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arXiv:1510.00608 · Physical Review A

Coherent exciton dynamics in a dissipative environment maintained by an off-resonant vibrational mode

E. K. Levi, E. K. Twyeffort Irish, Brendon W. Lovett

Published Apr 14, 2016• 11 citations
arXivHTMLPDF

Abstract

The interplay between an open quantum system and its environment can lead to both coherent and incoherent behavior. We explore the extent to which strong coupling to a single bosonic mode can alter the coherence properties of a two-level system in a structured environment. This mode is treated exactly, with the rest of the environment comprising a Markovian bath of bosonic modes. The strength of the coupling between the two-level system and the single mode is varied for a variety of forms for the bath spectral density in order to assess whether the coherent dynamics of the two-level system are modified. We find a clear renormalization of the site population oscillation frequency that causes an altered interaction with the bath. This leads to enhanced or reduced coherent behavior of the two-level system, depending on the form of the spectral density function. We present an intuitive interpretation, based on an analytical model, to explain the behavior.

DOI
10.1103/physreva.93.042109

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The interplay between an open quantum system and its environment can lead to both coherent and incoherent behavior. We explore the extent to which strong coupling to a single bosonic mode can alter the coherence properties of a two-level system in a structured environment. This mode is treated exactly, with the rest of the environment comprising a Markovian bath of bosonic modes. The strength of the coupling between the two-level system and the single mode is varied for a variety of forms for the bath spectral density in order to assess whether the coherent dynamics of the two-level system are modified. We find a clear renormalization of the site population oscillation frequency that causes an altered interaction with the bath. This leads to enhanced or reduced coherent behavior of the two-level system, depending on the form of the spectral density function. We present an intuitive interpretation, based on an analytical model, to explain the behavior.
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We derive the exact out-of-equilibrium Wigner function of a bosonic mode linearly coupled to a bosonic bath of arbitrary spectral density. Our solution does not rely on any master equation approach and it therefore also correctly describes a bosonic mode which is initially entangled with its environment. It has been recently suggested that non-Markovian quantum effects lead to dissi- pationless dynamics in the case of a strong coupling to a bath whose spectral density has a support bounded from below. We show in this work that such a system undergoes a quantum phase transi- tion at some critical bath coupling strength. The apparent dissipationless dynamics then correspond to the relaxation towards the new ground-state.
The decoherence of a two-state system coupled with a sub-Ohmic bath is investigated theoretically by means of the perturbation approach based on a unitary transformation. It is shown that the decoherence depends strongly and sensitively on the structure of environment. Nonadiabatic effect is treated through the introduction of a function ${\ensuremath{\xi}}_{k}$ which depends on the boson frequency and renormalized tunneling. The results are as follows: (i) the nonequilibrium correlation function P(t)P(t)P(t), the dynamical susceptibility ${\ensuremath{\chi}}^{\ensuremath{''}}(\ensuremath{\omega})$, and the equilibrium correlation function C(t)C(t)C(t) are analytically obtained for $s\ensuremath{\leqslant}1$; (ii) the phase diagram of thermodynamic transition shows the delocalized-localized transition point ${\ensuremath{\alpha}}_{l}$ which agrees with exact results and numerical data from the numerical renormalization group; (iii) the dynamical transition point ${\ensuremath{\alpha}}_{c}$ between coherent and incoherent phase is explicitly given. A crossover from the coherent oscillation to incoherent relaxation appears with increasing coupling (for $\ensuremath{\alpha}>{\ensuremath{\alpha}}_{c}$, the coherent dynamics disappear); (iv) the Shiba's relation and sum rule are exactly satisfied when $\ensuremath{\alpha}\ensuremath{\leqslant}{\ensuremath{\alpha}}_{c}$; (v) an underdamping-overdamping transition point ${\ensuremath{\alpha}}_{c}^{*}$ exists in the function $S(\ensuremath{\omega})$. Consequently, the dynamical phase diagrams in both ohmic and sub-Ohmic case are mapped out. For $\ensuremath{\Delta}⪡{\ensuremath{\omega}}_{c}$, the critical couplings (${\ensuremath{\alpha}}_{l},{\ensuremath{\alpha}}_{c}$, and ${\ensuremath{\alpha}}_{c}^{*}$) are proportional to ${\ensuremath{\Delta}}^{1\ensuremath{-}s}$.
The character of evolution of an open quantum system is often encoded in the correlation function of the environment or, equivalently, in the spectral density function of the interaction. When the environment is heterogeneous, e.g., consists of several independent subenvironments with different spectral functions, one of the subenvironments can be considered auxiliary and used to control decoherence of the open quantum system in the remaining part of the environment. The control can be realized, for example, by adjusting the character of interaction with the subenvironment via suitable parameters of its spectral density. We investigate non-Markovian evolution of a two-level system (qubit) under influence of three independent decoherence channels: two of them have classical nature and originate from interaction with a stochastic field, and the third is a quantum channel formed by interaction with a bosonic bath. By modifying spectral densities of the channels, we study their impact on steady states of the two-level system, evolution of its density matrix, and the equilibrium emission spectra. Additionally, we investigate the impact of the rotation-wave approximation applied to the bath channel on accuracy of the results.
The dynamical behavior of a two-level system coupled linearly to a dissipative bath of two-level systems whose tunneling splittings and coupling parameters are distributed according to an Ohmic spectrum is studied using numerical path integral methods as well as the noninteracting blip approximation for an equivalent harmonic environment characterized by a scaled spectral density. Comparisons with the behaviors of the conventional spin-boson model of similar coupling strength reveal a weaker quenching of coherence in the present case. Finally, the boundary in parameter space between coherent and incoherent dynamics is mapped.
We investigate the exact dynamics of first-order system--bath coherence induced by excitation exchange in bilinear bosonic models. By solving the linear Heisenberg equations, we obtain the exact evolution of system and bath operators and evaluate the first-order coherence between the system mode and the collective bath mode directly coupled to it. We analyze how this coherence depends on initial occupations, coupling strength, spectral width, and detuning, showing that its buildup and oscillatory behavior are closely related to excitation exchange and reservoir memory. We further examine controlled coherence dynamics under leakage-elimination-operator inspired modulation of the system frequency. The results show that random modulation can suppress excitation leakage and maintain finite and relatively stable coherence fluctuations at long times. These results clarify the evolution and control of first-order system--bath coherence in settings where a localized bosonic mode is coupled to a structured bosonic reservoir.