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arXiv:1511.03684 · Physical Review Letters

Quantum Effects in Higher-Order Correlators of a Quantum-Dot Spin Qubit

A. Bechtold, Fuxiang Li, Kai Müller, Tobias Simmet, P.-L. Ardelt, Jonathan James Finley, Nikolai A. Sinitsyn

Published Jul 6, 2016• 31 citations
arXivHTMLPDF

Abstract

We measure time correlators of a spin qubit in an optically active quantum dot beyond the second order. Such higher-order correlators are shown to be directly sensitive to pure quantum effects that cannot be explained within the classical framework. They allow direct determination of ensemble and quantum dephasing times, T_{2}^{*} and T_{2}, using only repeated projective measurements and without the need for coherent spin control. Our method enables studies of purely quantum behavior in solid state systems, including tests of the Leggett-Garg type of inequalities that rule out local hidden variable interpretation of the quantum-dot spin dynamics.

DOI
10.1103/physrevlett.117.027402

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We measure time correlators of a spin qubit in an optically active quantum dot beyond the second order. Such higher-order correlators are shown to be directly sensitive to pure quantum effects that cannot be explained within the classical framework. They allow direct determination of ensemble and quantum dephasing times, T_{2}^{*} and T_{2}, using only repeated projective measurements and without the need for coherent spin control. Our method enables studies of purely quantum behavior in solid state systems, including tests of the Leggett-Garg type of inequalities that rule out local hidden variable interpretation of the quantum-dot spin dynamics.
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Solid state based quantum information processing is focused on physical implementation of all necessary elements of quantum computation and quantum information in solid state systems, mainly due to their scalability compared to e.g. optical systems. Among many proposals to realize these types of devices, such as quantum dots as charge qubits or Josephson junction circuits, we study here one of the most promising candidates, i.e., the spin of an electron confined to a quantum dot as a qubit. Experimentally, it has been shown that the relaxation rate of this two level system can be pushed above few seconds in low magnetic fields. Moreover, using spin echo techniques, \nthe spin dephasing time can be maximized up to milliseconds with the current technology. This long spin decay time is one of the main reasons that make this system desirable for quantum computation and quantum information purposes. \nWe reexamined the recent measurement based proposal called one-way quantum computation which exploits entanglement and local measurements as tools to perform quantum computation on N qubits. Although it was suggested in the original work to entangle the qubits via the nearest neighbor Ising interaction, we investigated how one can generate the so-called cluster states with the Heisenberg interaction. We extended our method to include more general forms of Heisenberg interaction such as asymmetric coupling of adjacent qubits. These forms of couplings, rather than Ising interaction, are more encountered in solid state devices, and therefore make it possible to perform one-way quantum computation with electron spins in quantum dots coupled via exchange interaction to their adjacent spins. \n \nChapters II, III, and IV of my thesis are devoted to the study of the spin-orbit interaction in heterostructure quantum dots and its effect on the spin dynamics. We observed that one can actually use spin-orbit interaction to manipulate the spin state of an electron on time scales much smaller than the spin dephasing time. Specifically, in chapter II, we studied the effect of a nearby functioning quantum point contact (QPC) on the relaxation of the electron spin and show that the charge fluctuations in QPC lead to spin relaxation of the confined electron in the presence of spin-orbit interactiom and an applied magnetic field. We also addressed the relation of this rate to the microscopic parameters of the system and found some geometrical dependence of the spin relaxation time on the orientation of the QPC on the substrate. Moreover, we showed in chapters III and IV that the spin-orbit interaction can play a positive role, in order to rotate the spin around the Bloch sphere. We considered different mechanisms, particularly, Electron Dipole Spin Resonance (EDSR) and holonomic unitary gates in quantum dots. We verified that these mechanisms of spin manipulation can be realized in solid state systems with the state of the art semiconductor technologies. \n \nChapter V of the thesis covers a slightly different topic and focuses on the role of the Coulomb interaction in electronic transport. There, we reviewed the non-analytic corrections to the Fermi liquid behavior and their consequences on the momentum occupation number of the electrons in a two dimensional electron gas (2DEG). As an example, we calculated the tunneling rate from an interacting electron reservoir onto a quantum dot and compared our result to the corresponding case for electron tunneling between bilayer 2DEGs. Moreover, within RPA approximation, we found that the electron-plasmon coupling leads to a quadratic frequency dependence of the electron self-energy at low frequencies at the Fermi surface. This correction suppresses the same order corrections due to the particle-hole bubble. \n \n \n
We show that the correlations in stochastic outputs of time-distributed weak measurements can be used to study the dynamics of an individual quantum object, with a proof-of-principle setup based on small Faraday rotation caused by a single spin in a quantum dot. In particular, the third-order correlation can reveal the 'true' spin decoherence, which would otherwise be concealed by the inhomogeneous broadening effect in the second-order correlations. The viability of such approaches lies in the fact that (i) in weak measurement the state collapse that would disturb the system dynamics occurs at a very low probability and (ii) a shot of measurement projecting the quantum object to a known basis state serves as a starter or stopper of the evolution without pumping or coherently controlling the system as otherwise required in conventional spin echo.
In the tests for macrorealism proposed by Leggett and Garg, the temporal correlation functions of a dichotomic variable QQQ must be measured in a noninvasive way to rule out alternative classical explanations of Leggett-Garg inequality violations. Ideal negative measurements in which a null result is argued to be a noninvasive determination of the system's state are often used. From a quantum-mechanical perspective, such a measurement collapses the wave function and will therefore typically be found to be invasive under any experimental check. Here, a simple modified ideal negative measurement protocol is described for measuring the correlation functions, which is argued to be noninvasive from both classical and quantum perspectives and hence the noninvasiveness can then be checked experimentally, thereby permitting a quantitative measure of the degree of clumsiness of the measurement. It is also shown how this procedure may be extended to measure higher-order correlation functions, and a number of higher-order conditions for macrorealism are derived.
We briefly review the physics of gate operations between quantum dot spin-qubits and analyze the dynamics of quantum entanglement in such processes. The indistinguishable character of the electrons whose spins realize the qubits gives rise to further entanglement-like quantum correlations that go beyond simple antisymmetrization effects. We also summarize further recent results concerning this type of quantum correlations of indistinguishable particles. Finally we discuss decoherence properties of spin-qubits when coupled to surrounding nuclear spins in a semiconductor nanostructure
In the present paper we introduce a way of identifying quantum phase transitions of many-body systems by means of local time correlations and Leggett-Garg inequalities. This procedure allows us to experimentally determine the quantum critical points not only of finite-order transitions but also those of infinite order, as the Kosterlitz-Thouless transition that is not always easy to detect with current methods. By means of simple analytical arguments for a general spin-1/21/21/2 Hamiltonian, and matrix product simulations of one-dimensional XXZXXZXXZ and anisotropic XYXYXY models, we argue that finite-order quantum phase transitions can be determined by singularities of the time correlations or their derivatives at criticality. The same features are exhibited by corresponding Leggett-Garg functions, which noticeably indicate violation of the Leggett-Garg inequalities for early times and all the Hamiltonian parameters considered. In addition, we find that the infinite-order transition of the XXZXXZXXZ model at the isotropic point can be revealed by the maximal violation of the Leggett-Garg inequalities. We thus show that quantum phase transitions can be identified by purely local measurements and that many-body systems constitute important candidates to observe experimentally the violation of Leggett-Garg inequalities.