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arXiv:1507.08038 · Physical review. B./Physical review. B

Plaquette-triplon analysis of magnetic disorder and order in a trimerized spin-1 kagome Heisenberg antiferromagnet

Pratyay Ghosh, Akhilesh Kumar Verma, Brijesh Kumar

Published Jan 19, 2016• 16 citations
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Abstract

A spin-1 Heisenberg model on trimerized kagome lattice is studied by doing a low-energy bosonic theory in terms of plaquette triplons defined on its triangular unit cells. The model considered has an intratriangle antiferromagnetic exchange interaction $J$ (set to 1) and two intertriangle couplings ${J}^{\ensuremath{'}}>0$ (nearest neighbor) and ${J}^{\ensuremath{''}}$ (next nearest neighbor; of both signs). The triplon analysis performed on this model investigates the stability of the trimerized singlet ground state (which is exact in the absence of intertriangle couplings) in the ${J}^{\ensuremath{'}}\ensuremath{-}{J}^{\ensuremath{''}}$ plane. It gives a quantum phase diagram that has two gapless antiferromagnetically ordered phases separated by the spin-gapped trimerized singlet phase. The trimerized singlet ground state is found to be stable on ${J}^{\ensuremath{''}}=0$ line (the nearest-neighbor case), and on both sides of it for ${J}^{\ensuremath{''}}\ensuremath{\ne}0$, in an extended region bounded by the critical lines of transition to the gapless antiferromagnetic phases. The gapless phase in the negative ${J}^{\ensuremath{''}}$ region has a coplanar ${120}^{\ensuremath{\circ}}$ antiferromagnetic order with $\sqrt{3}\ifmmode\times\else\texttimes\fi{}\sqrt{3}$ structure. In this phase, all the magnetic moments are of equal length, and the angle between any two of them on a triangle is exactly ${120}^{\ensuremath{\circ}}$. The magnetic lattice in this case has a unit cell consisting of three triangles. The other gapless phase, in the positive ${J}^{\ensuremath{''}}$ region, is found to exhibit a different coplanar antiferromagnetic order with ordering wave vector $\mathbf{q}=(0,0)$. Here, two magnetic moments in a triangle are of the same magnitude, but shorter than the third. While the angle between two short moments is ${120}^{\ensuremath{\circ}}\ensuremath{-}2\ensuremath{\delta}$, it is ${120}^{\ensuremath{\circ}}+\ensuremath{\delta}$ between a short and the long one. Only when ${J}^{\ensuremath{''}}={J}^{\ensuremath{'}}$, their magnitudes become equal and the relative angles ${120}^{\ensuremath{\circ}}$. The magnetic lattice in this $\mathbf{q}=(0,0)$ phase has the translational symmetry of the kagome lattice with triangular unit cells of reduced (isosceles) symmetry. This reduction in the point-group symmetry is found to show up as a difference in the intensities of certain Bragg peaks, whose ratio ${I}_{(1,0)}/{I}_{(0,1)}=4{sin}^{2}(\frac{\ensuremath{\pi}}{6}+\ensuremath{\delta})$ presents an experimental measure of the deviation $\ensuremath{\delta}$ from the ${120}^{\ensuremath{\circ}}$ order.

