismatch between quantum systems, paving the road toward hybrid quantum network.
Manipulating the frequency and bandwidth of nonclassical light is essential for implementing frequency-encoded/multiplexed quantum computation, communication, and networking protocols, and for bridging spectral mismatch among various quantum systems. However, quantum spectral control requires a strong nonlinearity mediated by light, microwave, or acoustics, which is challenging to realize with high efficiency, low noise, and on an integrated chip. Here, we demonstrate both frequency shifting and bandwidth compression of heralded single-photon pulses using an integrated thin-film lithium niobate (TFLN) phase modulator. We achieve record-high electro-optic frequency shearing of telecom single photons over terahertz range (±641 GHz or ±5.2 nm), enabling high visibility quantum interference between frequency-nondegenerate photon pairs. We further operate the modulator as a time lens and demonstrate over eighteen-fold (6.55 nm to 0.35 nm) bandwidth compression of single photons. Our results showcase the viability and promise of on-chip quantum spectral control for scalable photonic quantum information processing.
Spectral-temporal manipulation of optical pulses has enabled numerous developments within a broad range of research topics, ranging from fundamental science to practical applications. Within quantum optics spectral-temporal degree of freedom of light offers a promising platform for integrated photonic quantum information processing. An important challenge in experimentally realizing spectral-temporal manipulation of quantum states of light is the need for highly efficient manipulation tools. In this context the intrinsically deterministic electro-optic methods show great promise for quantum applications. We experimentally demonstrate application of electro-optic platform for spectral-temporal manipulation of ultrashort pulsed quantum light. Using techniques analogous to serrodyne frequency shifting we show active spectral translation of few-picosecond single photon pulses by up to 0.5 THz. By employing an approach based on an electro-optic time lens we demonstrate up to 6-fold spectral compression of heralded single photon pulses with efficiency that enables us to significantly increase single photon flux through a narrow bandpass filter. We realize the required temporal phase manipulation by driving a lithium niobate waveguided electrooptic modulator with 33 dBm sinusoidal RF field at the frequency of either 10 GHz or 40 GHz. We use a phase lock loop to temporally lock the RF field to the 80 MHz repetition rate of approximately 1 ps long optical pulses. Heralded single photon wavepackets are generated by means of spontaneous parametric down-conversion in potassium dihydrogen phosphate (KDP) crystal, which enables preparation of spectrally pure single photon wavepackets without the need for spectral filtering. Spectral shifting is achieved by locking single-photon pulses to the linear slope of sinusoidal 40 GHz RF phase modulation. We verify the spectral shift by performing spectrally resolved heralded single photon counting, using frequency-to-time conversion by means of a highly dispersive chirped fiber Bragg grating. We verify the non-classicality of spectrally shifted single photons by measuring high-visibility Hong-Ou-Mandel interference using a reference single photon pulse. Spectral compression is based on the time lens principle, which requires locking optical pulses to approximately quadratic region of sinusoidal phase modulation. We utilize both 10 GHz and 40 GHz RF driving frequencies. Bandwidth compression is achieved by chirping the single photon pulse using an appropriate length of single-mode fibre and subsequently subjecting it to the action of the time lens. We verify spectral compression directly using the aforementioned spectrally-resolved heralded single photon counting method. We achieve 3-fold spectral compression of 2 nm bandwidth single photon pulses using 40 GHZ modulation frequency, and 6-fold spectral compression of 0.9 nm bandwidth single photon pulses using 10 GHz modulation frequency. Overall transmission of our set-up exceeding 30% enables practical usability of our spectral compression method which we demonstrate experimentally by showing an increased photon flux through a narrowband filter. Our results present an important contribution towards implementing quantum information processing in the spectral-temporal degree of freedom of a photon. In the context of quantum networks they present an enabling tool towards efficient photonic interfacing of different quantum information processing platforms.
