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arXiv:1606.04105 · Physical review. B./Physical review. B

Electronic quasiparticles in the quantum dimer model: Density matrix renormalization group results

Junhyun Lee, Subir Sachdev A, Steven R. White

Published Sep 7, 2016• 15 citations
arXivHTMLPDF

Abstract

We study a recently proposed quantum dimer model for the pseudogap metal state of the cuprates. The model contains bosonic dimers, representing a spin-singlet valence bond between a pair of electrons, and fermionic dimers, representing a quasiparticle with spin-1/2 and charge $+e$. By density matrix renormalization group calculations on a long but finite cylinder, we obtain the ground-state density distribution of the fermionic dimers for a number of different total densities. From the Friedel oscillations at open boundaries, we deduce that the Fermi surface consists of small hole pockets near $(\ensuremath{\pi}/2,\ensuremath{\pi}/2)$, and this feature persists up to a doping density of 1/16. We also compute the entanglement entropy and find that it closely matches the sum of the entanglement entropies of a critical boson and a low density of free fermions. Our results support the existence of a fractionalized Fermi liquid in this model.

DOI
10.1103/physrevb.94.115112

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We study a recently proposed quantum dimer model for the pseudogap metal state of the cuprates. The model contains bosonic dimers, representing a spin-singlet valence bond between a pair of electrons, and fermionic dimers, representing a quasiparticle with spin-1/2 and charge +e+e+e. By density matrix renormalization group calculations on a long but finite cylinder, we obtain the ground-state density distribution of the fermionic dimers for a number of different total densities. From the Friedel oscillations at open boundaries, we deduce that the Fermi surface consists of small hole pockets near (\ensuremathπ/2,\ensuremathπ/2)(\ensuremath{\pi}/2,\ensuremath{\pi}/2)(\ensuremathπ/2,\ensuremathπ/2), and this feature persists up to a doping density of 1/16. We also compute the entanglement entropy and find that it closely matches the sum of the entanglement entropies of a critical boson and a low density of free fermions. Our results support the existence of a fractionalized Fermi liquid in this model.
We present an exact ground state solution of a quantum dimer model introduced by Punk, Allais, and Sachdev [Quantum dimer model for the pseudogap metal, Proc. Natl. Acad. Sci. U.S.A. 112, 9552 (2015).PNASA60027-842410.1073/pnas.1512206112], which features ordinary bosonic spin-singlet dimers as well as fermionic dimers that can be viewed as bound states of spinons and holons in a hole-doped resonating valence bond liquid. Interestingly, this model captures several essential properties of the metallic pseudogap phase in high-T_{c} cuprate superconductors. We identify a line in parameter space where the exact ground state wave functions can be constructed at an arbitrary density of fermionic dimers. At this exactly solvable line the ground state has a huge degeneracy, which can be interpreted as a flat band of fermionic excitations. Perturbing around the exactly solvable line, this degeneracy is lifted and the ground state is a fractionalized Fermi liquid with a small pocket Fermi surface in the low doping limit.
The Fermi liquid theory is a central concept in modern condensed matter physics used to describe conventional metals. A state of this universality class consists of well-defined quasiparticles, which occupy a finite number of states within a Fermi volume defined in momentum space. According to the Luttinger’s theorem, such a state encloses a Fermi volume proportional to the electron density modulo the filled bands if no symmetry is broken. In the past decades strong deviations from Fermi liquid theory have been observed in the scaling behavior of thermodynamic observables in different materials, among which are for instance cuprates and iron pnictides. This thesis is about two prototypical systems that can not be described by Fermi liquid theory. The first part of this work investigates two-dimensional effective models, which are in a Mott insulating state at half-filling and have a finite conductivity when doped with holes. In such a Mott insulating state, the charge carriers are strongly localized due to the Coulomb repulsion. Hence, strong correlations are assumed to have a strong impact on the formation of the ground state, also in the regime of small hole concentration. In a first project we have used a so-called spinon dopon mean-field theory to represent the two-dimensional Fermi-Hubbard model with strong on-site repulsive interaction in effective degrees of freedom, in which the holes can be embedded into a quantum spin liquid. The corresponding SU(2) invariant ground state belongs to the class of fractionalized Fermi liquids. In a second project we investigate a quantum dimer model, an effective model based on a Hilbert space spanned by short range singlets and bound states of holes and spins. The focus here is on the calculation of the hole-part of the electron spectral function by using exact diagonalization and its comparison with two analytic methods, a diagrammatic computation based on the Bethe-Salpeter equation and a so-called two-mode approximation. The electron spectral function shows a similar analytic form in momentum space between nodal and antinodal point when compared to results from photoemission spectroscopy experiments on cuprates. Furthermore, in a subsequent work we calculate the exact ground state of the quantum dimer model along a certain parameter line. In order to analyze the behavior of the elctron spectral function when increasing the density of holes, we investigate the Fermi-Hubbard model in a current project using a dynamical mean-field approach. To solve the 4-site cluster impurity problem, we use a numerical renormalization group approach. However, numerical limitations force us to restrict the analysis to spin-polarized baths. According to the spectral data, the system is similar to the SU(2) invariant case at half-filling in a Mott insulating state and posseses a momentum-selective energy gap at finite doping. The topology of the Fermi surface shows a Lifshitz transition when increasing the hole concentration. Here, the curvature of the Fermi surface changes from electron- to hole-like. For comparison we apply the dynamical mean-field theory also to the quantum dimer model and observe