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arXiv:1505.06141 · Optica

Interfacing transitions of different alkali atoms and telecom bands using one narrowband photon pair source

Gerhard Schunk, Ulrich Vogl, Dmitry Strekalov, Michael Förtsch, Florian Sedlmeir, Harald G. L. Schwefel, Manuela Göbelt, Silke H. Christiansen, Gerd Leuchs, Christoph Marquardt

Published Aug 24, 2015• 61 citations
arXivHTMLPDF

Abstract

Quantum information technology strongly relies on coupling of optical photons with narrowband quantum systems, such as quantum dots, color centers, and atomic systems. This coupling requires matching the optical wavelength and bandwidth to the desired system, which presents a considerable problem for most available sources of quantum light. Here we demonstrate coupling of alkali dipole transitions with a tunable source of photon pairs. Our source is based on spontaneous parametric down-conversion in a triply-resonant whispering-gallery mode resonator. For this, we have developed novel wavelength tuning mechanisms, which allow for a coarse tuning to either cesium or rubidium wavelength with subsequent continuous fine-tuning to the desired transition. As a demonstration of the functionality of the source, we performed a heralded single photon measurement of the atomic decay. We present a major advance in controlling the spontaneous down-conversion process, which makes our bright source of single photons now compatible with a plethora of narrow-band resonant systems.

