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arXiv:1605.08417 · Physical review. B./Physical review. B

Emergence of XY-like phase in deformed spin- 32 AKLT systems

Ching-Yu Huang, Maximilian Anton Wagner, Tzu-Chieh Wei

Published Oct 14, 2016• 14 citations
arXivHTMLPDF

Abstract

Affleck, Kennedy, Lieb, and Taski (AKLT) constructed an exemplary spin-3/2 valence-bond solid (VBS) state on the hexagonal lattice, which is the ground state of an isotropic quantum antiferromagnet and possesses no spontaneous magnetization but finite correlation length. This is distinct from the N\'eel ordered state of the spin-3/2 Heisenberg model on the same lattice. Niggemann, Kl\"umper, and Zittartz then generalized the AKLT Hamiltonian to one family invariant under spin rotation about the $z$ axis. The ground states of this family can be parameterized by a single parameter that deforms the AKLT state, and this system exhibits a quantum phase transition between the VBS and N\'eel phases, as the parameter increases from the AKLT point to large anisotropy. We investigate the opposite regime when the parameter decreases from the AKLT point and find that there appears to be a Berezinskii-Kosterlitz-Thouless-like transition from the VBS phase to an XY phase. Such a transition also occurs in the deformation of other types of AKLT states with triplet-bond constructions on the same lattice. However, we do not find such an XY-like phase in the deformed AKLT models on other trivalent lattices, such as square-octagon, cross, and star lattices. On the star lattice, the deformed family of AKLT states remain in the same phase as the isotropic AKLT state throughout the whole region of the parameter. However, for two triplet-bond generalizations, the triplet VBS phase is sandwiched between two ferromagnetic phases (for large and small deformation parameters, respectively), which are characterized by spontaneous magnetizations along different axes. Along the way, we also discuss how various deformed AKLT states can be used for the purpose of universal quantum computation.

