Abstract The properties of ultracold quantum gases of bosons with dipole–dipole interaction are investigated at finite temperature in the frame of representative ensembles theory. Self-consistent coupled equations of motion are derived for the condensate and the non-condensate components. Corrections due to the dipolar interaction to condensate depletion, the anomalous density and thermodynamic quantities such as the ground state energy, the equation of state, the compressibility and the presure are calculated in the homogeneous case at both zero and finite temperatures. Effects of interaction and temperature on the structure factor are also discussed. Within the realm of the local density approximation, we generalize our results to the case of a trapped dipolar gas.
Abstract The properties of ultracold quantum gases of bosons with dipole–dipole interaction are investigated at finite temperature in the frame of representative ensembles theory. Self-consistent coupled equations of motion are derived for the condensate and the non-condensate components. Corrections due to the dipolar interaction to condensate depletion, the anomalous density and thermodynamic quantities such as the ground state energy, the equation of state, the compressibility and the presure are calculated in the homogeneous case at both zero and finite temperatures. Effects of interaction and temperature on the structure factor are also discussed. Within the realm of the local density approximation, we generalize our results to the case of a trapped dipolar gas.
We present a systematic study of dilute three-dimensional dipolar Bose gas employing a finite temperature perturbation theory (beyond the mean field). We analyze in particular the behavior of the anomalous density, we find that this quantity has a finite value in the limit of weak interactions at both zero and finite temperatures. We show that the presence of the dipole–dipole interaction enhances fluctuations, the second order correlation function and thermodynamic quantities such as the chemical potential, the ground state energy, the compressibility and the superfluid fraction. We identify the validity criterion of the small parameter of the theory for Bose-condensed dipolar gases.
We theoretically investigate various beyond mean-field effects on Bose gases at zero temperature featuring the anisotropic and long-range dipole-dipole interaction in addition to the isotropic and short-range contact interaction. Within the realm of the Bogoliubov--de Gennes theory, we consider static properties and low-lying excitations of both homogeneous and harmonically trapped dipolar bosonic gases. For the homogeneous system, the condensate depletion, the ground-state energy, the equation of state, and the speed of sound are discussed in detail. Making use of the local density approximation, we extend these results in order to study the properties of a dipolar Bose gas in a harmonic trap and in the regime of large particle numbers. After deriving the equations of motion for the general case of a triaxial trap, we analyze the influence of quantum fluctuations on important properties of the gas, such as the equilibrium configuration and the low-lying excitations in the case of a cylinder-symmetric trap. In addition to the monopole and quadrupole oscillation modes, we also discuss the radial quadrupole mode. We find that the latter acquires a quantum correction exclusively due to the dipole-dipole interaction. As a result, we identify the radial quadrupole as a reasonably accessible source for the signature of dipolar many-body effects and stress the enhancing character that dipolar interactions have for quantum fluctuations in the other oscillation modes.
In this thesis we study the effects of the dipole-dipole interaction on the physics of ultracold quantum gases, both bosonic and fermionic, within the theoretical framework provided by the mean-field regime. This kind of interaction takes place in ultracold atomic gases (for instance 52Cr or 164Dy) due to their atomic magnetic dipole moment, and in ultracold molecular gases due to the magnetic or electric dipole moment. \n \nIn the case of quantum gases of bosonic atoms, or Bose-Einstein condensates, the dipole-dipole interaction can be studied within mean-field approximation using the Gross-Pitaevskii equation, which now contains a new non-linear term due to the dipole-dipole interaction. We investigate, on the one hand dipolar condensates confined in harmonic traps, and on the other dipolar condensates confined in toroidal traps. In the harmonic geometry, our focus is on the study of the ground state and the quantized vortex state, where the density profile is characterized as well as some properties leading to the process of vortex formation, such as the critical frequency and the energy barrier that has to be overcome to bring the vortex from the surface to the centre of the gas. We finish the study of dipolar condensates in harmonic traps by dynamically simulating the precession frequency of an off-center vortex in a non-rotating condensate. \n \nIn the toroidal geometry the dipolar effects are strongly magnified when the polarization axis of the dipoles is perpendicular to the trap symmetry axis. In this case, the anisotropic structure of the density can be understood as the response of the system to the double-well effective potential along the ring. We have studied the dynamics of this system when the initial number of atoms in the left and right wells is imbalanced, predicting Josephson and self-trapping oscillations depending on the initial condition. This has led us to name this new system as Self-induced Josephson Junction. We have studied in detail the self-trapping regime and we have seen that the particle flux inversion is closely related to the crossing of vortices across the Josephson junctions. This result opens the door to establishing a more direct connection between the phase-slip regime, widely addressed in superfluid helium, and the self-trapping regime of condensates. \n \nIn the case of quantum gases of fermionic dipolar particles, we have studied how the radial quadrupole mode allows one to distinguish between hydrodynamic and collisionless regimes. We have analytically calculated the frequency of this mode in the mean-field approximation, generalizing the results from the Thomas-Fermi approximation for trapped ideal Fermi gases. On the one hand, we observe that the frequency in the hydrodynamic regime is smaller than in non-dipolar Fermi gases, while in the collisionless regime the frequency is larger or smaller than that corresponding to the non-interacting system depending on the geometry of the harmonic trap. On the other hand, we predict that reducing the trap deformation (aspect ratio) an observable jump in the frequency of the radial quadrupole mode would take place, which would correspond to the transition between the collisionless and hydrodynamic regimes, for instance when the gas undergoes the transition to the superfluid state.
