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arXiv:1507.05124

Rabi oscillations in two-level systems beyond the rotating-wave approximation

Adriano A. Batista

Published Jul 17, 2015• 1 citation
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Abstract

Here we use perturbation techniques based on the averaging method to investigate Rabi oscillations in cw and pulse-driven two-level systems (TLS's). By going beyond the rotating-wave approximation, especifically to second-order in perturbation, we obtain the Bloch-Siegert shift of the TLS resonant frequency, in which the resonant frequency increases with the driving field amplitude. This frequency shift implies that short resonant $π$-pulses in which the Rabi frequency is approximately 40\% or higher of the transition frequency do not achieve complete inversion in TLS's. Hence, guided by analytical results based on the averaging technique, we propose two methods for obtaining population inversions in the TLS driven by short $π$-pulses: one with chirping and the other with pulse shaping and near resonance blue-shifted detuning. Both methods minimize dephasing due to the Bloch-Siegert shift, reduce the dependance of the excitation of the TLS on the pulse phase, and are very effective in achieving complete population inversions.

DOI
10.48550/arxiv.1507.05124

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Here we use perturbation techniques based on the averaging method to investigate Rabi oscillations in cw and pulse-driven two-level systems (TLS's). By going beyond the rotating-wave approximation, especifically to second-order in perturbation, we obtain the Bloch-Siegert shift of the TLS resonant frequency, in which the resonant frequency increases with the driving field amplitude. This frequency shift implies that short resonant πππ-pulses in which the Rabi frequency is approximately 40% or higher of the transition frequency do not achieve complete inversion in TLS's. Hence, guided by analytical results based on the averaging technique, we propose two methods for obtaining population inversions in the TLS driven by short πππ-pulses: one with chirping and the other with pulse shaping and near resonance blue-shifted detuning. Both methods minimize dephasing due to the Bloch-Siegert shift, reduce the dependance of the excitation of the TLS on the pulse phase, and are very effective in achieving complete population inversions.
In the framework of the nonsecular perturbation theory based on the Bogoliubov averaging method, the coherent dynamics of multiphoton Raman transitions in a two-level spin system driven by an amplitude-modulated microwave field is studied. Closed-form expressions for the Rabi frequencies of these transitions are obtained beyond the rotating-wave approximation for the low-frequency driving component. It is shown that spin states dressed by the high-frequency component of the driving field are shifted due to the Bloch-Siegert-like effect caused by antiresonant interactions with the strong low-frequency driving. We predict that with increasing the order of the Raman transition, the Rabi frequency decreases and the contribution of the Bloch-Siegert shift to this frequency becomes dominant. It is found that the amplitude and phase of the Rabi oscillations strongly depend on the initial phase of the low-frequency field as well as on detuning from multiphoton resonance. The recent experimental data for the second- and third-order Raman transitions observed for the nitrogen-vacancy center in diamond (Z. Shu et al., arXiv:1804.10492) are well described in the frame of our approach. Our results may provide new possibilities for coherent control of quantum systems.
In a direct two-level qubit system, when the Rabi frequency is comparable to the resonance frequency, the rotating wave approximation is not appropriate. In this case, the Rabi oscillation is accompanied by another oscillation at twice the frequency of the driving field, the so called Bloch-Siegert oscillation (BSO), which depends on the initial phase of the driving field. This oscillation may restrict the precise rotation of a qubit made of direct two-level system. Here, we show that in case of an effectively two-level lambda system, the BSO is inherently negligible, implying a greater precision for rotation of a qubit made of such a lambda system when compared to a direct two-level qubit in a strong driving field.
We obtain pulse-driven Rabi oscillations guided by a generalization of the rotating-wave approximation to include, in the optical-Bloch equations, two-level systems with a time-varying transition energy. We achieve this by using chirped pulses with the central frequency given by the time-varying transition energy. Using this approach, we predict Rabi oscillations in intersubband transitions in a two-subband n-type modulation-doped quantum well by taking into account the time-dependent intersubband energy-gap renormalization due to depolarization-shift effects. We obtain Rabi oscillations for jpi (j=0,1,2, ) pulses in the presence of dephasing.
