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arXiv:1602.00871 · Physical review. B./Physical review. B

Multiple particle-hole pair creation in the harmonically driven Fermi-Hubbard model

Nicolai ten Brinke, Manuel Ligges, U. Bovensiepen, Ralf Schützhold

Published May 10, 2017• 1 citation
arXivHTMLPDF

Abstract

We study the Fermi-Hubbard model in the strongly correlated Mott phase under the influence of a harmonically oscillating hopping rate $J(t)={J}_{0}+\mathrm{\ensuremath{\Delta}}Jcos(\ensuremath{\omega}t)$. Apart from the well-known fundamental resonance, where the frequency $\ensuremath{\omega}$ of this oscillation equals (or a little exceeds) the Mott gap, we also find higher-order resonances where multiple particle-hole pairs are created when $\ensuremath{\omega}$ is near an integer multiple of the gap. These findings should be relevant for experimental realizations such as ultracold fermionic atoms in optical lattices or pump-probe experiments using laser pulses incident on correlated electrons in solid-state materials.

DOI
10.1103/physrevb.95.195123

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We study the Fermi-Hubbard model in the strongly correlated Mott phase under the influence of a harmonically oscillating hopping rate J(t)=J0+\ensuremathΔJcos(\ensuremathωt)J(t)={J}_{0}+\mathrm{\ensuremath{\Delta}}Jcos(\ensuremath{\omega}t)J(t)=J0​+\ensuremathΔJcos(\ensuremathωt). Apart from the well-known fundamental resonance, where the frequency \ensuremathω\ensuremath{\omega}\ensuremathω of this oscillation equals (or a little exceeds) the Mott gap, we also find higher-order resonances where multiple particle-hole pairs are created when \ensuremathω\ensuremath{\omega}\ensuremathω is near an integer multiple of the gap. These findings should be relevant for experimental realizations such as ultracold fermionic atoms in optical lattices or pump-probe experiments using laser pulses incident on correlated electrons in solid-state materials.
Combining Floquet theory with the hierarchy of correlations (a method based on the formal expansion into inverse powers of the coordination number), we study the nonequilibrium dynamics of the Mott insulator state in the Fermi-Hubbard model under the influence of a harmonically oscillating electric field representing the pump laser. After deriving the associated Floquet exponents, we consider multiphoton resonances leading to the generation of higher harmonics. For weak electric field strengths, the strongest signal is obtained for the third harmonic when the driving frequency equals one-third of the Mott gap (because even harmonics are absent due to inversion symmetry). For stronger electric field strengths and lower driving frequencies, the higher-harmonic spectrum can also exhibit plateaulike structures extending over several harmonics (i.e., Floquet channels) below the resonance peak, which is consistent with previous findings.
Observing antiferromagnetic correlations in ultracold fermions on optical lattices is an important step towards quantum simulation of the repulsive Hubbard model. We show that optical lattice modulation spectroscopy can be used to detect antiferromagnetic order and probe the nature of quasiparticle excitations in a fermionic Mott insulator. At high temperatures, the rate of creation of double occupancies shows a broad peak at frequency of the on-site repulsion U, reflecting the incoherent nature of the hole excitations. At low temperatures, antiferromagnetic order leads to fine structure in the response consisting of a sharp absorption edge reflecting coherent propagation of holes and oscillations as a function of modulation frequency representing spin-wave shake-off processes.
Strongly correlated systems have rich and intriguing behaviors that have been at the focal point of modern condensed-matter physics. One promising research direction is the study of the Fermi-Hubbard model, which is thought to describe the essential physics of the cuprates and is naturally realized with ultracold atoms in optical lattices. The development of single-site control and readout on this platform has allowed for new methods in creating and studying states in the Fermi-Hubbard model. In this thesis, we discuss the engineering of low-entropy correlated states using a novel technique. By preparing a gapped band-insulator in the presence of an entropy reservoir, we create states with an entropy per particle of 0.016(3) k_B. We then demonstrate that the low-entropy band insulator can be used as a resource for creating strongly correlated states; by dynamically manipulating the on-site potentials we are able to convert the uncorrelated band insulator into a correlated Mott insulator. We also investigate if heating is responsible for the increase in entropy when creating the correlated phase and determine that it does not play a dominant role. In a separate experiment, we leverage the single-site manipulation capabilities in a different way by creating a single localized hole dopant in an antiferromagnetic state. We then allow the hole to delocalize by suddenly removing its pinning potential and study the resulting density and spin correlation evolution. As the hole delocalizes, we find that it displaces the surrounding spin correlations in a trajectory that is initially controlled by quantum interference. At later times, the hole delocalizes at a rate that scales with the spin exchange energy, revealing that the presence of magnetism fundamentally alters charge transport. These developments demonstrate continued progress in optical lattice quantum simulators and how they can play a role in unraveling the mysteries of the Fermi-Hubbard model.
