Strongly correlated systems have rich and intriguing behaviors that have been at the focal point of modern condensed-matter physics. One promising research direction is the study of the Fermi-Hubbard model, which is thought to describe the essential physics of the cuprates and is naturally realized with ultracold atoms in optical lattices. The development of single-site control and readout on this platform has allowed for new methods in creating and studying states in the Fermi-Hubbard model. In this thesis, we discuss the engineering of low-entropy correlated states using a novel technique. By preparing a gapped band-insulator in the presence of an entropy reservoir, we create states with an entropy per particle of 0.016(3) k_B. We then demonstrate that the low-entropy band insulator can be used as a resource for creating strongly correlated states; by dynamically manipulating the on-site potentials we are able to convert the uncorrelated band insulator into a correlated Mott insulator. We also investigate if heating is responsible for the increase in entropy when creating the correlated phase and determine that it does not play a dominant role. In a separate experiment, we leverage the single-site manipulation capabilities in a different way by creating a single localized hole dopant in an antiferromagnetic state. We then allow the hole to delocalize by suddenly removing its pinning potential and study the resulting density and spin correlation evolution. As the hole delocalizes, we find that it displaces the surrounding spin correlations in a trajectory that is initially controlled by quantum interference. At later times, the hole delocalizes at a rate that scales with the spin exchange energy, revealing that the presence of magnetism fundamentally alters charge transport. These developments demonstrate continued progress in optical lattice quantum simulators and how they can play a role in unraveling the mysteries of the Fermi-Hubbard model.
Strongly correlated systems have rich and intriguing behaviors that have been at the focal point of modern condensed-matter physics. One promising research direction is the study of the Fermi-Hubbard model, which is thought to describe the essential physics of the cuprates and is naturally realized with ultracold atoms in optical lattices. The development of single-site control and readout on this platform has allowed for new methods in creating and studying states in the Fermi-Hubbard model. In this thesis, we discuss the engineering of low-entropy correlated states using a novel technique. By preparing a gapped band-insulator in the presence of an entropy reservoir, we create states with an entropy per particle of 0.016(3) k_B. We then demonstrate that the low-entropy band insulator can be used as a resource for creating strongly correlated states; by dynamically manipulating the on-site potentials we are able to convert the uncorrelated band insulator into a correlated Mott insulator. We also investigate if heating is responsible for the increase in entropy when creating the correlated phase and determine that it does not play a dominant role. In a separate experiment, we leverage the single-site manipulation capabilities in a different way by creating a single localized hole dopant in an antiferromagnetic state. We then allow the hole to delocalize by suddenly removing its pinning potential and study the resulting density and spin correlation evolution. As the hole delocalizes, we find that it displaces the surrounding spin correlations in a trajectory that is initially controlled by quantum interference. At later times, the hole delocalizes at a rate that scales with the spin exchange energy, revealing that the presence of magnetism fundamentally alters charge transport. These developments demonstrate continued progress in optical lattice quantum simulators and how they can play a role in unraveling the mysteries of the Fermi-Hubbard model.
Analog quantum simulation provides a unique toolkit to investigate quantum many-body problems of whose solutions may be incredibly challenging. In particular, using ultracold fermionic atoms in optical lattices it realizes the Fermi Hubbard model, which is a fundamental model in condensed matter physics exhibiting properties relevant to many intriguing strongly-correlated systems. However, most quantum simulators of the Hubbard model have so far restricted to the square geometries. In addition, access to low temperatures where the exotic quantum phases are predicted to develop has still remained elusive. In this thesis, we engineer a novel optical lattice with dynamically tunable geometries and significantly reduced technical noises. We extend for the first time the study of quantum magnetism into the exotic phases in a Fermi Hubbard system with tunable geometric frustration. As we continuously tune our system from a square to a triangular lattice geometry, we observe a transition from a Néel antiferromagnet to a 120-degree spin spiral state. We then study, again for the first time, how doping affects a frustrated quantum magnet. To our surprise, we found an emergent ferromagnetic state with strong particle doping, which is absent on the hole-doped side and is in stark contrast with the particle-hole symmetric doping dependence in a square lattice. To shed light on the role of itinerant dopants in the emergence of these new magnetic properties, we furthermore leverage the unique single-particle resolution capabilities of our platform to probe higher-order density and spin correlations. These measurements hint at a new type of magnetism induced by kinetic frustration, which manifests as local antiferromagnetic correlations around hole dopants and and ferromagnetic correlations around particle dopants. Unlike magnetism induced by exchange or superexchange interactions, the energy associated with this mechanism is the kinetic energy, closely related to the famous rigorous results by Nagaoka. Furthermore, the dynamical tunability of the lattice allows adibatic engineering of quantum states in optical lattices. We discuss the preliminery efforts to prepare strongly-correlated states with significantly reduced temperatures, which may pave the way towards low temperature states in the Hubbard model.
