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arXiv:1510.07682 · Physical review. B./Physical review. B

Entanglement entropy and topological order in resonating valence-bond quantum spin liquids

Julia Wildeboer, Alexander Seidel, Roger G. Melko

Published Mar 6, 2017• 14 citations
arXivHTMLPDF

Abstract

On the triangular and kagome lattices, short-ranged resonating valence-bond wave functions can be sampled without the sign problem using a recently developed Pfaffian Monte Carlo scheme. In this Rapid Communication, we study the Renyi entanglement entropy in these wave functions using a replica-trick method. Using various spatial bipartitions, including the Levin-Wen construction, our finite-size scaled Renyi entropy gives a topological contribution consistent with $\ensuremath{\gamma}=ln(2)$, as expected for a gapped ${\mathbb{Z}}_{2}$ quantum spin liquid. We prove that the mutual statistics is consistent with the toric code anyon model and rule out any other quasiparticle statistics such as the double semion model.

DOI
10.1103/physrevb.95.100402

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On the triangular and kagome lattices, short-ranged resonating valence-bond wave functions can be sampled without the sign problem using a recently developed Pfaffian Monte Carlo scheme. In this Rapid Communication, we study the Renyi entanglement entropy in these wave functions using a replica-trick method. Using various spatial bipartitions, including the Levin-Wen construction, our finite-size scaled Renyi entropy gives a topological contribution consistent with \ensuremathγ=ln(2)\ensuremath{\gamma}=ln(2)\ensuremathγ=ln(2), as expected for a gapped Z2{\mathbb{Z}}_{2}Z2​ quantum spin liquid. We prove that the mutual statistics is consistent with the toric code anyon model and rule out any other quasiparticle statistics such as the double semion model.
We construct a short-range resonating-valence-bond (RVB) state on the ruby lattice, using projected entangled-pair states with bond dimension D=3D=3D=3. By introducing nonlocal moves to the dimer patterns on the torus, we distinguish four distinct sectors in the space of dimer coverings, which is a signature of the topological nature of the RVB wave function. Furthermore, by calculating the reduced density matrix of a bipartition of the RVB state on an infinite cylinder and exploring its entanglement entropy, we confirm the topological nature of the RVB wave function by obtaining a nonzero topological contribution, $\ensuremath{\gamma}=\ensuremath{-}\mathrm{ln}\phantom{\rule{4pt}{0ex}}2$, consistent with that of a Z2{\mathbb{Z}}_{2}Z2​ topological quantum spin liquid. We also calculate the ground-state energy of the spin-12\frac{1}{2}21​ antiferromagnetic Heisenberg model on the ruby lattice and compare it with the RVB energy. Finally, we construct a quantum dimer model for the ruby lattice and discuss it as a possible parent Hamiltonian for the RVB wave function.
Abstract We develop a nonequilibrium increment method in quantum Monte Carlo simulations to obtain the Rényi entanglement entropy of various quantum many-body systems with high efficiency and precision. To demonstrate its power, we show the results on a few important yet difficult (2 + 1)dquantum lattice models, ranging from the Heisenberg quantum antiferromagnet with spontaneous symmetry breaking, the quantum critical point with O(3) conformal field theory (CFT) to the toric code Z2{{\mathbb{Z}}}_{2}Z2​ Z2 topological ordered state and the Kagome Z2{{\mathbb{Z}}}_{2}Z2​ Z2 quantum spin liquid model with frustration and multi-spin interactions. In all these cases, our method either reveals the precise CFT data from the logarithmic correction or extracts the quantum dimension in topological order, from the dominant area law in finite-size scaling, with very large system sizes, controlled errorbars, and minimal computational costs. Our method, therefore, establishes a controlled and practical computation paradigm to obtain the difficult yet important universal properties in highly entangled quantum matter.