DOI
10.1103/physrevb.94.165130

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Affleck, Kennedy, Lieb, and Taski (AKLT) constructed an exemplary spin-3/2 valence-bond solid (VBS) state on the hexagonal lattice, which is the ground state of an isotropic quantum antiferromagnet and possesses no spontaneous magnetization but finite correlation length. This is distinct from the N'eel ordered state of the spin-3/2 Heisenberg model on the same lattice. Niggemann, Kl"umper, and Zittartz then generalized the AKLT Hamiltonian to one family invariant under spin rotation about the zzz axis. The ground states of this family can be parameterized by a single parameter that deforms the AKLT state, and this system exhibits a quantum phase transition between the VBS and N'eel phases, as the parameter increases from the AKLT point to large anisotropy. We investigate the opposite regime when the parameter decreases from the AKLT point and find that there appears to be a Berezinskii-Kosterlitz-Thouless-like transition from the VBS phase to an XY phase. Such a transition also occurs in the deformation of other types of AKLT states with triplet-bond constructions on the same lattice. However, we do not find such an XY-like phase in the deformed AKLT models on other trivalent lattices, such as square-octagon, cross, and star lattices. On the star lattice, the deformed family of AKLT states remain in the same phase as the isotropic AKLT state throughout the whole region of the parameter. However, for two triplet-bond generalizations, the triplet VBS phase is sandwiched between two ferromagnetic phases (for large and small deformation parameters, respectively), which are characterized by spontaneous magnetizations along different axes. Along the way, we also discuss how various deformed AKLT states can be used for the purpose of universal quantum computation.
We study spin-2 deformed-AKLT models on the square lattice, specifically a two-parameter family of O(2)O(2)O(2)-symmetric ground-state wave functions as defined by Niggemann, Kl\"umper, and Zittartz, who found previously that the phase diagram consists of a N\'eel-ordered phase and a disordered phase which contains the AKLT point. Using tensor-network methods, we not only confirm the N\'eel phase but also find an XY phase with quasi-long-range order and a region adjacent to it, within the AKLT phase, with very large correlation length, and investigate the consequences of a perfectly factorizable point at the corner of that phase.
We propose that a valence-bond-solid (VBS) order can be stabilized in certain two-dimensional antiferromagnets due to spin-lattice coupling. In contrast to the VBS state of the Affleck-Kennedy-Lieb-Tasaki (AKLT) type, the spin-lattice coupling-induced VBS state can occur when 2S2S2S is not an integer multiple of the coordination number zzz. S=2S=2S=2 spins on the triangular lattice with z=6z=6z=6 is discussed as an example. Within the Schwinger boson mean-field theory the ground state is derived as the direct product of states, one of which represents the conventional long-range ordered spins, and the other given by the $\sqrt{3}\ifmmode\times\else\texttimes\fi{}\sqrt{3}$ modulation of the valence bond amplitudes. Excitation spectrum for the modulated valence bond state is worked out within the single-mode approximation. The spectrum offers a new collective mode, distinct from the spin wave excitations of the magnetically ordered ground state, and observable in neutron scattering.
Abstract. We study the structure of quantum ground states of simplex solid models, which are generalizations of the valence bond construction for quantum antiferromagnets originally proposed by Affleck, Kennedy, Lieb, and Tasaki (AKLT) (1987 Phys. Rev. Lett . 59 799). Whereas the AKLT states are created by application of bond singlet operators for spins, the simplex solid construction is based on N -simplex singlet operators for spins. In both cases, a discrete one-parameter family of translationally-invariant models with exactly solvable ground states is defined on any regular lattice, and the equal time ground state correlations are given by the finite temperature correlations of an associated classical model on the same lattice, owing to the product form of the wave functions when expressed in a coherent state representation. We study these classical companion models via a mix of Monte Carlo simulations, mean-field arguments, and low-temperature effective field theories. Our analysis reveals that the ground states of edge- and face-sharing cubic lattice simplex solid models are long range ordered for sufficiently large values of the discrete parameter, whereas the ground states of the models on the kagome (2D) and hyperkagome (3D) lattices are always quantum disordered. The kagome simplex solid exhibits strong local order absent in its three-dimensional hyperkagome counterpart, a contrast that we rationalize with arguments similar to those leading to ‘order by disorder’.
The two-dimensional Affleck-Kennedy-Lieb-Tasaki (AKLT) model on a honeycomb lattice has been shown to be a universal resource for quantum computation. In this valence bond solid, however, the spin interactions involve higher powers of the Heisenberg coupling (S[over →](I)·S[over →](j))(n), making these states seemingly unrealistic on bipartite lattices, where one expects a simple antiferromagnetic order. We show that those interactions can be generated by orbital physics in multiorbital Mott insulators. We focus on t(2g) electrons on the honeycomb lattice and propose a physical realization of the spin-3/2 AKLT state. We find a phase transition from the AKLT to the Néel state on increasing Hund's rule coupling, which is confirmed by density matrix renormalization group simulations. An experimental signature of the AKLT state consists of protected, free S=1/2 spins on lattice vacancies, which may be detected in the spin susceptibility.
The qualitative difference in low-energy properties of spin S quantum antiferromagnetic chains with integer S and half-odd-integer S discovered by Haldane [F. D. M. Haldane, arXiv:1612.00076 (1981); Phys. Lett. A 93, 464–468 (1983); Phys. Rev. Lett. 50, 1153–1156 (1983)] and Tasaki [Tasaki, Graduate Texts in Physics (Springer, 2020)] can be intuitively understood in terms of the valence-bond picture proposed by Affleck et al. [I. Affleck, Phys. Rev. Lett. 59, 799 (1987); Commun. Math. Phys. 115, 477–528 (1988)]. Here, we develop a similarly intuitive diagrammatic explanation of the qualitative difference between chains with odd S and even S, which is at the heart of the theory of symmetry-protected topological (SPT) phases. (There is a 24 min video in which the essence of the present work is discussed: https://youtu.be/URsf9e_PLlc.) More precisely, we define one-parameter families of states, which we call the asymmetric valence-bond solid (VBS) states, that continuously interpolate between the Affleck–Kennedy–Lieb–Tasaki (AKLT) state and the trivial zero state in quantum spin chains with S = 1 and 2. The asymmetric VBS state is obtained by systematically modifying the AKLT state. It always has exponentially decaying truncated correlation functions and is a unique gapped ground state of a short-ranged Hamiltonian. We also observe that the asymmetric VBS state possesses the time-reversal, the Z2×Z2, and the bond-centered inversion symmetries for S = 2 but not for S = 1. This is consistent with the known fact that the AKLT model belongs to the trivial SPT phase if S = 2 and to a nontrivial SPT phase if S = 1. Although such interpolating families of disordered states were already known, our construction is unified and is based on a simple physical picture. It also extends to spin chains with general integer S and provides us with an intuitive explanation of the essential difference between models with odd and even spins.
The models constructed by Affleck, Kennedy, Lieb, and Tasaki (AKLT) [Phys. Rev. Lett. 59, 799 (1987)] describe a family of quantum antiferromagnets on arbitrary lattices, where the local spin SSS is an integer multiple MMM of half the lattice coordination number. The equal-time quantum correlations in their ground states may be computed as finite temperature correlations of a classical O(3)O(3)O(3) model on the same lattice, where the temperature is given by T=1/MT=1/MT=1/M. In dimensions d=1d=1d=1 and 2 this mapping implies that all AKLT states are quantum disordered. We consider AKLT states in d=3d=3d=3 where the nature of the AKLT states is now a question of detail depending upon the choice of lattice and spin; for sufficiently large SSS some form of N\'eel order is almost inevitable. On the unfrustrated cubic lattice, we find that all AKLT states are ordered, while for the unfrustrated diamond lattice the minimal S=2S=2S=2 state is disordered while all other states are ordered. On the frustrated pyrochlore lattice, we find (conservatively) that several states starting with the minimal S=3S=3S=3 state are disordered. The disordered AKLT models we report here are a significant addition to the catalog of magnetic Hamiltonians in d=3d=3d=3 with ground states known to lack order on account of strong quantum fluctuations.