Accessing new regimes in quantum simulation requires the development of new techniques for quantum state preparation. We demonstrate the quantum state engineering of a strongly correlated many-body state of the two-component repulsive Fermi-Hubbard model on a square lattice. Our scheme makes use of an ultralow entropy doublon band insulator created through entropy redistribution. After isolating the band insulator, we change the underlying potential to expand it into a half-filled system. The final many-body state realized shows strong antiferromagnetic correlations and a temperature below the exchange energy. We observe an increase in entropy, which we find is likely caused by the many-body physics in the last step of the scheme. This technique is promising for low-temperature studies of cold-atom-based lattice models.
Obtaining a microscopic understanding of the dynamics in strongly correlated electronic systems has remained a challenge for many decades. The interplay between the spin and charge degrees of freedom in these materials at different temperatures and dopant concentrations is not well understood and is still an area of intense scientific research. Recently, quantum simulators based on ultracold atoms in optical lattices have emerged as a promising platform to probe strongly correlated fermionic systems. This thesis reports on the work carried out with a quantum gas microscope of ultracold fermionic Li-6, where Fermi-Hubbard systems are prepared and imaged with single site spin and density resolution. The main results of the thesis explore the microscopic dynamics underlying one-dimensional materials, where individual constituents such as the electron with charge e and spin-1/2 are not relevant to the description of the system anymore and are instead replaced by spin and charge excitations that can propagate independent of one another - a phenomenon called spin-charge separation. In our quantum simulator, we use analogous one-dimensional Fermi-Hubbard chains of Li-6, to perform time- and space-resolved microscopy of the spin and charge excitations following a local quench. By extracting their strikingly different velocities and showing an absence of binding between the excitations, we demonstrate spin-charge separation. Our microscopic technique also allows us to quantitatively extract the excess spin carried by the spin excitiation, connecting our results to the phenomenon of fractionalization. In another set of experiments, Fermi-Hubbard chains are probed at equilibrium and incommensurate spin correlations arising in the presence of both density doping and spin polarization are observed. The wavevector of these incommensurate correlations are found to have a linear dependence on doping and polarization. Finally, the effect of the spin-charge interplay is probed in the crossover from one to two dimensions. The spin correlations across dopants are seen to be dramatically different in two dimensions, and the strong antiferromagnetic correlations across dopants present in one dimension disappear. For a single dopant in a fully two dimensional system, the spin-charge interplay manifests as a distorted spin cloud surrounding the dopant, indicating the formation of a magnetic polaron. The experiments reported here demonstrate the power of a quantum simulator; by probing the physics of strongly correlated systems in real space with unprecedented resolution, we can zoom into emergent phenomena, validate theories and access regimes that are not possible in other experimental settings.
