Quantum frequency conversion (QFC) of photonic signals preserves quantum information while simultaneously changing the signal wavelength. A common application of QFC is to translate the wavelength of a signal compatible with the current fiber-optic infrastructure to a shorter wavelength more compatible with high quality single-photon detectors and optical memories. Recent work has investigated the use of QFC to manipulate and measure specific temporal modes (TMs) through tailoring of the pump pulses. Such a scheme holds promise for multidimensional quantum state manipulation that is both low loss and re-programmable on a fast time scale. We demonstrate the first QFC temporal mode sorting system in a four-dimensional Hilbert space, achieving a conversion efficiency and mode separability as high as 92% and 0.84, respectively. A 20-GHz pulse train is projected onto 6 different TMs, including superposition states, and mode separability with weak coherent signals is verified via photon counting. Such ultrafast high-dimensional photonic signals could enable long-distance quantum communication with high rates.
Quantum frequency conversion (QFC) of photonic signals preserves quantum information while simultaneously changing the signal wavelength. A common application of QFC is to translate the wavelength of a signal compatible with the current fiber-optic infrastructure to a shorter wavelength more compatible with high quality single-photon detectors and optical memories. Recent work has investigated the use of QFC to manipulate and measure specific temporal modes (TMs) through tailoring of the pump pulses. Such a scheme holds promise for multidimensional quantum state manipulation that is both low loss and re-programmable on a fast time scale. We demonstrate the first QFC temporal mode sorting system in a four-dimensional Hilbert space, achieving a conversion efficiency and mode separability as high as 92% and 0.84, respectively. A 20-GHz pulse train is projected onto 6 different TMs, including superposition states, and mode separability with weak coherent signals is verified via photon counting. Such ultrafast high-dimensional photonic signals could enable long-distance quantum communication with high rates.
The temporal shape of single photons provides a high-dimensional basis of temporal modes, and can therefore support quantum computing schemes that go beyond the qubit. However, the lack of linear optical components to act as quantum gates has made it challenging to efficiently address specific temporal-mode components from an arbitrary superposition. Recent progress towards realizing such a "quantum pulse gate," has been proposed using nonlinear optical signal processing to add coherently the effect of multiple stages of quantum frequency conversion. This scheme, called temporal-mode interferometry [D. V. Reddy, Phys. Rev. A 91, 012323 (2015)], has been shown in the case of three-wave mixing to promise near-unity mode-sorting efficiency. Here we demonstrate that it is also possible to achieve high mode-sorting efficiency using four-wave mixing, if one pump pulse is long and the other short - a configuration we call asymmetrically-pumped Bragg scattering.
We experimentally demonstrate a programmable parametric mode sorter of high-dimensional signals in a composite spatiotemporal Hilbert space through mode-selective quantum frequency up-conversion. As a concrete example and with quantum communication applications in mind, we consider the Laguerre-Gaussian and Hermite-Gaussian modes as the spatial and temporal state basis for the signals, respectively. By modulating the spatiotemporal profiles of the up-conversion pump, we demonstrate the faithful selection of single photons in those modes and their superposition modes. Our results show an improvement in the quantum mode-sorting performance by coupling the up-converted light into a single-mode fiber and/or operating the upconversion at the edge of phase matching. By optimizing pump temporal profiles only, we achieve more than 12 dB extinction for mutually unbiased basis (MUB) sets of the spatiotemporal modes. This fully programmable and efficient system could serve as a viable resource for quantum communications, quantum computation, and quantum metrology.
Quantum frequency conversion (FC) in nonlinear optical media is a powerful tool for temporal-mode selective manipulation of light. Recent attempts at achieving high mode selectivities and/or fidelities have had to resort to multi-dimensional optimization schemes to determine the system's natural Schmidt modes. Certain combinations of relative-group velocities between the relevant frequency bands, medium length, and temporal pulse widths have been known to achieve good selectivities (exceeding 80%) for temporal modes that are nearly identical to pump pulse shapes, even for high conversion efficiencies. Working in this parameter regime using an off-the-shelf, second-harmonic generation, MgO:PPLN waveguide, and with pulses on the order of 500 fs at wavelengths around 800 nm, we verify experimentally that model-predicted Schmidt modes provide the high temporal-mode selectivity expected. The good agreement between experiment and theory paves the way to the implementation of a proposed two-stage FC scheme that is predicted by the present theory to reach near-perfect (100%) selectivity.
In high-dimensional quantum communication networks, the quantum frequency converter (QFC) is indispensable as an interface in the frequency domain. For example, many QFCs have been built to link atomic memories and fiber channels. However, almost all QFCs work in a two-dimensional space. It is still a pivotal challenge to construct a high-quality QFC for some complex quantum states, e.g., a high-dimensional single-photon state that refers to a qudit. Here, we firstly propose a high-dimensional QFC for an orbital-angular-momentum qudit via sum-frequency conversion with a flat-top beam pump. As a proof-of-principle demonstration, we realize quantum frequency conversions for a qudit from infrared to visible range. Based on the qudit quantum state tomography, the fidelities of a converted state are 98.29(95.02)%, 97.42(91.74)%, and 86.75(67.04)% for a qudit without (with) accidental counts in 2, 3, and 5 dimensions, respectively. The demonstration is very promising for constructing a high-capacity quantum communication network.
Long-distance quantum communication relies on storing and retrieving photonic qubits in orthogonal field modes. The available degrees of freedom for photons are polarization, spatial-mode profile, and temporal/spectral profile. To date, methods exist for decomposing, manipulating, and analyzing photons into orthogonal polarization modes and spatial modes. Here we propose and theoretically verify the first highly efficient method to carry out analogous operations for temporally and spectrally overlapping, but field-orthogonal, temporal modes. The method relies on cascaded nonlinear-optical quantum frequency conversion.
Signal photons emitted by quantum nodes typically fall outside the low-loss telecom window of optical fibers, leading to severe transmission losses. Quantum frequency conversion (QFC) offers an effective optical interface that bridges quantum nodes with telecom-band channels, enabling long-distance quantum communication. In this work, we demonstrate a compact, fiber-integrated QFC system with low noise and a high signal-to-noise ratio (SNR). Using a periodically poled lithium niobate (PPLN) waveguide, input photons at 637.2 nm are down-converted to telecom photons at 1588.3 nm. Our system achieves a total conversion efficiency of approximately 9%, with pump-induced noise suppressed to 154 Hz. For input photon rates of 32.7, 118.0, and 327.7 kHz, the corresponding SNRs are 12.3, 43.9, and 117.8, respectively. We further develop a theoretical model to simulate the entanglement fidelity between nitrogen-vacancy (NV) center spins and the frequency-converted telecom photons. At the emission rate of an NV center, our QFC system maintains an expected fidelity exceeding 52% over a transmission distance of 100 km. These findings highlight the potential of our QFC system for scalable, long-distance quantum networking.