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arXiv:1505.04779 · Optics Communications

Time-resolved UV–IR pump-stimulated emission pump spectroscopy to probe collisional relaxation of the 8p2P3/2 state of Cs I

Mohammed Salahuddin, Phillip T. Arndt, Jacob McFarland, Servet Bayram

Published Sep 16, 2015• 0 citations
arXivHTMLPDF
DOI
10.1016/j.optcom.2015.07.088

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Time-resolved UV-IR Pump-stimulated Emission Pump Spectroscopy: Probing Collisional Relaxation of 8p2P3/28p^{2}P_{3/2}8p2P3/2​ Cs I
Measurements of hyperfine polarization quantum beats are used to determine the magnetic dipole (A) and electric quadrupole (B) coupling constants in the excited atomic Cs 8p2P3/28p{\phantom{\rule{0.16em}{0ex}}}^{2}{P}_{3/2}8p2P3/2​ level. The experimental approach is a combination of pulsed optical pumping and time-delayed stimulated-emission probing of the excited level. From the measured evolution of the atomic linear polarization degree as a function of probe delay time, we determine the hyperfine coupling constants A=7.42(6)A=7.42(6)A=7.42(6) MHz and B=0.14(29)B=0.14(29)B=0.14(29) MHz.