DOI
10.1103/physrevb.93.014427

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A spin-1 Heisenberg model on trimerized kagome lattice is studied by doing a low-energy bosonic theory in terms of plaquette triplons defined on its triangular unit cells. The model considered has an intratriangle antiferromagnetic exchange interaction JJJ (set to 1) and two intertriangle couplings J\ensuremath′>0{J}^{\ensuremath{'}}>0J\ensuremath′>0 (nearest neighbor) and J\ensuremath′′{J}^{\ensuremath{''}}J\ensuremath′′ (next nearest neighbor; of both signs). The triplon analysis performed on this model investigates the stability of the trimerized singlet ground state (which is exact in the absence of intertriangle couplings) in the J\ensuremath′\ensuremath−J\ensuremath′′{J}^{\ensuremath{'}}\ensuremath{-}{J}^{\ensuremath{''}}J\ensuremath′\ensuremath−J\ensuremath′′ plane. It gives a quantum phase diagram that has two gapless antiferromagnetically ordered phases separated by the spin-gapped trimerized singlet phase. The trimerized singlet ground state is found to be stable on J\ensuremath′′=0{J}^{\ensuremath{''}}=0J\ensuremath′′=0 line (the nearest-neighbor case), and on both sides of it for J\ensuremath′′\ensuremath≠0{J}^{\ensuremath{''}}\ensuremath{\ne}0J\ensuremath′′\ensuremath=0, in an extended region bounded by the critical lines of transition to the gapless antiferromagnetic phases. The gapless phase in the negative J\ensuremath′′{J}^{\ensuremath{''}}J\ensuremath′′ region has a coplanar 120\ensuremath∘{120}^{\ensuremath{\circ}}120\ensuremath∘ antiferromagnetic order with 3\ifmmode×\else\texttimes\fi3\sqrt{3}\ifmmode\times\else\texttimes\fi{}\sqrt{3}3​\ifmmode×\else\texttimes\fi3​ structure. In this phase, all the magnetic moments are of equal length, and the angle between any two of them on a triangle is exactly 120\ensuremath∘{120}^{\ensuremath{\circ}}120\ensuremath∘. The magnetic lattice in this case has a unit cell consisting of three triangles. The other gapless phase, in the positive J\ensuremath′′{J}^{\ensuremath{''}}J\ensuremath′′ region, is found to exhibit a different coplanar antiferromagnetic order with ordering wave vector q=(0,0)\mathbf{q}=(0,0)q=(0,0). Here, two magnetic moments in a triangle are of the same magnitude, but shorter than the third. While the angle between two short moments is 120\ensuremath∘\ensuremath−2\ensuremathδ{120}^{\ensuremath{\circ}}\ensuremath{-}2\ensuremath{\delta}120\ensuremath∘\ensuremath−2\ensuremathδ, it is 120\ensuremath∘+\ensuremathδ{120}^{\ensuremath{\circ}}+\ensuremath{\delta}120\ensuremath∘+\ensuremathδ between a short and the long one. Only when J\ensuremath′′=J\ensuremath′{J}^{\ensuremath{''}}={J}^{\ensuremath{'}}J\ensuremath′′=J\ensuremath′, their magnitudes become equal and the relative angles 120\ensuremath∘{120}^{\ensuremath{\circ}}120\ensuremath∘. The magnetic lattice in this q=(0,0)\mathbf{q}=(0,0)q=(0,0) phase has the translational symmetry of the kagome lattice with triangular unit cells of reduced (isosceles) symmetry. This reduction in the point-group symmetry is found to show up as a difference in the intensities of certain Bragg peaks, whose ratio I(1,0)/I(0,1)=4sin2(\ensuremathπ6+\ensuremathδ){I}_{(1,0)}/{I}_{(0,1)}=4{sin}^{2}(\frac{\ensuremath{\pi}}{6}+\ensuremath{\delta})I(1,0)​/I(0,1)​=4sin2(6\ensuremathπ​+\ensuremathδ) presents an experimental measure of the deviation \ensuremathδ\ensuremath{\delta}\ensuremathδ from the 120\ensuremath∘{120}^{\ensuremath{\circ}}120\ensuremath∘ order.
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We study the ground-state phase diagram of the spin-1/21/21/2 antiferromagnetic Heisenberg model on the square-kagome lattice using infinite projected entangled-pair states (iPEPS). By systematically varying the ratio of exchange couplings on triangular and square plaquettes, we establish a complete quantum phase diagram in the thermodynamic limit. In the intermediate-coupling regime, we identify four distinct nonmagnetic phases that are unambiguously characterized as valence-bond crystals (VBCs) by their symmetry-inequivalent patterns of strong and weak spin-spin correlations. These include a plaquette crossed-dimer VBC, a loop-six VBC stabilized around the isotropic point, a generalized pinwheel VBC with reduced rotational symmetry, and a decorated loop-six VBC proximate to ferrimagnetic order. We determine the phase boundaries using a combination of bond-resolved correlation functions, entanglement entropy, and magnetization. For transitions not accompanied by sharp entanglement signatures, we extract the spin gap from finite-field simulations, allowing us to distinguish gapped and gapless VBC phases. At larger coupling ratios, the system undergoes transitions into imperfect and perfect ferrimagnetic states. Our results resolve long-standing ambiguities in the square-kagome Heisenberg model and provide a quantitatively reliable reference for future theoretical and experimental studies of frustrated quantum magnets.
