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arXiv:1601.03344 · Applied Physics Letters

Tunable open-access microcavities for on-chip cavity quantum electrodynamics

C. A. Potts, A. Melnyk, H. Ramp, M. H. Bitarafan, D. Vick, L. J. LeBlanc, J. P. Davis, R. G. DeCorby

Published Jan 25, 2016• 21 citations
arXivHTMLPDF

Abstract

We report on the development of on-chip microcavities and show their potential as a platform for cavity quantum electrodynamics experiments. Microcavity arrays were formed by the controlled buckling of SiO2/Ta2O5 Bragg mirrors and exhibit a reflectance-limited finesse of 3500 and mode volumes as small as 35λ3. We show that the cavity resonance can be thermally tuned into alignment with the D2 transition of 87Rb and outline two methods for providing atom access to the cavity. Owing to their small mode volume and high finesse, these cavities exhibit single-atom cooperativities as high as C1=65. A unique feature of the buckled-dome architecture is that the strong-coupling parameter g0/κ is nearly independent of the cavity size. Furthermore, strong coupling should be achievable with only modest improvements in mirror reflectance, suggesting that these monolithic devices could provide a robust and scalable solution to the engineering of light-matter interfaces.

DOI
10.1063/1.4940715

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•Jan 1, 2015•0 citations
We report on the development of on-chip microcavities and show their potential as a platform for cavity quantum electrodynamics experiments. Microcavity arrays were formed by the controlled buckling of SiO2/Ta2O5 Bragg mirrors and exhibit a reflectance-limited finesse of 3500 and mode volumes as small as 35λ3. We show that the cavity resonance can be thermally tuned into alignment with the D2 transition of 87Rb and outline two methods for providing atom access to the cavity. Owing to their small mode volume and high finesse, these cavities exhibit single-atom cooperativities as high as C1=65. A unique feature of the buckled-dome architecture is that the strong-coupling parameter g0/κ is nearly independent of the cavity size. Furthermore, strong coupling should be achievable with only modest improvements in mirror reflectance, suggesting that these monolithic devices could provide a robust and scalable solution to the engineering of light-matter interfaces.
This thesis reports on the development of an array of plane-concave Fabry-Perot microcavities containing atoms (or other quantum emitters), interconnected by UV-written waveguides on a silica-on-silicon chip. The microcavities are formed by a mirror coated on the end facet of the chip and an array of spherical micromirrors etched on silicon. This is to our knowledge the first attempt at implementing the emerging coupled-cavities QED paradigm. The device we propose possesses a degree of control, flexibility and tuning unmatched in other suggested implementations: The atoms can be manipulated inside the cavity by auxiliary lasers and the cavity-cavity coupling rate as well as the atom-cavity coupling can be tuned. It is highly scalable. Calculation of the complete (classical) optical spectrum of the device is presented. The quantum dynamics that may eventually be observed has also been studied. Waveguide chips containing couplers and phase shifter have been fabricated. We have successfully demonstrated the operation of the elementary sub-systems: the strong optical coupling between a microcavity and a waveguide resonator, and the tunable strong coupling between two evanescently coupled waveguide resonators. No experiments with atoms or other quantum emitters were attempted, because the waveguide propagation loss is so large that no quantum physics can be observed. There is hope that this can be overcome in the future by using other waveguide technologies.
Neutral-atom array and cavity quantum electrodynamics offer complementary strengths for quantum science: scalable, reconfigurable qubit architectures and strong coherent light-matter coupling. Combining them in a single platform requires an optical cavity with simultaneously high cooperativity, sufficient mode volume to accommodate atom array, and ample side optical access for atom trapping, imaging, cooling, and rearrangement, a combination that is challenging to achieve. Here we realize an atomic array integrated with a millimeter-scale Fabry--Pérot cavity whose optically-characterized single-atom cooperativity reaches ηcav=125±13η_{\mathrm{cav}}=125\pm13ηcav​=125±13. Atom-cavity transmission spectra of trapped atoms yield an effective spectroscopic cooperativity ηspec=106±3η_{\mathrm{spec}}=106\pm 3ηspec​=106±3, providing an in-situ verification of strong coupling in the integrated platform. In this integrated system, we achieve a state-measurement fidelity of 99.925−18+15%99.925^{+15}_{-18}\%99.925−18+15​% for a single atom with a 4-μμμs readout time. We also demonstrate simultaneous coupling of up to 21 individually trapped atoms to the antinode of the cavity mode. The key technical advance is a two-step mirror-fabrication method combining precision mechanical shaping and carbon-dioxide laser polishing, which produces concave fused-silica mirrors with sub-millimeter radii of curvature and residual roughness below 2 A˚2~Å2 A˚. Our results establish a regime of cavity-integrated atomic array that simultaneously provides high cooperativity, large mode volume, and flexible manipulation of individual atoms, opening opportunities for cavity-assisted quantum state readout and long-range entanglement-engineering in atom-array platforms.