DOI
10.1364/optica.2.000773

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Quantum information technology strongly relies on coupling of optical photons with narrowband quantum systems, such as quantum dots, color centers, and atomic systems. This coupling requires matching the optical wavelength and bandwidth to the desired system, which presents a considerable problem for most available sources of quantum light. Here we demonstrate coupling of alkali dipole transitions with a tunable source of photon pairs. Our source is based on spontaneous parametric down-conversion in a triply-resonant whispering-gallery mode resonator. For this, we have developed novel wavelength tuning mechanisms, which allow for a coarse tuning to either cesium or rubidium wavelength with subsequent continuous fine-tuning to the desired transition. As a demonstration of the functionality of the source, we performed a heralded single photon measurement of the atomic decay. We present a major advance in controlling the spontaneous down-conversion process, which makes our bright source of single photons now compatible with a plethora of narrow-band resonant systems.
Quantum repeaters rely on an interfacing of flying qubits with quantum memories. The most common implementations include a narrowband single photon matched in bandwidth and central frequency to an atomic system. Previously, we demonstrated the compatibility of our versatile source of heralded single photons, which is based on parametric down-conversion in a triply-resonant whispering-gallery mode resonator, with alkaline transitions [Schunk et al., Optica 2, 773 (2015)]. In this paper, we analyze our source in terms of phase matching, available wavelength-tuning mechanisms, and applications to narrow-band atomic systems. We resonantly address the D1 transitions of cesium and rubidium with this optical parametric oscillator pumped above its oscillation threshold. Below threshold, the efficient coupling of single photons to atomic transitions heralded by single telecom-band photons is demonstrated. Finally, we present an accurate analytical description of our observations. Providing the demonstrated flexibility in connecting various atomic transitions with telecom wavelengths, we show a promising approach to realize an essential building block for quantum repeaters.
Single-photon sources play a crucial role in quantum information processing. Among the various methods for generating single photons, spontaneous parametric down-conversion (SPDC) is one of the most widely used. Numerous studies have demonstrated the implementation of SPDC sources across different platforms. Among these, crystalline whispering-gallery-mode resonators (WGMRs) represent an intriguing platform for realizing SPDC-based sources. WGMR-based SPDC sources have been shown to be capable of efficiently interacting with alkali atoms due to the narrow and tunable emission bandwidths. Moreover, they operate with relatively low pump power, which is advantageous for large-scale integration and power-constrained applications. In this work, we further demonstrate the versatility of WGMR-based SPDC sources through three key experiments. First, we generate polarization-entangled photon pairs using an interferometric scheme, achieving a Clauser–Horne–Shimony–Holt (CHSH) inequality parameter of 𝑆 =2.54 ±0.06, violating the classical bound by over eight standard deviations. Second, we observe Hong–Ou–Mandel interference with visibilities of 74 ±5% and 76 ±4% for photons from one and two independent WGMRs, respectively, using an in-coupled pump power as low as 50 nW. Finally, we demonstrate photon--ion interaction between a WGMR-generated photon and a ¹⁴⁷Yb⁺ ion with a success probability of 8%. These results highlight the potential of WGMR-based SPDC sources for scalable quantum networks and hybrid quantum systems.
Abstract We demonstrate an ultrabright, narrow-band and frequency-tunable photon-pair source based on cavity-enhanced spontaneous parametric down conversion (SPDC) which is compatible with atomic transition of rubidium D 2 -line (780 nm) or cesium D 2 -line (852 nm). With the pump beam alternating between a high and a low power phase, the output is switching between the optical parametric oscillator (OPO) and photon-pair generation mode. We utilize the OPO output light to lock the cavity length to maintain the double resonances of signal and idler, as well as to lock the signal frequency to cesium atomic transition. With a type-II phase matching and a double-passed pump scheme such that the cluster frequency spacing is larger than the SPDC bandwidth, the photon-pair output is in a nearly single-mode operation as confirmed by a scanning Fabry–Perot interferometer with its output detected by a photomultiplier. The achieved generation and detection rates are 7.24 × 10 5 and 6142 s −1 mW −1 , respectively. The correlation time of the photon pair is 21.6(2.2) ns, corresponding to a bandwidth of 2 π × 6.6(6) MHz. The spectral brightness is 1.06 × 10 5 s −1 mW −1 MHz −1 . This is a relatively high value under a single-mode operation with the cavity-SPDC scheme. The generated single photons can be readily used in experiments related to atomic quantum memories.
We describe a cavity-enhanced spontaneous parametric down-conversion (CE-SPDC) source for narrowband photon pairs with filters designed such that 97.7% of the correlated photons are in a single mode of 4.3(4) MHz bandwidth. Type-II phase matching, a tuneable-birefringence resonator, MHz-resolution pump tuning, and tuneable Fabry-Perot filters are used to achieve independent signal and idler tuning. We map the CE-SPDC spectrum using difference frequency generation to precisely locate the emission clusters, demonstrate CE-SPDC driven atomic spectroscopy, and measure a contribution from unwanted modes of 7.7%. The generated photon pairs efficiently interact with neutral rubidium, a well-developed system for quantum networking and quantum simulation. The techniques are readily extensible to other material systems.
Cavity-enhanced spontaneous parametric down-conversion is capable of efficient generation of single photons with suitable spectral properties for interfacing with the atoms. However, beside the remarkable progress of this technique, multimode longitudinal emission remains a major drawback. Here, we demonstrate a bright source of single photons that overcomes this limitation by a novel mode-selection technique based on the introduction of an additional birefringent element to the cavity. This enables us to tune the double resonance condition independent of the phase matching and thus to achieve single-mode operation without mode filters. Our source emits single-frequency-mode photons at 852 nm, which is compatible to the Cs D2 line, with a bandwidth of 10.9 MHz and a detected photon-pair rate of 2.5 kHz at 10 mW of pump power, while maintaining g(2)(0) = 0.13. The efficiency of our source is further underlined by detecting a four-photon rate of 0.28 Hz at 20 mW of pump power. These detected rates correspond to a photon-pair generation rate of 47.5 Hz, and a four-photon generation rate of 37 Hz. Such photon generation rates open up a variety of new applications reaching from hybrid light-matter interactions to optical quantum information tasks based on long temporal coherence.
Generating single-mode, narrow-band photons with high purity and brightness has proven to be difficult. Researchers at the University of Vienna have designed a photon source using Spontaneous Parametric Down-Conversion (SPDC) with a doubly resonant Optical Parametric Oscillator (OPO) utilizing an additional birefringent crystal to tune clusters independent of SPDC phase-matching. Achieving the doubly resonant condition in the OPO that enables a single mode is the challenge when creating a photon source with both single-mode and narrow-bandwidth. This is resolved here, as the resulting photon source has a bandwidth of 10.9 MHz to match the linewidths of atomic transitions. The source also produces single mode photon pairs at a rate of 47.5 Hz without mode filters reducing loss in the system. This novel design enables research and applications in the quantum realm using hybrid light-matter interactions.