This thesis reports on new experimental techniques for the study of strongly correlated states of ultracold atoms in optical lattices. We used a high numerical aperture imaging system to probe 87Rb atoms in a two-dimensional lattice with single-site resolution. Fluorescence imaging allows to detect single atoms with a large signal to noise ratio and to reconstruct the atom distribution on the lattice. We applied this new technique to a two-dimensional Mott insulator and directly observed number squeezing and the emerging shell structure. A comparison of the radial density and variance distributions to theory provides a precise in situ temperature and entropy measurement from single images. We find entropies around the critical value for quantum magnetism. In a second series of experiments, we demonstrated two-dimensional single-site spin control in the optical lattice. The differential light shift of a tightly focused laser beam shifts selected atoms into resonance with a microwave field driving a spin flip. In this way, we reach sub-diffraction limited spatial resolution well below the lattice spacing. Starting from a Mott insulator with unity filling we were able to create arbitrary spin patterns. We used this ability to prepare atom distributions to study one-dimensional single-particle tunneling dynamics in a lattice. By discriminating the dynamics of the ground state and of the first excited band, we find that our addressing scheme leaves most atoms in the vibrational ground state. Moreover, we studied coherent light scattering from the atoms in the optical lattice and found diffraction maxima in the far-field. We showed that an antiferromagnetic order leads to additional diffraction peaks which can be used to detect this order also when single-site resolution is not available. The new techniques described in this thesis open the path to a wide range of novel applications from quantum dynamics of spin impurities, entropy transport, implementation of novel cooling schemes, and engineering of quantum many-body phases to quantum information processing.
Studying the low-temperature phases of doped Hubbard models, including the emergence of collective order and exotic normal phases, is at the heart of strongly correlated physics. This thesis offers new theoretical insights into the low-energy physics of doped Hubbard models, with a particular emphasis on leveraging quantum simulation as a powerful investigative tool. We explore the emergence of collective order driven by many-body interactions, by predicting and observing stripe-like structures in quantum gas microscopes of engineered Hamiltonians. These fluctuating stripe patterns are developed into a theoretical framework for the pseudogap— a highly enigmatic phase in hole-doped cuprates—where we show how fluctuating domain walls yield effective toric code descriptions. Ultracold atoms in optical lattices provide a unique platform for directly probing and testing this theory. We further investigate unconventional bilayer nickelate superconductors, predicting an exceptionally stable superfluid state in a single-band Hubbard model at experimentally accessible temperatures. By proposing schemes to observe coherent pair-pair correlations, this advances the long-standing goal of realizing and observing long-range superconducting order in ultracold atomic systems in optical lattices. On non-bipartite lattices, we examine kinetic magnetism in Hubbard models and moiré heterostructures. Additionally, the low-temperature regime of doped Hubbard models with enhanced symmetries is analyzed, revealing exotic phenomena such as sub-dimensional polaronic particles. We develop machine learning techniques to extract key physical insights from many-body snapshots, offering a new avenue for understanding intricate quantum phases. Finally, we go beyond the Fermi-Hubbard paradigm and show how non-local strongly correlated models can be leveraged to address classical optimization problems through quantum annealing.
Exotic phenomena in strongly correlated electron systems emerge from the interplay between spin and motional degrees of freedom. For example, doping an antiferromagnet is expected to give rise to pseudogap states and high-temperature superconductors. Quantum simulation with ultracold fermions in optical lattices offers the potential to answer open questions about the doped Hubbard Hamiltonian, and has recently been advanced by quantum gas microscopy. In order to take advantage of these possibilities, a stable, high-power, 2D square lattice system was developed and coupled with an image plane based spatial light modulator. The ability to finely tune the atomic potential has made it possible to realize an antiferromagnet in a repulsively interacting Fermi gas on a 2D square lattice. At our lowest temperatures of T/t=0.25(2), antiferromagnetic long-range order (LRO) manifests through the divergence of the correlation length that reaches the size of the system, the development of a peak in the spin structure factor and a value of the staggered magnetization approaching the ground state value. Similarly, by carefully shaping the confinement, we have produced ultra-low entropy band insulators, which promise to be a perfect starting point for more advanced cooling schemes. In addition to the production of new states, Fermi gas microscopy is superbly well suited to studies of many-body dynamics. To this end I report on preliminary measurements of the propagation of holes in a Mott insualtor. These results demonstrate that Fermi gas microscopy can address open questions on the low-temperature Hubbard model.