Open-access microcavities are a powerful tool to enhance light–matter interactions for solid-state quantum and nanosystems and are key to advance applications in quantum technologies. For this purpose, the cavities should simultaneously meet two conflicting requirements—full tunability to cope with spatial and spectral inhomogeneities of a material and highest stability under operation in a cryogenic environment to maintain resonance conditions. To tackle this challenge, we have developed a fully tunable, open-access, fiber-based Fabry–Pérot microcavity platform that can be operated under increased noise levels in a closed-cycle cryostat. It comprises custom-designed monolithic micro- and nanopositioning elements with up to mm-scale travel range that achieve a passive cavity length stability at low temperature of only 15 pm rms in a closed-cycle cryostat and 5 pm in a more quiet flow cryostat. This can be further improved by active stabilization, and even higher stability is obtained under direct mechanical contact between the cavity mirrors, yielding 0.8 pm rms during the quiet phase of the closed-cycle cryocooler. The platform provides the operation of cryogenic cavities with high finesse and small mode volume for strong enhancement of light–matter interactions, opening up novel possibilities for experiments with a great variety of quantum and nanomaterials.
Open microcavities provide a powerful platform for studying cavity quantum electrodynamics in solid-state systems. However, operating open microcavities at cryogenic temperatures, as required for many solid-state quantum emitters, typically demands bulky and cryostat-specific vibration-mitigation setups. Here we report a compact, robust, and tunable mechanical host for an open microcavity. The complete mechanical assembly fits within a footprint of 1′′×1′′×0.5′′1'' \times 1'' \times 0.5''1′′×1′′×0.5′′. Using this mechanical host, we observe no vibration-induced cavity broadening for an open microcavity with finesse exceeding 1,000 without cryostat customization or active locking. The assembly also enables in situ tuning of the cavity resonance over 3 nm, and the resonance of the same cavity remains within this range across multiple cooldowns. To further showcase the capability of this assembly, we demonstrate coupling between an InGaAs quantum dot and an open microcavity with a cooperativity exceeding unity. This platform provides a versatile testbed for fundamental cavity quantum electrodynamics and a scalable route to portable quantum light sources and spin-photon interfaces for quantum repeaters, quantum networks, and photonic quantum computing.
The interaction of light with matter is at the heart of quantum optics, which itself enables insight into the fundamental aspects of quantum mechanics. First experimental access to this research field has been realized by coupling atoms to light. Here, the transition between discrete energy states of the atom is associated with the absorption and emission of a photon, a single quantum of the electromagnetic field. As a central aspect of quantum optics, the light-emitter interaction can be significantly enhanced by placing the emitter in optical cavity that is on resonance with the emitter. In recent years, this has led to a rapidly evolving research field known as cavity quantum electrodynamics (CQED). In CQED two different regimes are distinguished: the strong and the weak coupling regimes. In the strong coupling regime, the emitted photon is reflected from the cavity mirrors and eventually reabsorbed by the emitter. In contrast, the weak coupling regime describes the irreversible emission, where the photon leaks out of the cavity before it can be reabsorbed. Both the weak and strong coupling regimes enabled fundamental experiments for a better understanding of quantum optical phenomena. \n \n \n \nCQED grants access to the quantum world and hence offers potentially revolutionizing applications, particularly in the field of quantum information processing. A central aspect for the successful implementation of quantum applications is the system's scalability. Unfortunately, placing atoms deterministically inside a cavity remains technologically elaborate and hence minimizes the prospect of scaling a atom-CQED system. \n \nA possibility to address this issue is to implement CQED in the solid state, where sophisticated fabrication strategies allow miniaturization and scalability of the system. Particularly the development of self-assembled quantum dots (QD) in semiconductors represent a promising route. QDs can be considered as artificial atoms that mimic the atomic two-level system. These structures interact strongly with light and therefore have the potential for replacing atoms in CQED. As a central advantage, QDs are naturally trapped, which greatly simplifies the deterministic incorporation into the cavity. \n \nIn recent years, many efforts have been made to couple self-assembled QDs to microcavities. Generally, the successful implementation of CQED requires a cavity with a high quality factor Q and a low mode volume. In a majority of the approaches, the high Q/small mode volume cavities were monolithically defined around the QD, embedding the QD at a fixed position inside the cavity. Both the weak and strong coupling regimes have been reached with these systems. However, for future applications they suffer from several disadvantages. The fixed position of the QD inside the cavity minimizes the prospects for spectral tunability and spatial positioning the QD inside the cavity. Furthermore, prospects for further increasing of the cavity Q-factor and minimization of the mode volume remain limited in these systems. \n \nIn this thesis the mentioned disadvantages are addressed by developing a fully tunable miniaturized Fabry-Pérot microcavity with low mode volume. The design enables both spatial positioning of the emitter inside the cavity and spectral tunability. Successful coupling of a single QD to the microcavity is demonstrated including the strong coupling regime. Further a new approach to decrease the cavity mode volume is presented, where we demonstrate weak coupling is achieved