Far-field interference of a neutron white beam and the applications to noninvasive phase-contrast imaging
Dmitry A. Pushin, Dusan Sarenac, Daniel Seth Hussey, Houxun Miao, M. Arif, David G. Cory, M. G. Huber, David L. Jacobson, Jacob Michael LaManna, Joseph Don Parker, T. Shinohara, Wakana Ueno, Han Wen
The phenomenon of interference plays a crucial role in the field of precision measurement science. Wave-particle duality has expanded the well-known interference effects of electromagnetic waves to massive particles. The majority of the wave-particle interference experiments require a near monochromatic beam which limits its applications due to the resulting low intensity. Here we demonstrate white beam interference in the far-field regime using a two-phase-grating neutron interferometer and its application to phase-contrast imaging. The functionality of this interferometer is based on the universal moir\'e effect that allows us to improve upon the standard Lau setup. Interference fringes were observed with monochromatic and polychromatic neutron beams for both continuous and pulsed beams. Far-field neutron interferometry allows for the full utilization of intense neutron sources for precision measurements of gradient fields. It also overcomes the alignment, stability, and fabrication challenges associated with the more familiar perfect-crystal neutron interferometer, as well as avoids the loss of intensity due to the absorption analyzer grating requirement in Talbot-Lau interferometer.
The phenomenon of interference plays a crucial role in the field of precision measurement science. Wave-particle duality has expanded the well-known interference effects of electromagnetic waves to massive particles. The majority of the wave-particle interference experiments require a near monochromatic beam which limits its applications due to the resulting low intensity. Here we demonstrate white beam interference in the far-field regime using a two-phase-grating neutron interferometer and its application to phase-contrast imaging. The functionality of this interferometer is based on the universal moir'e effect that allows us to improve upon the standard Lau setup. Interference fringes were observed with monochromatic and polychromatic neutron beams for both continuous and pulsed beams. Far-field neutron interferometry allows for the full utilization of intense neutron sources for precision measurements of gradient fields. It also overcomes the alignment, stability, and fabrication challenges associated with the more familiar perfect-crystal neutron interferometer, as well as avoids the loss of intensity due to the absorption analyzer grating requirement in Talbot-Lau interferometer.
Long-wavelength neutron interferometry using discrete optical elements is notoriously challenging due to stringent alignment and stability requirements. Here, we introduce a monolithic double-Laue neutron interferometer fabricated from a stack of commercial Bayfol HX photopolymer films. By recording holographic gratings simultaneously in multiple layers, we create a robust device that is inherently aligned, bypassing traditional stability problems. We demonstrate the device's function by observing the characteristic interference fringes in the diffracted intensity of both light and very cold neutrons. The interferometer is then used to perform in-situ characterization of the neutron beam's spectral profile, demonstrating its utility as a compact spectrometer. Our work establishes stacked holographic gratings as a simple, versatile, and powerful platform for matter-wave interferometry and metrology.
In the experiment described in this paper, a chopper serves as a source of neutron intensity pulses which pass through a perfect Si-crystal neutron interferometer (NI), where they are split coherently into two parts that recombine and interfere. As the occupation number of a single pulse is much smaller than unity, the results very clearly demonstrate the single-particle interference phenomena of neutron interferometry experiments. While traveling the pulses spread, with faster (slower) neutrons tending toward the leading (trailing) edge. The coherence length of the neutrons depends on the spectral width of their wavelength distribution. When a material with a neutron-nuclear optical potential is placed in one beam path in the NI, there is a loss of fringe visibility (contrast), which depends on the coherence length. By using time-of-flight techniques, we divide the pulse into time segments. Within a given time slice, the wavelength spectrum is narrower than in the pulse as a whole. As a result, contrast remains in the time slices even when it disappears in the overall pulse. We also observe an additional contrast modulation due to the overlap of neighboring pulses.
This thesis describes theoretical work carried out in connection with the high-mass matter-wave interference experiments at the University of Vienna. Its scope ranges from the simulation and analysis of experimental data to the proposal of a trapped interference scheme applicable to a variety of matter-wave platforms. The first main result of the thesis is the phase-space description of a near-field interferometer with any number of gratings. This theory is used to analyze a four-grating Talbot-Lau interferometer, in which passive compensation of low-frequency vibrations and of the Coriolis force are expected. The compensation is numerically confirmed and its effectiveness is compared to existing techniques. The second main result is the demonstration of Bragg diffraction of complex molecules on optical gratings, to which the author contributed the basic experimental design, simulations, and the interpretation of the data. This demonstration is a first step towards applying large momentum transfer coherent manipulation techniques to the interference of heavy molecules and clusters. The third main result is a new interference scheme for matter waves in toroidal confinement. The beam splitting and recombination in this scheme rely on the free evolution in the waveguide and require no interaction with the matter waves. The scheme is within reach of state-of-the-art experiments with Bose-Einstein condensates, where it could be used to measure weak atom-atom interactions or magnetic field gradients.