We examine in details the connections between topological and entanglement properties of short-range resonating valence bond (RVB) wave functions using projected entangled pair states (PEPS) on kagome and square lattices on (quasi)infinite cylinders with generalized boundary conditions (and perimeters with up to 20 lattice spacings). By making use of disconnected topological sectors in the space of dimer lattice coverings, we explicitly derive (orthogonal) ``minimally entangled'' PEPS RVB states. For the kagome lattice, using the quantum Heisenberg antiferromagnet as a reference model, we obtain the finite-size scaling with increasing cylinder perimeter of the vanishing energy separations between these states. In particular, we extract two separate (vanishing) energy scales corresponding (i) to insert a vison line between the two ends of the cylinder and (ii) to pull out and freeze a spin at either end. We also investigate the relations between bulk and boundary properties and show that, for a bipartition of the cylinder, the boundary Hamiltonian defined on the edge can be written as a product of a highly nonlocal projector, which fundamentally depends upon boundary conditions, with an emergent (local) SU(2)(2)(2)-invariant one-dimensional (superfluid) ttt-JJJ Hamiltonian, which arises due to the symmetry properties of the auxiliary spins at the edge. This multiplicative structure, a consequence of the disconnected topological sectors in the space of dimer lattice coverings, is characteristic of the topological nature of the states. For minimally entangled RVB states, it is shown that the entanglement spectrum, which reflects the properties of the (gapless or gapped) edge modes, is a subset of the spectrum of the local Hamiltonian, e.g., half of it for the kagome RVB state, providing a simple argument on the origin of the topological entanglement entropy ${S}_{0}=\ensuremath{-}\mathrm{ln}2$ of the Z2{\mathbb{Z}}_{2}Z2​ spin liquid. We propose to use these features to probe topological phases in microscopic Hamiltonians, and some results are compared to existing density matrix renormalization group data.
Gapped Z2{\mathbb{Z}}_{2}Z2​ spin liquids have been proposed as candidates for the ground state of the S=1/2S=1/2S=1/2 quantum antiferromagnet on the kagome lattice. We extend the use of projected entangled pair states to construct (on the cylinder) resonating valence bond (RVB) states including both nearest-neighbor and next-nearest-neighbor singlet bonds. Our ansatz---dubbed ``simplex spin liquid''---allows for an asymmetry between the two types of triangles (of order 22%--3%2 in the energy density after optimization) leading to the breaking of inversion symmetry. We show that the topological Z2{\mathbb{Z}}_{2}Z2​ structure is still preserved and, by considering the presence or the absence of spinon and vison lines along an infinite cylinder, we explicitly construct four orthogonal RVB minimally entangled states. The spinon and vison coherence lengths are extracted from a finite size scaling with regard to the cylinder perimeter of the energy splittings of the four sectors and are found to be of the order of the lattice spacing. The entanglement spectrum of a partitioned (infinite) cylinder is found to be gapless, suggesting the occurrence, on a cylinder with real open boundaries, of gapless edge modes formally similar to Luttinger liquid (nonchiral) spin and charge modes. When inversion symmetry is spontaneously broken, the RVB spin liquid exhibits an extra Ising degeneracy, which might have been observed in recent exact diagonalization studies.
The topological entanglement entropy (TEE) of Gutzwiller projected RVB state is studied with Monte Carlo simulation. With tricks to speed up the convergence of TEE, we are able to show that the spin liquid state studied in Zhang et al. [Phys. Rev. B 84, 075128 (2011)] actually does not support Z2{Z}_{2}Z2​ topological order. We find that both an approximate Marshall sign structure and a long-ranged RVB amplitude are responsible for the suppression of the vison gap in this spin liquid state. On the other hand, a TEE of ln2\mathrm{ln}2ln2 is clearly demonstrated for a short range RVB state on triangular lattice proposed in Yunoki et al. [Phys. Rev. B 74, 014408 (2006)]. We find the TEE of the RVB wave function is mainly determined by its phase rather than its amplitude. Our results indicate that the effective field theory misses some key information for the topological property of a RVB state.
We introduce a Monte Carlo scheme based on sampling of Pfaffians to investigate Anderson's resonating-valence-bond (RVB) spin liquid wave function on the kagome and the triangular lattice. This eliminates a sign problem that prevents utilization of the valence bond basis in Monte Carlo studies for nonbipartite lattices. Studying lattice sizes of up to 600 sites, we calculate singlet-singlet and spin-spin correlations and demonstrate how the lattice symmetry is restored within each topological sector as the system size is increased. Our findings are consistent with the expectation that the nearest-neighbor RVB states describe a topological spin liquid on these nonbipartite lattices.