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arXiv:1502.04450 · New Journal of Physics

Spontaneous four-wave mixing in liquid-core fibers: towards fibered Raman-free correlated photon sources

Margaux Barbier, Isabelle Zaquine, Philippe Delaye

Published May 20, 2015• 38 citations
arXivHTMLPDF

Abstract

We experimentally demonstrate, for the first time to our knowledge, the generation of correlated photon pairs in a liquid-core photonic crystal fiber. Moreover, we show that, thanks to the specific Raman properties of liquids, the Raman noise (which is the main limitation of the performance of silica-core fiber-based correlated photon pair sources) is highly reduced. With a demonstrated coincident-to-accidental ratio equal to 63 and a pair generation efficiency of about 10 −4 per pump pulse, this work contributes to the development of high-quality correlated photon pair sources for quantum communications.

DOI
10.1088/1367-2630/17/5/053031

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We experimentally demonstrate, for the first time to our knowledge, the generation of correlated photon pairs in a liquid-core photonic crystal fiber. Moreover, we show that, thanks to the specific Raman properties of liquids, the Raman noise (which is the main limitation of the performance of silica-core fiber-based correlated photon pair sources) is highly reduced. With a demonstrated coincident-to-accidental ratio equal to 63 and a pair generation efficiency of about 10 −4 per pump pulse, this work contributes to the development of high-quality correlated photon pair sources for quantum communications.
Weexperimentally demonstrate, for the first time to our knowledge, the generation of correlated photon pairs in a liquid-core photonic crystalfiber.Moreover, we show that, thanks to the specific Raman properties of liquids, the Ramannoise (which is themain limitation of the performance of silica-core fiber-based correlated photon pair sources) is highly reduced.With a demonstrated coincident-to-accidental ratio equal to 63 and a pair generation efficiency of about 10 per pump pulse, this work contributes to the development of high-quality correlated photon pair sources for quantumcommunications.
We demonstrate greatly improved results for the production of correlated photon-pairs using the four-photon scattering process in silica fiber. We achieve a true-coincidence-count to accidental-coincidence-count ratio greater than 10, when the photon-pair production rate is about 0.04 /pulse. This represents a four-fold improvement over our previous results. The contribution of spontaneous Raman scattering, the primary cause of uncorrelated photons that degrades the fidelity of this source, is reduced by decreasing the wavelength detuning between the correlated photons and the pump photons and by using polarizers to remove the cross-polarized Raman-scattered photons. Excess Raman scattering could be further suppressed by cooling the silica fiber. Even without cooling the fiber, the achieved 10 to 1 ratio of true-coincidence to accidental-coincidence makes the fiber source of correlated photon-pairs a useful tool for realizing various quantum-communication protocols.
Fibered sources of photon pairs can be easily integrated into future quantum communication networks. However, in silica-core fibres, the broadband spectrum of spontaneous Raman scattering strongly contributes to uncorrelated noise photons degrading the quality of the source. To overcome the problem of the silica Raman scattering, a new architecture was recently proposed, with hollow-core photonic crystal fibers (LF-HCPF) whose core and cladding are filled with a non-linear liquid. As opposed to the Raman scattering spectrum of silica, which is broadband and continuous, the Raman scattering spectrum of liquids is composed of narrow lines. Thus, generating photon pairs between these narrow lines permits to avoid the spectral overlap between the SFWM pairs and the Raman photons. A near infra-red LF-HCPCF photon pair source has been demonstrated, featuring a three order of magnitude suppression of the Raman noise [1]. We have also demonstrated the first non-linear LF-PCF with a transmission band and a zero-dispersion-wavelength (ZDW) in the telecom wavelength range combined with a non-linearity of the same order of magnitude as the one of silica, as a first step towards a Raman-free photon pair source in the telecom band [2]. Injecting light on both sides of this fiber in a Sagnac loop configuration can then be used to obtain entanglement.
Raman-scattering noise in silica has been the key obstacle toward the realisation of high quality fiber-based photon-pair sources. Here, we experimentally demonstrate how to get past this limitation by dispersion tailoring a xenon-filled hollow-core photonic crystal fiber. The source operates at room temperature, and is designed to generate Raman-free photon-pairs at useful wavelength ranges, with idler in the telecom, and signal in the visible range. We achieve a coincidence-to-accidentals ratio as high as 2740 combined with an ultra low heralded second order coherence [Formula: see text], indicating a very high signal to noise ratio and a negligible multi-photon emission probability. Moreover, by gas-pressure tuning, we demonstrate the control of photon frequencies over a range as large as 13 THz, covering S-C and L telecom band for the idler photon. This work demonstrates that hollow-core photonic crystal fiber is an excellent platform to design high quality photon-pair sources, and could play a driving role in the emerging quantum technology.
Sources of photon pairs based on spontaneous four-wave mixing in silica fibers are generally considered limited by the spectrally broad spontaneous Raman scattering noise. I experimentally show that fluorescence from native or residual doping defects in silica fibers can become preponderant in situations where Raman scattering is normally eliminated, revealing a new, to the best of my knowledge, source of noise in silica-fiber-based sources of pairs of photons. I show that this noise depends on the fiber used, and that a new parameter must be carefully surveyed for the optimization of a fibered source of entangled pairs of photons.