We examine how partial coherence and wavefront curvature of beams affect interference fringes behind diffraction gratings. We simulate (1) the Talbot effect, (2) far-field diffraction, (3) Mach-Zehnader interferometers, (4) Talbot-Lau interferometers, and (5) Lau interferometers using a numerically efficient expression. We show how interference fringes in each case depend on the beam's initial width, its coherence width (transverse coherence length), and its wavefront curvature in directions both parallel and perpendicular to the grating bars. The separation between gratings and the rotational alignment of the gratings about the optical axis are also considered. The formula used for our simulations is derived using the mutual intensity function of a Gaussian Schell-model beam.
We show our progress in setting up a three grating near-field Talbot-Lau interferometer (TLI) for large molecules such as C60. The TLI is the preferred tool for showing the wave nature of large particles, as it accepts beams of poor spatial coherence and because of its scaling properties with increasing mass of the particles. The spatial coherence is prepared by the first grating, it can be seen as an array of many collimation slits. Our setup is highly flexible in terms of the possibility of changing most of the parameters (such as distances between the gratings and grating angles) from the outside of the UHV-chamber. As the interferometer and the molecular beam source are place in separate vacuum chambers, refilling the oven and adjusting the setup parameters to different molecules is possible without opening the interferometer chamber. This is necessary, as the pressure in the interferometer chamber has to be lower than 5.10-7 mbar in order to observe high interference contrast. The TLI is highly sensitive to vibrations, especially in the range of 1 kHz (the inverse time-of-flight of the molecules through the interferometer), which makes vibration damping crucial for the success of observing interference. We observed vibration amplitudes of up to 75 nm at low frequencies (158 Hz). Compared to the inverse time-of-flight of the molecules, these vibrations are not 'seen' by the molecules and are non-critical. We observed interference of C60 with a contrast of 27 %, by scanning the self-image of the diffraction grating. In the present setup, an interference contrast of 60 % should be observed with perfect alignment of the gratings. Time-of-flight measurements showed small modulations of the velocity distribution at for interference expected distances of 2.5 ms. We also show the possibility of reconstructing the Wigner distribution function out of measurements for the case of Talbot interference under experimental conditions.
Abstract Among the various areas of neutron optical research, neutron interferometry has provided some of the most challenging and spectacular developments. In most cases, separated coherent beams are used which are produced either by wavefront division (Young’s type) or by amplitude division (Mach− Zehnder type). These beams are subsequently coherently superposed after passing through regions of space where the neutron wavefunction is modified in phase and amplitude by various interactions: nuclear, magnetic, electromagnetic, gravitational, or by geometry and topology (as in Aharonov−Bohm-type experiments). Various types of neutron interferometers that have been tested are shown in Fig. 2.1. The first neutron interferometer was based upon wavefront division and biprism deflection, but it had several constraints for interferometric applications mainly due to the small beam separation (100 μm) (Maier-Leibnitz and Springer 1962). Nevertheless, this method gained further interest for diffraction experiments from macroscopic objects and for the detection of weak interaction effects where the long flight paths (10 m) enhance the sensitivity for the measurements of these effects (Gähler et al. 1980; Klein et al. 1981a). The perfect-crystal interferometer (Rauch et al. 1974) provides widely separated coherent beams and has become a standard method for advanced neutron optical investigations. The development of diffraction and phase grating interferometers extended the Mach-Zehnder interferometer method to very slow neutrons (loffe et al. 1985; Gruber et al. 1989). The superposition of spin-up and spin-down states in the longitudinal direction provides the basis for Larmor and Ramsey interferometry, where no lateral beam splitting is necessary. The well-known spin-echo systems (Mezei 1972) and zero-field spin-echo systems (Gähler and Golub 1987; Dubbers et al. 1989) are examples of such interferometers, which also play an important role in atom interferometry (Bord é 1989; Kasevich and Chu 1991; Riehle et al. 1991).