Single-photon frequency conversion for quantum interface plays an important role in quantum communications and networks, which is crucial for the realization of quantum memory, faithful entanglement swapping and quantum teleportation. In this talk, I will present our recent experiments about single-photon frequency conversion based on quadratic nonlinear processes. Firstly, we demonstrated spectrum compression of broadband single photons at the telecom wavelength to the near-visible window. A positively chirped single-photon-level laser pulse and a negatively chirped classical one are converted to a narrowband single-photon pulse, with a spectrum compression factor of 58, through sum-frequency generation (SFG), marking a critical step towards coherent photonic interface. Secondly, we demonstrated the nonlinear interaction between two chirped broadband single-photon-level coherent states. A high SFG efficiency of 1.06 × 10−7 is realized, which may be utilized to achieve heralding entanglement at a distance. Finally, we theoretically introduced and experimentally demonstrated single-photon frequency conversion in the telecom band, enabling switching of single photons between dense wavelength-division multiplexing channels. Using cascaded quasi-phase matched sum/difference frequency generation, the signal photon of a photon pair from spontaneous down-conversion is precisely shifted to identically match its counterpart, i.e. idler photon, in frequency to manifest a clear non-classical dip in the Hong-Ou-Mandel interference. Moreover, quantum entanglement between the photon pair is maintained after the frequency conversion. Our researches have realized three significant quantum interfaces via single-photon frequency conversion, which hold great promise for the development of quantum communications and networks.
Single-photon frequency conversion for quantum interface plays an important role in quantum communications and networks, which is crucial for the realization of quantum memory, faithful entanglement swapping and quantum teleportation. In this chapter, we will present our recent experiments about single-photon frequency conversion based on quadratic nonlinear processes. Firstly, we demonstrated spectrum compression of broadband single photons at the telecom wavelength to the near-visible window, marking a critical step towards coherent photonic interface. Secondly, we demonstrated the nonlinear interaction between two chirped broadband single-photon-level coherent states, which may be utilized to achieve heralding entanglement at a distance. Finally, we theoretically introduced and experimentally demonstrated single-photon frequency conversion in the telecom band, enabling switching of single photons between dense wavelength-division multiplexing channels. Moreover, quantum entanglement between the photon pair is maintained after the frequency conversion. Our researches have realized three significant quantum interfaces via single-photon frequency conversion, which hold great promise for the development of quantum communications and networks.
Abstract Manipulating the frequency and bandwidth of nonclassical light is essential for implementing frequency-encoded/multiplexed quantum computation, communication, and networking protocols, and for bridging spectral mismatch among various quantum systems. However, quantum spectral control requires a strong nonlinearity mediated by light, microwave, or acoustics, which is challenging to realize with high efficiency, low noise, and on an integrated chip. Here, we demonstrate both frequency shifting and bandwidth compression of nonclassical light using an integrated thin-film lithium niobate (TFLN) phase modulator. We achieve record-high electro-optic frequency shearing of telecom single photons over terahertz range (± 641 GHz or ± 5.2 nm), enabling high visibility quantum interference between frequency-nondegenerate photon pairs. We further operate the modulator as a time lens and demonstrate over eighteen-fold (6.55 nm to 0.35 nm) bandwidth compression of single photons. Our results showcase the viability and promise of on-chip quantum spectral control for scalable photonic quantum information processing.
We demonstrate a quantum interface that simultaneously converts the wavelength, bandwidth, and duration of single-photon-level pulses, enabling compatibility between disparate quantum systems. Using difference frequency generation in a lithium niobate waveguide driven by a highly chirped pump, we transform pulses from 798 nm, 5 GHz, 150 ps (quantum dot-like) to 1300 nm, 35 GHz, < 25 ps (telecom standard). This nonlinear optical time lens achieves over 80% internal conversion efficiency and compresses output pulses below detector resolution. The device offers a compact solution for integrating quantum emitters, memories, and telecom networks, with potential for further pulse shape control.