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arXiv:1505.05414 · Optics Express

Superradiance of a subwavelength array of classical nonlinear emitters

Nikita E. Nefedkin, E. S. Andrianov, A. A. Zyablovsky, A. A. Pukhov, A. V. Dorofeenko, A. P. Vinogradov, A. A. Lisyansky

Published Feb 10, 2016• 7 citations
arXivHTMLPDF

Abstract

We suggest a mechanism by which a superradiant burst emerges from a subwavelength array of nonlinear classical emitters that are not initially synchronized. The emitters interact via the field of their common radiative response. We show that only if the distribution of initial phases is not uniform does a non-zero field of radiative response arise, leading to a superradiant burst. Although this field cannot synchronize the emitters, it engenders long period envelopes for their fast oscillations. Constructive interference in the envelopes of several emitters creates a large fluctuation in dipole moments that results in a superradiant pulse. The intensity of this pulse is proportional to the square of the number of emitters participating in the fluctuation.

DOI
10.1364/oe.24.003464

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We suggest a mechanism by which a superradiant burst emerges from a subwavelength array of nonlinear classical emitters that are not initially synchronized. The emitters interact via the field of their common radiative response. We show that only if the distribution of initial phases is not uniform does a non-zero field of radiative response arise, leading to a superradiant burst. Although this field cannot synchronize the emitters, it engenders long period envelopes for their fast oscillations. Constructive interference in the envelopes of several emitters creates a large fluctuation in dipole moments that results in a superradiant pulse. The intensity of this pulse is proportional to the square of the number of emitters participating in the fluctuation.
In 1954, Dicke predicted that a system of quantum emitters confined to a subwavelength volume would produce a superradiant burst. For such a burst to occur, the emitters must be in the special Dicke state with zero dipole moment. We show that a superradiant burst may also arise for non-Dicke initial states with a nonzero dipole moment. Both for Dicke and non-Dicke initial states, superradiance arises due to a decrease in the dispersion of the quantum phase of the emitter state. For non-Dicke states, the quantum phase is related to the phase of long-period envelopes which modulate the oscillations of the dipole moments. A decrease in the dispersion of the quantum phase causes a decrease in the dispersion of envelope phases that results in constructive interference of the envelopes and the superradiant burst.
Ordered atomic arrays with subwavelength lattice spacing emit light collectively. For fully inverted atomic arrays, this results in an initial burst of radiation and a fast buildup of coherences between the atoms at initial times. Based on a cumulant expansion of the equations of motion, we derive exact analytical expressions for the emission properties and numerically analyze the full many-body problem resulting in the collective decay process for unprecedented system sizes of up to a few hundred atoms. We benchmark the cumulant expansion approach and show that it correctly captures the cooperative dynamics resulting in superradiance. For fully inverted arrays, this allows us to extract the scaling of the superradiant peak with particle number. For partially excited arrays where no coherences are shared among atoms, we also determine the critical number of excitations required for the emergence of superradiance in one- and two-dimensional geometries. In addition, we study the robustness of superradiance in the case of non-unit filling and position disorder.
Photon-mediated interactions within an excited ensemble of emitters can result in Dicke superradiance, where the emission rate is greatly enhanced, manifesting as a high-intensity burst at short times. The superradiant burst is most commonly observed in systems with long-range interactions between the emitters, although the minimal interaction range remains unknown. Here, we put forward a new theoretical method to bound the maximum emission rate by upper bounding the spectral radius of an auxiliary Hamiltonian. We harness this tool to prove that for an arbitrary ordered array with only nearest-neighbor interactions in all dimensions, a superradiant burst is not physically observable. We show that Dicke superradiance requires minimally the inclusion of next-nearest-neighbor interactions. For exponentially decaying interactions, the critical coupling is found to be asymptotically independent of the number of emitters in all dimensions, thereby defining the threshold interaction range where the collective enhancement balances out the decoherence effects. Our findings provide key physical insights to the understanding of collective decay in many-body quantum systems, and the designing of superradiant emission in physical systems for applications such as energy harvesting and quantum sensing.
Fully-excited two-level atoms separated by less than the transition wavelength cooperatively emit light in a short burst, a phenomenon called superradiance by R. Dicke in 1954. The burst is characterized by a maximum intensity scaling with the square of the number of atoms NNN and a temporal width reduced by NNN compared to the single atom spontaneous decay time. Both effects are usually attributed to a synchronization of the electric dipole moments of the atoms occurring during the process of light emission. Contrary to this explanation, it was recently shown by use of a quantum path description that the peak intensity results from the quantum correlations among the atoms when occupying symmetric Dicke states. Here we investigate from this perspective the temporal evolution of the ensemble, starting in the small sample limit, i.e., when the atoms have mutual separations much smaller than the transition wavelength λλλ and pass down the ladder of symmetric Dicke states. In addition, we explore the temporal evolution for the case of non-interacting atoms with mutual separations much larger than λλλ. We show that in this case a similar superradiant burst of the emitted radiation is observed if the quantum correlations of the atoms are generated by conditional photon measurements retaining the atomic ensemble within or close to the symmetric subspace.
Superradiant burst often arises from photon-mediated interactions within an excited ensemble of emitters, where collective emission leads to a sharp increase in photon intensity. Here, we focus on a nuclear ensemble with cooperative excitations and propose, for the first time, the generation of superradiant burst of x-ray photons. We establish the required excitation conditions to observe x-ray superradiant bursts, offering guidance for the experiments utilizing state-of-the-art x-ray sources. Building on this, we investigate the dynamics of the x-ray superradiant burst and reveal novel nonlinear relationships between the time required to reach the peak intensity and the excitation number, as well as between the peak intensity and the excitation number. Additionally, we introduce a dimensionless parameter that serves as an indicator of the system, reflecting how strongly the burst can occur in a given configuration. Our work provides fresh insights into the understanding of collective emission in many-body x-ray-nuclei systems within the nonlinear regime, opening new avenues for x-ray quantum optics.
In contrast to free space, in waveguides the dispersive and dissipative dipole–dipole interactions among quantum emitters exhibit a periodic behavior over remarkably long distances. We propose a novel setup, to our knowledge, exploiting this long-range periodicity in order to create highly excited subradiant states and facilitate fast controlled collective energy transport among far-apart ensembles coupled to a waveguide. For sufficiently large ensembles, collective superradiant emission into the fiber modes dominates over its free space counterpart. We show that, for a large number of emitters, a fast transverse coherent pulse can create almost perfect subradiant states with up to 50% excitation. On the other hand, for a coherent excitation of one sub-ensemble above an overall excitation fraction of 50% we find a nearly lossless and fast energy transfer to the ground state sub-ensemble. This transport can be enhanced or suppressed by controlling the positions of the ensembles relative to each other, while it can also be realized with a random position distribution. In the optimally enhanced case this fast transfer appears as superradiant emission with subsequent superabsorption, yet, without a superradiant decay after the absorption. The highly excited subradiant states, as well as the superradiant excitation transfer, appear as suitable building blocks in applications such as active atomic clocks, quantum batteries, quantum information protocols, and quantum metrology procedures such as fiber-based Ramsey schemes.