Quantum tunneling is one of the most fundamental processes in nature. Single particle hopping of ultracold atoms in optical lattices changes its character dramatically when the ensemble is prepared in strongly correlated quantum phases due to atom-atom interactions. Correlated hopping in a Mott-insulating chain of bosons that is tilted to the Mott gap has recently been employed to study long-range order in the 1D transvers Ising model [1,2]. We study correlated tunneling dynamics for an ensemble of tilted 1D Mott chains after a sudden quench to the vicinity of the Ising paramagnetic to antiferromagnetic phase transition point [3]. The quench results in coherent oscillations for the orientation of effective Ising spins, detected via oscillations in the number of doubly occupied lattice sites. We characterize the quench by varying the system parameters. We report significant modification of the tunneling rate induced by interactions and show clear evidence for collective effects in the oscillatory response. We observe higher-order many-body tunneling processes over up to five lattice sites when the tilt per site is tuned to integer fractions of the Mott gap. Secondand third-order tunneling shows up in the transient response after the quench, from which we extract the characteristic scaling in accordance with perturbation theory and numerical simulations. In a second set of experiments we study the response of an ensemble of 1D superfluids in the Bose-Hubbard regime when subject to a tilt [4]. For large values of the tilt, we observe interaction-induced coherent decay and matter-wave quantum phase revivals of the Bloch oscillating ensemble. We analyze the revival period dependence on interactions by means of a Feshbach resonance. When reducing the value of the tilt, we observe the disappearance of the quasi-periodic phase revival signature towards an irreversible decay of Bloch oscillations, indicating the transition from regular to quantum chaotic dynamics.
This thesis presents quantum simulation of strongly-correlated systems beyond standard Hubbard models, using ultracold fermionic potassium atoms in both static and periodically-driven optical superlattices. For this study, we utilize a three-dimensional optical lattice setup, controlling particle interactions via magnetic Feshbach resonances and tunneling between lattice sites through optical lattice intensity. High-resolution absorption imaging combined with radio-frequency spectroscopy distinguishes between singly and doubly occupied sites. To enhance our systems capabilities beyond the standard Hubbard model, we extend the apparatus with an in-plane optical superlattice, creating a bi-chromatic structure by superposition of two optical lattices with commensurate lattice spacings. Using a phase locked loop with an environmental feed forward, we create an excellent phase stability of the superlattice exceeding 3 mrad. This precision allows us to explore both static and periodically-driven one-dimensional tight-binding models with strong interactions. We characterize the static superlattice through radio-frequency spectroscopy and Rabi oscillations, and validate the experimental data against theoretical calculations. In a tilted superlattice configuration, we successfully prepare and detect repulsively bound atom pairs, representing a highly excited eigenstate of the system. Furthermore, we demonstrate control over pair tunneling dynamics in a double-well potential using Floquet engineering, employing a low-noise periodic modulation of the optical superlattice tilt. Using an adiabatic band mapping technique, we directly observe the tunneling dynamics in the driven superlattice. We realize dynamic localization in quarter-filled wells and density-assisted tunneling up to the third harmonic order in half-filled wells. We observe a crossover from density-assited tunneling to dominant pair tunneling by tuning the effective interactions. Remarkably, the pair tunneling is not only enhanced relative to the suppressed single-particle tunneling but also exceeds the superexchange rate of a static double-well by more than a factor of two. This opens the possibility to study many-body systems with dominant pair tunneling, that extend beyond the standard Hubbard model.
The Fermi-Hubbard model is a key concept in condensed matter physics and provides crucial insights into electronic and magnetic properties of materials. Yet, the intricate nature of Fermi systems poses a barrier to answering important questions concerning d-wave superconductivity and quantum magnetism. Recently, it has become possible to experimentally realize the Fermi-Hubbard model using a fermionic quantum gas loaded into an optical lattice. In this atomic approach to the Fermi-Hubbard model, the Hamiltonian is a direct result of the optical lattice potential created by interfering laser fields and short-ranged ultracold collisions. It provides a route to simulate the physics of the Hamiltonian and to address open questions and novel challenges of the underlying many-body system. This review gives an overview of the current efforts in understanding and realizing experiments with fermionic atoms in optical lattices and discusses key experiments in the metallic, band-insulating, superfluid, and Mott-insulating regimes.