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arXiv:1604.08882 · Physical review. B./Physical review. B

Detecting a preformed pair phase: Response to a pairing forcing field

Agnese Tagliavini, Massimo Capone, A. Toschi

Published Oct 10, 2016• 18 citations
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Abstract

The normal state of strongly coupled superconductors is characterized by the presence of ``preformed'' Cooper pairs well above the superconducting critical temperature. In this regime, the electrons are paired, but they lack the phase coherence necessary for superconductivity. The existence of preformed pairs implies the existence of a characteristic energy scale associated with a pseudogap. Preformed pairs are often invoked to interpret systems where some signatures of pairing are present without actual superconductivity, but an unambiguous theoretical characterization of a preformed-pair system is still lacking. To fill this gap, we consider the response to an external pairing field of an attractive Hubbard model, which hosts one of the cleanest realizations of a preformed pair phase, and a repulsive model where $s$-wave superconductivity cannot be realized. Using dynamical mean-field theory to study this response, we identify the characteristic features which distinguish the reaction of a preformed pair state from a normal metal without any precursor of pairing. The theoretical detection of preformed pairs is associated with the behavior of the second derivative of the order parameter with respect to the external field, as confirmed by analytic calculations in limiting cases. Our findings provide a solid test bed for the interpretation of state-of-the-art calculations for the normal state of the doped Hubbard model in terms of $d$-wave preformed pairs and, in perspective, of nonequilibrium experiments in high-temperature superconductors.