The work of this thesis concerns the properties of a Bose gas of polarised dipoles that have long-range and anisotropic interactions. Our work is divided into two parts. First, the stability of a dipolar Bose gas at finite temperature (both above and below the critical Bose-Einstein condensation (BEC) temperature Tc). Second, the fluctuations of a dipolar BEC at zero and small finite temperature (T ≪ Tc) in a regime where rotonic excitations emerge. \n \nPart I: Stability of a Trapped Finite Temperature Dipolar Bose Gas: Above Tc we implement a semiclassical Hartree-Fock theory and characterise the dependence of the stability boundary on temperature, trap geometry and the strength of the dipole-dipole interaction and contact interaction. We find that stability is greatly enhanced above Tc and that trap geometry continues to play a key role. Furthermore, we find that for oblate traps a novel double instability feature emerges. \nTo extend our stability analysis to the low temperature regime, T < Tc, we develop a beyond semiclassical Hartree theory. We use this to characterise the stability boundary as a function of geometry. Interestingly, we find large beyond semiclassical effects above Tc for prolate trapping geometries. We characterise thermal effects on biconcave condensate states. \n \nPart II: Rotons and Fluctuations in a Trapped Dipolar Condensate: To study density fluctuations we implement a numerical scheme to solve the Gross-Pitaevskii equation and the Bogoliubov de Gennes equations. We find that the phonon and roton gases spatially separate and we characterise the role of the anomalous density on the density fluctuations of the thermally activated rotons. We develop a numerical scheme that calculates number fluctuations within cells of various shapes and sizes, and find a strong peak in the fluctuations when the cell size is around half the roton wavelength, which should be detectable by current experiments. By tailoring the cell shape we predict that experiments should be able to detect the effects of individual roton modes. \nFor the study of zero temperature fluctuations we deploy the Gross-Pitaevskii and Bogoliubov de Gennes equations to calculate the dynamic and static structure factors for a highly oblate BEC. We find a clear signature of the roton gas dispersion relation within the structure factors. This signature should be detectible in current experiments using Bragg spectroscopy.
This thesis contains a study of ultracold paramagnetic atoms or polar molecules characterized by a long-range anisotropic dipolar interaction. We particularly focus on two aspects of ultracold dipolar gases. In the first problem the ground state properties of dipolar Bose-Einstein condensates (BEC) are investigated. This problem has gained importance due to recent experimental advances in achieving a condensate of Chromium atoms and ongoing research to produce quantum degenerate polar molecules. In the second problem, we consider possible applications of ultracold polar molecules to rotation sensing and interferometry. First, we concentrate on the interplay between the trapping geometry and dipole-dipole interaction for a polarized dipolar bosonic condensate. As the dipole-dipole interaction is attractive along the polarized direction, the lowest energy state of the BEC is always a collapsed state. However by applying a trapping potential along the polarization direction it is possible to achieve a metastable dipolar BEC. By numerically solving the Gross-Pitaevskii equation, we show that below a critical interaction strength, a metastable state exists depending on the trapping geometry. We also show that a novel feature of dipolar BEC is the appearance of different structural metastable ground states for certain combinations of trapping geometry and particle number. Next, by mixing in single component fermions we show that dipolar BEC can be stabilized against collapse in pancake shaped or cylindrical traps. We also show that the excitation spectrum of the BEC may have a minimum for non-zero momentum, termed a “roton minimum”. This minimum leads to a transition to stable or metastable density-wave states depending on the density of the bosons and boson-fermion interaction strength. In the second problem, we study a proposal for a large-angle coherent beam splitter for polar molecules. By taking into account the effect of a quasi-static external electric field on the rotational levels of the polarized molecules we show that it is possible to coherently split a stationary cloud of molecules into two counter-propagating components. We then investigate the effect of longitudinal acceleration on the transverse motion of the particles, assuming that the longitudinal motion of the molecules can be approximated classically by a wave packet with some mean velocity while the transverse motion is governed by quantum mechanics. We propose a particular time-dependent shape of acceleration to minimize the excitations in the transverse motion. Our theory is also applicable to the general case of particles moving along a circular guide with time-dependent longitudinal velocity. In addition, we include the effects of velocity fluctuations due to noise in the accelerating field.
The low-density expansions for the energy, chemical potential, and condensate depletion of the homogeneous dilute dipolar Bose gas are obtained by regularizing the dipole-dipole interaction at long distances. It is shown that the leading term, proportional to the density, allows a simple physical interpretation and consistently describes the thermodynamic stability of the system. The long-range asymptotics are obtained analytically for the normal and anomalous one-particle correlation functions and the pair distribution function. We discuss the properties of the two-body scattering with zero relative momentum for the dipole-dipole interaction; in particular, we derive the asymptotics of the wave function and a correction to the scattering length for small values of the dipolar range. We show how the density expansions can be derived within the Bogoliubov model of weakly interacting particles without any divergence from the assumption of universality of the expansions at low densities.