that the electron spectral functions at finite doping are qualitatively similar to that of the two-dimensional Fermi-Hubbard model. The second half of the work is about Tomonaga-Luttinger liquid theory, which is used to describe the low-energy effective degrees of freedom of one-dimensional systems. Here, we first discuss a conceptional extension of the operator-based bosonization theory for one-dimensional systems. This extension is especially suited for inhomogeneous one-dimensional systems. First, we investigate a one-dimensional system with a local interation potential and compute an exact solution of the single particle propagator at T = 0. The critical exponent of the single particle propagator has an unconventional form as a function of the microscopic Tomonaga-Luttinger parameters, which is not covered by the original Luttinger paradigm postulated by F. Duncan M. Haldane. In a second project on one-dimensional systems, we study the impact of scattering processes among bosonic low-energy excitations on the thermalization process. Such scattering processes are irrelevant on large length scales, however strongly affect the dynamics. In our analytic analysis we focus on a experimental setup, where a one-dimensional Bose gas is instantaneously splitted in two identical, however strongly correlated, halves of one-dimensional electronic systems. In the following, the corresponding non-equilibrium state runs through multiple regimes in time, such as a metastable prethermalization regime. However, above a certain threshold in time such scattering processes cause an effective thermalization of the system. In order to demonstrate this, we compute the kinetic equation in the Keldysh field integral formalism from a diagrammatic expansion based on a self-consistent Born approximation.
We present a slave-particle mean-field study of the mixed boson+fermion quantum dimer model introduced by Punk et al. [Proc. Natl. Acad. Sci. USA 112, 9552 (2015)] to describe the physics of the pseudogap phase in cuprate superconductors. Our analysis naturally leads to four charge eee fermion pockets whose total area is equal to the hole doping ppp for a range of parameters consistent with the $t\ensuremath{-}J$ model for high-temperature superconductivity. Here we find that the dimers are unstable to ddd-wave superconductivity at low temperatures. The region of the phase diagram with ddd-wave rather than sss-wave superconductivity matches well with the appearance of the four fermion pockets. In the superconducting regime, the dispersion contains eight Dirac cones along the diagonals of the Brillouin zone.
The pseudogap metal phase of hole-doped cuprates can be described by small Fermi surfaces of electronlike quasiparticles, which enclose a volume violating the Luttinger relation. This violation requires the existence of additional fractionalized excitations which can be viewed as fractionalized remnants of the paramagnon. We fractionalize the paramagnon into the bosonic spinons of the spin liquid described by the CP1{\mathbb{CP}}^{1}CP1 U(1) gauge theory, and we present a gauge theory of the bosonic spinons, a Higgs field, and an ancilla layer of fermions coupled to the original electrons. Along with the small Fermi surface pseudogap metal, this theory displays conventional phases: the large Fermi surface Fermi liquid with a low-energy paramagnon mode, and phases with spin density wave order. We describe the evolution of the electronic photoemission spectrum across these quantum phase transitions. We consider both the two-sublattice N\'eel and incommensurate spin density wave phases, and we find that the latter has spiral spin correlations.
Insulating quantum spin liquids can undergo a confinement transition to a valence bond solid via the condensation of topological excitations of the associated gauge theory. We extend the theory of such transitions to fractionalized Fermi liquids (FL*): These are metallic doped spin liquids in which the Fermi surfaces only have gauge neutral quasiparticles. Using insights from a duality transform on a doped quantum dimer model for the U(1)-FL* state, we show that projective symmetry group of the theory of the topological excitations remains unmodified, but the Fermi surfaces can lead to additional frustrating interactions. We propose a theory for the confinement transition of Z2{\mathbb{Z}}_{2}Z2​-FL* states via the condensation of visons. A variety of confining, incommensurate density wave states are possible, including some that are similar to the incommensurate ddd-form factor density wave order observed in several recent experiments on the cuprate superconductors.
Two of the iconic phases of the hole-doped cuprate materials are the intermediate temperature pseudogap metal and the lower temperature ddd-wave superconductor. Following the suggestion of P. W. Anderson, there were early theories of these phases as doped quantum spin liquids. However, these theories have had difficulties with two prominent observations: (i) angle-dependent magnetoresistance measurements (ADMR) in the pseudogap metal, including observation of the Yamaji effect, present convincing evidence of small hole pockets which can tunnel coherently between square lattice layers (Fang et al., Nature Physics 18, 558 (2022); Chan et al., Nature Physics 21, 1753 (2025)) and (ii) the velocities of the nodal Bogoliubov quasiparticles in the ddd-wave superconductor are highly anisotropic, with vF≫vΔv_F \gg v_ΔvF​≫vΔ​ (Chiao et al., Phys. Rev. B 62, 3554 (2000)). These notes review how the fractionalized Fermi Liquid (FL*) state, which dopes quantum spin liquids with gauge-neutral electron-like quasiparticles, resolves both difficulties. Theories of insulating quantum spin liquids employing fractionalization of the electron spin into bosonic or fermionic partons are discussed. Doping the bosonic parton theory leads to a holon metal theory: while not appropriate for the cuprate pseudogap, this theory is argued to apply to ultracold atom experiments on the Lieb lattice. Doping the fermionic parton theory leads to a ddd-wave superconductor with nearly isotropic quasiparticle velocities. The construction of the FL* state in a single band Hubbard-type model is described using a quantum dimer model, followed by a more realistic description using the Ancilla Layer Model (ALM), which is then used to obtain the theory of the pseudogap and the ddd-wave superconductor. The ALM also leads to a wavefunction for the FL* state of the Hubbard model, which agrees with ultracold atom observations.