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We study the spin-1∕21∕21∕2 Heisenberg model in a lattice that interpolates between the triangular and the kagome lattices. The exchange interaction along the bonds of the kagome lattice is JJJ, and the one along the bonds connecting kagome and nonkagome sites is ${J}^{\ensuremath{'}}$, so that ${J}^{\ensuremath{'}}=J$ corresponds to the triangular limit and ${J}^{\ensuremath{'}}=0$ to the kagome one. We use variational and exact diagonalization techniques. We analyze the behavior of the order parameter for the antiferromagnetic phase of the triangular lattice, the spin gap, and the structure of the spin excitations as functions of ${J}^{\ensuremath{'}}∕J$. Our results indicate that the antiferromagnetic order is not affected by the reduction of ${J}^{\ensuremath{'}}$ down to ${J}^{\ensuremath{'}}∕J\ensuremath{\simeq}0.2$. Below this value, antiferromagnetic correlations grow weaker, a description of the ground state in terms of a N\'eel phase renormalized by quantum fluctuations becomes inadequate, and the finite-size spectra develop features that are not compatible with antiferromagnetic ordering. However, this phase does not appear to be connected to the kagome phase as well, as the low-energy spectra do not evolve with continuity for ${J}^{\ensuremath{'}}\ensuremath{\rightarrow}0$ to the kagome limit. In particular, for any nonzero value of ${J}^{\ensuremath{'}}$, the latter interaction sets the energy scale for the low-lying spin excitations, and a gapless triplet spectrum, destabilizing the kagome phase, is expected.
We use the coupled-cluster method to study the zero-temperature properties of an extended two-dimensional Heisenberg antiferromagnet formed from spin-12\frac{1}{2}21​ moments on an infinite spatially anisotropic kagome lattice of corner-sharing isosceles triangles, with nearest-neighbor bonds only. The bonds have exchange constants J1>0{J}_{1}>0J1​>0 along two of the three lattice directions and ${J}_{2}\ensuremath{\equiv}\ensuremath{\kappa}{J}_{1}>0$ along the third. In the classical limit, the ground-state (GS) phase for $\ensuremath{\kappa}<\frac{1}{2}$ has collinear ferrimagnetic (N\'eel${}^{\ensuremath{'}}$) order where the J2{J}_{2}J2​-coupled chain spins are ferromagnetically ordered in one direction with the remaining spins aligned in the opposite direction, while for $\ensuremath{\kappa}>\frac{1}{2}$ there exists an infinite GS family of canted ferrimagnetic spin states, which are energetically degenerate. For the spin-12\frac{1}{2}21​ case, we find that quantum analogs of both these classical states continue to exist as stable GS phases in some regions of the anisotropy parameter $\ensuremath{\kappa}$, namely, for $0<\ensuremath{\kappa}<{\ensuremath{\kappa}}_{{c}_{1}}$ for the N\'eel${}^{\ensuremath{'}}$ state and for (at least part of) the region $\ensuremath{\kappa}>{\ensuremath{\kappa}}_{{c}_{2}}$ for the canted phase. However, they are now separated by a paramagnetic phase without either sort of magnetic order in the region ${\ensuremath{\kappa}}_{{c}_{1}}<\ensuremath{\kappa}<{\ensuremath{\kappa}}_{{c}_{2}}$, which includes the isotropic kagome point $\ensuremath{\kappa}=1$ where the stable GS phase is now believed to be a topological (Z2{\mathbb{Z}}_{2}Z2​) spin liquid. Our best numerical estimates are ${\ensuremath{\kappa}}_{{c}_{1}}=0.515\ifmmode\pm\else\textpm\fi{}0.015$ and ${\ensuremath{\kappa}}_{{c}_{2}}=1.82\ifmmode\pm\else\textpm\fi{}0.03$.
We consider the triangular kagome XXZ-Ising model (TKL XXZ-Ising model) formed by inserting small triangles ("a-trimers") with XXZ spin-1 inside the triangles of the kagome lattice ("b-trimers"). It is a mixed spin system and can be solved exactly by transforming into the kagome lattice with the general transformation method for decorated spin systems. In the absence of an external field, we integrate out the quantum spins of the a-trimers and map the TKL model to the kagome Ising model exactly. We obtain the full phase diagram and their zero-temperature entropies (e.g., s_{max}=5.48895 per unit cell is given for the phase with the maximum entropy). When an external field is applied, 20 phases are found due to the quantum fluctuations of a-trimers. Moreover, the high spins in the a-trimers can lead to a stable quantized growth of the magnetization process in the Heisenberg limit.