DOI
10.1103/physrevb.94.155114

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The normal state of strongly coupled superconductors is characterized by the presence of ``preformed'' Cooper pairs well above the superconducting critical temperature. In this regime, the electrons are paired, but they lack the phase coherence necessary for superconductivity. The existence of preformed pairs implies the existence of a characteristic energy scale associated with a pseudogap. Preformed pairs are often invoked to interpret systems where some signatures of pairing are present without actual superconductivity, but an unambiguous theoretical characterization of a preformed-pair system is still lacking. To fill this gap, we consider the response to an external pairing field of an attractive Hubbard model, which hosts one of the cleanest realizations of a preformed pair phase, and a repulsive model where sss-wave superconductivity cannot be realized. Using dynamical mean-field theory to study this response, we identify the characteristic features which distinguish the reaction of a preformed pair state from a normal metal without any precursor of pairing. The theoretical detection of preformed pairs is associated with the behavior of the second derivative of the order parameter with respect to the external field, as confirmed by analytic calculations in limiting cases. Our findings provide a solid test bed for the interpretation of state-of-the-art calculations for the normal state of the doped Hubbard model in terms of ddd-wave preformed pairs and, in perspective, of nonequilibrium experiments in high-temperature superconductors.
The finite-temperature phase diagram of the attractive Hubbard model is studied by means of the dynamical mean-field theory. We first consider the normal phase of the model by explicitly frustrating the superconducting ordering. In this case, we obtain a first-order pairing transition between a metallic phase and a paired phase formed by strongly coupled incoherent pairs. The transition line ends in a finite temperature critical point, but a crossover between two qualitatively different solutions still occurs at higher temperature. Comparing the superconducting- and the normal-phase solutions, we find that the superconducting instability always occurs before the pairing transition in the normal phase, i.e. T c > T pairing . Nevertheless, the high-temperature phase diagram at T > T c is still characterized by a crossover from a metallic phase to a preformed pair phase. We characterize this crossover by computing different observables that can be used to identify the pseudogap region, like the spin susceptibility, the specific heat and the single-particle spectral function.
We propose a scenario for superconductivity at strong electron-electron attractive interaction, in the case when the increase of the interaction strength promotes the nucleation of the local Cooper pairs and forms a state with a spatially phase incoherent Cooper pair order parameter. We show that this state can be characterized by a pseudogap which is determined by the electron scattering by phase fluctuations. At low temperatures, however, long-range correlations between the regions with different phases become important and establish global phase coherence and hence superconductivity in the system. We develop a mean-field theory to describe a phase transition between the preformed Cooper pair and superconducting states. This scenario of superconductivity applies not only to conductors with parabolic bands but also to the flat-band systems in which flat and dispersive bands coexist and are responsible for the formation of Cooper pairs as well as their phase synchronization.
We propose a scenario for superconductivity at strong electron-electron attractive interaction, in the case when the increase of the interaction strength promotes the nucleation of the local Cooper pairs and forms a state with a spatially phase incoherent Cooper pair order parameter. We show that this state can be characterized by a pseudogap which is determined by the electron scattering by phase fluctuations. At low temperatures, however, long-range correlations between the regions with different phases become important and establish global phase coherence and hence superconductivity in the system. We develop a mean-field theory to describe a phase transition between the preformed Cooper pair and superconducting states. This scenario of superconductivity applies not only to conductors with parabolic bands but also to the flat-band systems in which flat and dispersive bands coexist and are responsible for the formation of Cooper pairs as well as their phase synchronization.
A weak-coupling scenario wherein bosonic preformed electron pairs emerge upon cooling from two-electron correlations can explain the pseudogap phase consisting of segments where a Bogoliubov-like energy-momentum relation gapped spectrum alternates with a normal ungapped one. Bose–Einstein condensation (BEC) of preformed pairs interacting with the background fermions leads to either - or -wave-like superconducting gaps, the result being sensitive to the magnitude of the total number density of pairs at which BEC occurs and becomes possible already for a moderately anisotropic -wave pairing of fermions repelling each other via isotropic coulombic forces. The present model is compatible with the coexistence of pseudogap and of superconductivity phenomena.
This paper is a continuation and a partial summary of our analysis of the pairing at a quantum-critical point (QCP) in a metal for a set of quantum-critical systems, whose low-energy physics is described by an effective model with dynamical electron-electron interaction $V({\mathrm{\ensuremath{\Omega}}}_{m})=(\overline{g}/|{\mathrm{\ensuremath{\Omega}}}_{m}{|)}^{\ensuremath{\gamma}}$ (the $\ensuremath{\gamma}$ model). Examples include pairing at the onset of various spin and charge-density-wave and nematic orders and pairing in SYK-type models. In previous papers, we analyzed the physics for $\ensuremath{\gamma}<2$. We have shown that the onset temperature for the pairing Tp{T}_{p}Tp​ is finite, of order g‾\overline{g}g​, yet the gap equation at T=0T=0T=0 has an infinite set of solutions within the same spatial symmetry. As the consequence, the condensation energy Ec{E}_{c}Ec​ has an infinite number of minima. The spectrum of Ec{E}_{c}Ec​ is discrete, but becomes more dense as $\ensuremath{\gamma}$ increases. Here we consider the case $\ensuremath{\gamma}=2$. The $\ensuremath{\gamma}=2$ model attracted special interest in the past as it describes the pairing by an Einstein phonon in the limit when the dressed phonon mass ${\ensuremath{\omega}}_{D}$ vanishes. We show that for $\ensuremath{\gamma}=2$, the spectrum of Ec{E}_{c}Ec​ becomes continuous. We argue that the associated gapless ``longitudinal'' fluctuations destroy superconducting phase coherence at a finite TTT, such that at 0<T<Tp0<T<{T}_{p}0<T<Tp​, the system displays pseudogap behavior of preformed pairs. We show that for each gap function from the continuum spectrum, there is an infinite array of dynamical vortices in the upper half-plane of frequency. For the electron-phonon case, our results show that Tp=0.1827g‾{T}_{p}=0.1827\overline{g}Tp​=0.1827g​, obtained in earlier studies, marks the onset of the pseudogap behavior, while the actual superconducting Tc{T}_{c}Tc​ vanishes at ${\ensuremath{\omega}}_{D}\ensuremath{\rightarrow}0$.
The pseudogap state of cuprate high-temperature superconductors has been often viewed as either a yet unknown competing order or a precursor state to superconductivity. While awaiting the resolution of the pseudogap problem in cuprates, we demonstrate that local pairing fluctuations, vortex liquid dynamics, and other precursor phenomena can emerge quite generally whenever fermionic excitations remain gapped across the superconducting transition, regardless of the gap origin. Our choice of a tractable model is a lattice band insulator with short-range attractive interactions between fermions in the sss-wave channel. An effective crossover between Bardeen-Cooper-Schrieffer (BCS) and Bose-Einstein condensate (BEC) regimes can be identified in any band insulator above two dimensions, while in two dimensions only the BEC regime exists. The superconducting transition is ``unconventional'' (non-pair-breaking) in the BEC regime, identified by either the bosonic mean field or XY\mathit{XY}XY universality class. The insulator adjacent to the superconductor in the BEC regime is a bosonic Mott insulator of Cooper pairs, which may be susceptible to charge density wave ordering. We construct a function of the many-body excitation spectrum whose nonanalytic changes define a sharp distinction between band and Mott insulators. The corresponding ``second-order transition'' can be observed out of equilibrium by driving a Cooper pair laser in the Mott insulator. We explicitly show that the gap for charged bosonic excitations lies below the threshold for Cooper pair breakup in any BEC regime, despite quantum fluctuations. Our discussion ends with a view of possible consequences for cuprates, where antinodal pair dynamics has certain features in common with our simple sss-wave picture.