We investigate the dynamics of a driven two-level system (classical Rabi model) using the counter-rotating-hybridized rotating-wave method (CHRW), which is a simple method based on a unitary transformation with a parameter $\ensuremath{\xi}$. This approach is beyond the traditional rotating-wave approximation (Rabi-RWA) and more importantly, remains the RWA form with a renormalized tunneling strength and a modified driving strength. The reformulated rotating-wave method not only possesses the same mathematical simplicity as the Rabi-RWA but also allows us to explore the effects of counter-rotating (CR) components. We focus on the properties of off-resonance cases for which the Rabi-RWA method breaks down. After comparing the results of different RWA schemes and those of the numerically exact method in a wide range of parameter regime, we show that the CHRW method gives the accurate driven dynamics which is in good agreement with the numerical method. Moreover, the other RWA methods appear as various limiting cases of the CHRW method. The CHRW method reveals the effects of the CR terms clearly by means of coherent destruction of tunneling and Bloch-Siegert shift. Our main results are as follows: (i) the dynamics of the coherent destruction of tunneling is explicitly given and its dependence on $\ensuremath{\Delta}$ is clarified, which is quantitatively in good agreement with the exact results; (ii) the CR modulated Rabi frequency and the Bloch-Siegert shift are analytically calculated, which is the same as the exact results up to fourth order; (iii) the validity of parameter regions of different RWA methods are given and the comparison of dynamics of these methods are shown. Since the CHRW approach is mathematically simple as well as tractable and physically clear, it may be extended to some complicated problems where it is difficult to do a numerical study.
We study the interaction of an ac electric field with a semiconductor quantum well by using the effective nonlinear Bloch equations. Only the first two electron subbands in the well are considered. We apply the rotating wave approximation and derive analytical solutions for the Bloch equations for two different values of the detuning. At exact resonance we find a critical value of the Rabi frequency around which the dynamics of the system changes abruptly. Above this critical value one obtains electron oscillations with complete inversion in the two-subband system, while below this value we obtain electron oscillations without complete inversion and with the majority of the electron population on average in the lower subband. We also present numerical calculations for a specific quantum well structure and assess the limits of validity of the analytical results.
We investigate the bias-modulated dynamics of a strongly driven two-level system using the counterrotating-hybridized rotating-wave (CHRW) method. This CHRW method treats the driving field and the bias on equal footing by a unitary transformation with two parameters $\ensuremath{\xi}$ and $\ensuremath{\zeta}$, and is nonperturbative in driving strength, tunneling amplitude, or bias. In addition, this CHRW method is beyond the traditional rotating-wave approximation (Rabi-RWA) and yet by properly choosing the two parameters $\ensuremath{\xi}$ and $\ensuremath{\zeta}$, the transformed Hamiltonian takes the RWA form with a renormalized energy splitting and a renormalized driving strength. The reformulated CHRW method possesses the same mathematical simplicity as the Rabi-RWA approach and thus allows us to calculate analytically the dynamics and explore explicitly the effect of the bias. We show that the CHRW method gives the accurate driven dynamics for a wide range of parameters as compared to the numerically exact results. When energy scales of the driving are comparable to the intrinsic energy scale of the two-level systems, the counterrotating interactions and static bias profoundly influence the generalized Rabi frequency. In this regime, where ordinary perturbation approaches fail, the CHRW works very well and efficiently. We also demonstrate the dynamics of the system in the strong-driving and off-resonance cases for which the Rabi-RWA method breaks down but the CHRW method remains valid. We obtain analytical expressions for the generalized Rabi frequency and bias-modulated Bloch-Siegert shift as functions of the bias, tunneling, and driving field parameters. The CHRW approach is a mathematically simple and physically clear method. It can be applied to treat some complicated problems for which a numerical study is difficult to perform.