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arXiv:1606.09372 · Journal of Physics B Atomic Molecular and Optical Physics

Competition between finite-size effects and dipole–dipole interactions in few-atom systems

François Damanet, John Martin

Published Oct 26, 2016• 13 citations
arXivHTMLPDF

Abstract

In this paper, we study the competition between finite-size effects (i.e. discernibility of particles) and dipole–dipole interactions in few-atom systems coupled to the electromagnetic field in vacuum. We consider two hallmarks of cooperative effects, superradiance and subradiance, and compute for each the rate of energy radiated by the atoms and the coherence of the atomic state during the time evolution. We adopt a statistical approach in order to extract the typical behaviour of the atomic dynamics and average over random atomic distributions in spherical containers with prescribed with k 0 the radiation wavenumber and R the average interatomic distance. Our approach allows us to highlight the tradeoff between finite-size effects and dipole–dipole interactions in superradiance/subradiance. In particular, we show the existence of an optimal value of for which the superradiant intensity and coherence pulses are the less affected by dephasing effects induced by dipole–dipole interactions and finite-size effects.

DOI
10.1088/0953-4075/49/22/225501

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Optics and Spectroscopy•Nov 1, 2011•3 citations
In this paper, we study the competition between finite-size effects (i.e. discernibility of particles) and dipole–dipole interactions in few-atom systems coupled to the electromagnetic field in vacuum. We consider two hallmarks of cooperative effects, superradiance and subradiance, and compute for each the rate of energy radiated by the atoms and the coherence of the atomic state during the time evolution. We adopt a statistical approach in order to extract the typical behaviour of the atomic dynamics and average over random atomic distributions in spherical containers with prescribed with k 0 the radiation wavenumber and R the average interatomic distance. Our approach allows us to highlight the tradeoff between finite-size effects and dipole–dipole interactions in superradiance/subradiance. In particular, we show the existence of an optimal value of for which the superradiant intensity and coherence pulses are the less affected by dephasing effects induced by dipole–dipole interactions and finite-size effects.
When atoms are coupled to a common electromagnetic environment, the exchange of photons through dipole-dipole interactions leads to the emergence of cooperative effects. As a particular example, superradiance arises from spontaneous emission when this exchange leads to constructive interference of the emitted photons. Here, we introduce an integrated method for studying cooperative radiation in many-body systems. This method, which allows to study extended systems with arbitrarily large number of particles, can be formulated by an effective, nonlinear, two-atom master equation that describes the dynamics using a closed form which treats single- and many-body terms on an equal footing. We apply this method to a homogeneous gas of initially inverted two-level atoms, and demonstrate the appearance of both superradiance and subradiance, identifying a many-body coherence term as the source of these cooperative effects. We describe the many-body induced broadening -- which is analytically found to scale with the optical depth of the system -- and light shifts, and distinguish spontaneous effects from induced ones. In addition, we theoretically predict the time-dependence of subradiance, and the phase change of the radiated field during the cooperative decay.
Decoherence, known as the consequence of the coupling of any quantum system to its environment, causes information loss in the system and represents a major problem in the physical realization of quantum computers [1]. Decoherence-Free States (DFS) are considered as a possible solution to this problem. A set of trapped cold atoms placed in a DFS state will be immune against decoherence due to spontaneous emission. However, because of dipole-dipole interactions between atoms, induced dephasing effects are likely to destroy the coherence and drive the system out of its DFS [1, 2]. In this work, we study numerically the dynamics of a set of two-level atoms initially in a DFS with respect to dissipative processes by solving the master equation including both dissipative dynamics and dipole dipole interactions. We fo- cus our attention on the infuence of dipolar coupling on the radiated energy rate and coherence of the system as in [3]. In particular, by averaging over many realizations of close randomly distributed atomic positions, we show the formation of a superradiant-like pulse and we study its properties as a function of the dipolar coupling strength. [1] D. A. Lidar & K. B. Whaley, Lectures Notes in Phys., Vol. 622, p83-120, Springer (2003). [2] M. Gross & S. Haroche, Physics reports 93, 301-396 (1982). [3] W. Feng, Y. Li & S-Y. Zhu, Phys. Rev. A 88, 033856 (2013).
