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arXiv:1606.02219 · SpringerPlus

A translation invariant bipolaron in the Holstein model and superconductivity

Victor Dmitrievich Lakhno

Published Aug 8, 2016• 18 citations
arXivHTMLPDF

Abstract

Large-radius translation invariant (TI) bipolarons are considered in a one-dimensional Holstein molecular chain. Criteria of their stability are obtained. The energy of a translation invariant bipolaron is shown to be lower than that of a bipolaron with broken symmetry. The results obtained are applied to the problem of superconductivity in 1D-systems. It is shown that TI-bipolaron mechanism of Bose-Einstein condensation can support superconductivity even for infinite chain.

DOI
10.1186/s40064-016-2975-x

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Large-radius translation invariant (TI) bipolarons are considered in a one-dimensional Holstein molecular chain. Criteria of their stability are obtained. The energy of a translation invariant bipolaron is shown to be lower than that of a bipolaron with broken symmetry. The results obtained are applied to the problem of superconductivity in 1D-systems. It is shown that TI-bipolaron mechanism of Bose-Einstein condensation can support superconductivity even for infinite chain.
The properties of a Bose gas of translation-invariant (TI) bipolarons analogous to Cooper pairs are considered. As in the BCS theory, the description of a TI-bipolaron gas is based on the electron-phonon interaction and Froehlich Hamiltonian. As distinct from the BCS theory, when the correlation length greatly exceeds the mean distance between the pairs, here we deal with the opposite case when the correlation length is much less than the distance between the pairs. We calculate the critical temperature of the transition of a TI-bipolaron Bose-gas into the superconducting state, its energy, heat capacity and heat of the transition. The results obtained are used to explain the experiments on high-temperature superconductors. Possible ways of raising the critical temperature of high-temperature superconductors are discussed.
The monograph presents the theory of translation-invariant polarons and bipolarons based on the theory of squeezed vacuum wave functions. It is shown that the Tulub ansatz, which establishes a connection between the generalized Bogolyubov transformation with the unitary squeezed operator gives a solution to the spectral problem for a bipolaron. The solutions obtained are used to construct a theory of superconductivity based on the Froehlich Hamiltonian with a strong electron-phonon interaction. The role of Cooper pairs in it is played by TI bipolarons of spatially delocalized electrons with a small correlation length. The theory developed explains a large number of experiments on the thermodynamic, spectroscopic and transport characteristics of high-temperature superconductors, Josephson tunneling, angle-resolved photoemission spectroscopy, neutron scattering, etc. The book is intended for physicists and mathematicians who work in the field of the theory of condensed matter, as well as graduate students and senior students of universities.
Differences between translation-invariant and broken-symmetry bipolaron theories are analyzed in detail. It is shown that the Bogolyubov?Tyablikov canonical transformation allows collective coordinates to be introduced in a regular way for two particles in a quantum field and that for the case of the bipolaron the resulting electron?electron interaction in a phonon field depends on the electron coordinate difference alone. Predictions using a revised solution of the nonlinear differential equations for a bipolaron are given. It is shown that solving bipolaron equations numerically reduces the total bipolaron energies compared to known variational results.