We have developed a novel method to describe superradiance and related cooperative and collective effects in a closed form. Using the method we derive a two-atom master equation in which any complexity of atomic levels, semiclassical coupling fields and quantum fluctuations in the fields can be included, at least in principle. As an example, we consider the dynamics of an initially inverted two-level system and show how even such in a simple system phenomena such as the initial radiation burst or broadening due to dipole-dipole interactions occur, but it is also possible to estimate the population of the subradiant state during the radiative decay. Finally, we find that correlation only, not entanglement is responsible for superradiance.
We study effects of direct interatomic interaction on cooperative processes in atom-photon dynamics. Using a model of two-level atoms with Ising-type interaction as an example, it is demonstrated that interparticle interaction combined with atom-field coupling can introduce additional interatomic correlations acting as a phase synchronizing factor. For the case of weakly interacting atoms with $J<\ensuremath{\hbar}{\ensuremath{\omega}}_{0}$, where JJJ is the interparticle coupling constant and ${\ensuremath{\omega}}_{0}$ is the atomic frequency, dynamical regimes of cooperative relaxation of atoms are analyzed in the Born-Markov approximation both numerically and using the mean field approximation. We show that interparticle correlations induced by the direct interaction result in inhibition of incoherent spontaneous decay leading to the regime of collective pulse relaxation which differs from superradiance in nature. For superradiant transition, the synchronizing effect of interatomic interaction is found to manifest itself in enhancement of superradiance. When the interaction is strong and $J>\ensuremath{\hbar}{\ensuremath{\omega}}_{0}$, one-particle one-photon transitions are excluded and transition to the regime of multiphoton relaxation occurs. Using a simple model of two atoms in a high-QQQ single mode cavity we show that such transition is accompanied by Rabi oscillations involving many-atom multiphoton states. Dephasing effects of dipole-dipole interaction and solitonic mechanism of relaxation are discussed.
The collective scattering of light by a large number of coupled scatterers yields a rich many-body physics, yet treating such a problem in the quantum regime is a challenge.In this thesis, we consider a large atomic cloud in free space and driven by a monochromatic light, where the vacuum modes induce long-range dipole-dipole interactions.In order to study clouds of hundreds of particles, higher order correlation terms are neglected, keeping only quantum correlations between pair of atoms: this allows to reduce the number of degrees of freedom from 2 2N in the full quantum model to N 2 .Most of the works in the literature on dipole-dipole interactions have been performed in the linear optics limit, and our techniques allow to compare classical to beyond-semi-classical results.In particular, superradiance and subradiance have been reported in the decay dynamics of the cloud.Differently, by considering a system in the ground state and switching on the pump, we show that superradiance is also present in the Rabi oscillations at a rate obtained from using a single-dipole model for the radiated intensity.A frequency shift in the Rabi oscillations is also reported, which can be interpreted, in a linear dispersion theory, as a signature of a collective multimode vacuum Rabi splitting.While the classical dipoles model captures correctly the dynamics in the low-intensity regime, it fails for higher saturation, where semi-classical methods can be applied successfully.In particular, we observe a quantum subradiant decay in the intensity of the radiated field in the saturated regime.Furthermore, considering the decay dynamics starting from an initially strongly driven cloud, we observed that the states with n < N/2 excited atoms decays much slower than the ones with n > N/2: in other words, the upper part of the Dicke ladder is characterized by a superradiant emission, and the lower part by a subradiant one.Finally, investigating the fluorescence spectrum, we obtained quantum cooperative effects that modify the steady-state spectrum: additional sidebands at twice the Rabi frequency for the system driven at resonance and, out of resonance, an asymmetry in the peaks at the generalized Rabi frequency, and for all detection angles.We also present preliminary results of a sensor model that can capture the time evolution of the spectrum in the decay dynamics, a situation that the quantum regression theorem fails to describe.Several of these results were discussed in parallel with experimental data obtained by an experimental group of collaborators, and others aim to guide future experiments.
We study effects of direct interatomic interaction on cooperative processes in atom-photon dynamics. Using a model of two-level atoms with Ising-type interaction as an example, it is demonstrated that interparticle interaction can promote cooperative radiative relaxation. For small number of atoms this results in inhibition of incoherent spontaneous decay leading to the regime of collective pulse relaxation. Above superradiance threshold increase in delay time and enhancement of superradiance is occurred. In the case of strong interaction (as compared to excitation energy of an atom) transition to the regime of multiphoton relaxation occurs, which we discuss using a simple model of two atoms in a high-Q single mode cavity. It is shown that such transition is accompanied by Rabi oscillations involving many-atom multiphoton states. Dephasing effect of dipole-dipole interaction and solitonic mechanism of relaxation are discussed as well.